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Journal of Experimental and Theoretical Physics

Single-atom laser: Coherent and nonclassical effects in the regime of a strong atom-field correlation

S. Ya. Kilin, T. B. Karlovich

Published Nov 1, 2002• 39 citations
Publisher

Abstract

Based on the approximation of strong correlations between an atom and an intracavity field, which implies the equal probabilities of finding the atom in the ground state and n photons in the field and of finding the atom in an excited state and n −1 photons in the field, it is shown that the conditional states of a field generated by a single-atom laser are described by the diagonal part of the generalized coherent Mittag-Leffler state. The quasi-distributions P and Q of the intracavity-field probability amplitude are found, and the boundedness of the Glauber function on a segment is shown. The possibility of inversionless lasing is demonstrated, and the absence of a lasing threshold is found for some region of parameters. The regimes of generation of the amplitude-squeezed states of the field are studied and the parameters of the system providing the maximum squeezing are determined. It is shown that the atom-field states are entangled at weak pump intensities.

DOI
10.1134/1.1528672

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Based on the approximation of strong correlations between an atom and an intracavity field, which implies the equal probabilities of finding the atom in the ground state and n photons in the field and of finding the atom in an excited state and n −1 photons in the field, it is shown that the conditional states of a field generated by a single-atom laser are described by the diagonal part of the generalized coherent Mittag-Leffler state. The quasi-distributions P and Q of the intracavity-field probability amplitude are found, and the boundedness of the Glauber function on a segment is shown. The possibility of inversionless lasing is demonstrated, and the absence of a lasing threshold is found for some region of parameters. The regimes of generation of the amplitude-squeezed states of the field are studied and the parameters of the system providing the maximum squeezing are determined. It is shown that the atom-field states are entangled at weak pump intensities.
Properties of a laser formed by a high-Q cavity and a single incoherently excited atom are studied on the basis of analytical solutions obtained for the quasi-probability P -function. Expressions for the boundaries separating various operating regimes of a one-atom laser (below threshold, above threshold, and self-quenching) are found. It is shown that lasing without inversion and lasing with the decay rate of the excited state exceeding the pump intensity are possible in the system. The degree of coherence of laser radiation is studied.
Although conventional lasers operate with a large number of intracavity atoms, the lasing properties of a single atom in a resonant cavity have been theoretically investigated for more than a decade. Here we report the experimental realization of such a one-atom laser operated in a regime of strong coupling. Our experiment exploits recent advances in cavity quantum electrodynamics that allow one atom to be isolated in an optical cavity in a regime for which one photon is sufficient to saturate the atomic transition. In this regime the observed characteristics of the atom-cavity system are qualitatively different from those of the familiar many atom case. Specifically, we present measurements of intracavity photon number versus pump intensity that exhibit "thresholdless" behavior, and infer that the output flux from the cavity mode exceeds that from atomic fluorescence by more than tenfold. Observations of the second-order intensity correlation function demonstrate that our one-atom laser generates manifestly nonclassical light that exhibits both photon antibunching and sub-Poissonian photon statistics.
The statistical properties of fluorescent light from a single two-level atom driven by nonclassical light beams that exhibit antibunching and squeezing are discussed in the weak-field limit. The fields produced in intracavity second-harmonic generation and those produced by superposing the light from a degenerate parametric oscillator with a coherent field are considered to be the models of nonclassical light beams. These fields can be described in terms of real Gaussian random processes with nonzero mean coherent components. Analytical expressions for the fluorescent light intensity, the second-order intensity correlation function, and the variance of the photon number in the steady state are obtained. The effects of driving-field correlations, detuning, and other parameters characterizing the atom-field interaction on the statistics of scattered light are investigated. It is found that for a certain range of parameters the second-order intensity correlation function may vanish at nonzero times. Under certain other circumstances the antibunching of the fluorescent photons is enhanced. These and other interesting features that appear in the scattered light are discussed.
