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Optics Letters

Spin relaxation of optically trapped atoms by light scattering

Robert A. Cline, Joseph D. Miller, M. R. Matthews, Daniel J. Heinzen

Published Feb 1, 1994• 90 citations
Publisher

Abstract

We study spin relaxation of optically trapped atoms that is due to light scattering from the trap laser. We observe relaxation times greater than 2 s for ground-state hyperfine-level populations of 85Rb atoms trapped in an optical dipole force trap operating as much as 65 nm to the red of the D1 line. The measured relaxation rate can be more than 100 times slower than the atoms’ total spontaneous scatter rate from the trap laser. This enhancement in atomic ground-state lifetime is due to an interference effect in spontaneous Raman scattering far from atomic resonance.

DOI
10.1364/ol.19.000207

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arXiv:physics/0409146•Journal of Optics B Quantum and Semiclassical Optics•Jul 11, 2005•18 citations
We study spin relaxation of optically trapped atoms that is due to light scattering from the trap laser. We observe relaxation times greater than 2 s for ground-state hyperfine-level populations of 85Rb atoms trapped in an optical dipole force trap operating as much as 65 nm to the red of the D1 line. The measured relaxation rate can be more than 100 times slower than the atoms’ total spontaneous scatter rate from the trap laser. This enhancement in atomic ground-state lifetime is due to an interference effect in spontaneous Raman scattering far from atomic resonance.
We study a novel property of light scattering by Rb atoms confined in a far off-resonance optical dipole force trap. The trapping laser wavelength varies from 780 nm to 860 nm and its intensity is about 1 MW/cm{sup 2}. Spontaneous Raman scattering of photons from the trapping laser can change the ground-state hyperfine quantum number F of the atoms. We observe the relaxation time by measuring the population of the F=3 level after optically pumping the atoms into the F=2 level. Spontaneous photon scatter rates as low as 10{sup 3} s{sup -1} have been observed, corresponding to recoil heating rates below 1 mK/s. For detuning from resonance {Delta} greater than the excited-state fine-structure splitting the total scatter rate, including Rayleigh scattering, decreases as {Delta}{sup 2} while the spontaneous Raman scatter rate decreases as {Delta}{sup 4}. This is due to interference between the Raman scattering amplitudes from the two excited-state fine-structure levels in the Kramers-Heisenberg formula. Because Rayleigh scattering dominates, the atoms` F and M{sub F} quantum numbers are preserved even after many scattering events. This makes far off-resonance optical traps ideal for studies of state-selective collisions and collective phenomena.
A scheme to trap atoms in a blue-detuned optical dipole trap, formed with a single laser beam and a holographic phase plate, is demonstrated. 105{10}^{5}105 rubidium atoms are trapped for (1/e lifetime) \ensuremath{\sim}300 msec, at temperatures of \ensuremath{\sim}24 \ensuremath{\mu}K and a density of $\ensuremath{\sim}7\ifmmode\times\else\texttimes\fi{}{10}^{11}{\mathrm{a}\mathrm{t}\mathrm{o}\mathrm{m}\mathrm{s}/\mathrm{c}\mathrm{m}}^{3},$ for a trapping beam detuning of 0.1--30 nm. The time for a trapped atom to scatter one photon off the trapping beam is measured and found to be linear in the trapping laser detuning. At a detuning of 0.5 nm from resonance this time was measured to be \