We consider a laser model consisting of a single four-level or three-level atom, an optical cavity, and an incoherent pump. Results for photon statistics for varying pump levels are obtained using a quantum trajectory algorithm. In particular, we calculate the mean photon number, Fano factor (which is the variance over the mean). We examine that the behavior of the single-atom device as \ensuremath{\beta}, the fraction of spontaneous emission into the lasing mode, is varied. Typical values considered for \ensuremath{\beta} are $0.01<\ensuremath{\beta}<1.0.$ We find that for large enough \ensuremath{\beta}, lasing action, with properties similar to those predicted by semiclassical theories that factorize atom-field correlations and use a small-noise approximation, can occur. Squeezing can occur as \ensuremath{\beta} is increased. There is no evidence of a sharp phase transition from weakly excited thermal light to coherent light at a particular pump power. This is consistent with work on many-atom lasers with \ensuremath{\beta} values in the range considered here. As \ensuremath{\beta} is increased, the output goes from quasithermal light to coherent and finally to squeezed light, progressing into a fully quantum-mechanical regime. We also consider the effects of cavity damping and spontaneous emission rates on these results.
Light emitted from laser-driven atoms often has squeezed quadrature fluctuations reflecting the phase dependence of the atomic source excited into a coherent superposition by the driving field. In this paper, we study the maximum squeezing in the emitted light fields from three-level atoms, paying particular attention to the role of atomic coherences in governing the optimum squeezing which is possible. Some phase dependent nonlinear optical processes have the potential for substantial quantum noise reduction at useful intensities: for example, four-wave mixing involving atomic systems has already been used to generate quadrature-squeezed light. The threoretical description of such a source is generally complicated with damping processes, coherent and incoherent pumping, and so on, all needing to be taken into account. Fully quantum treatments are available, but the basic physics of the process is often difficult to grasp in the necessarily complicated analysis. Although less important from the point of view of efficient practical sources of squeezed light, studying the generation of squeezed light in simpler systems such as two- or three-level atoms interacting with one or two modes (as in Jaynes-Cummings models) or in spontaneous emission or resonance fluorescence gives greater insight into the fundamentals of the squeezing process. In particular, the relationship between the atomic coherences and the degree of squeezing in the generated fields can be explored. We study the maximum (optimized) squeezing that can be obtained in the emitted fields from the irreversible decay from three-level atoms for any choice of initial conditions, excitations and decay process, for all quadrature components and for all possible configurations (V, \ensuremath{\Lambda}, and ``ladder'' systems).We show that for V and \ensuremath{\Lambda} systems, optimum squeezing is actually associated with a two-level state (in a suitable basis) involving a single one-photon coherence, but for ladder systems the state for maximum noise reduction is not equivalent to a two-level system and involves a single two-photon coherence and no intermediate state population. We pay particular attention to whether the total field is in a minimum uncertainty state, and the nature of the atomic state associated with maximum squeezing, especially whether it is a mixed or pure state. In the case where the initial free field has a zero amplitude at the detector and the source atoms are confined to a region small compared to the wavelength (Dicke source) we show that the squeezing in the total field is given in terms of the squeezing in the source field, and hence related to atomic populations and atomic one-photon and two-photon coherences for the case of three level atom. Previously unconsidered source-free field interferences terms are shown to be zero. The choice of quadrature phase and frequency is optimized to minimize the source field normally ordered variance. We then minimize further with respect to the choice of atomic density matrix elements subject to the constraints that the density matrix is Hermitean, positive, and has a trace equal to unity. In all cases we find that the optimum squeezing is produced when the source field is in a minimum uncertainty state.
Our recent paper reports the experimental realization of a one-atom laser in a regime of strong coupling [J. McKeever, A. Boca, A. D. Boozer, J. R. Buck, and H. J. Kimble, Nature (London) 425, 268 (2003)]. Here we provide the supporting theoretical analysis relevant to the operating regime of our experiment. By way of a simplified four-state model, we investigate the passage from the domain of conventional laser theory into the regime of strong coupling for a single intracavity atom pumped by coherent external fields. The four-state model is also employed to exhibit the vacuum-Rabi splitting and to calculate the optical spectrum. We next extend this model to incorporate the relevant Zeeman hyperfine states as well as a simple description of the pumping processes in the presence of polarization gradients and atomic motion. This extended model is employed to make quantitative comparisons with our earlier measurements for the intracavity photon number versus pump strength and for the photon statistics as expressed by the intensity correlation function ${g}^{(2)}(\ensuremath{\tau})$.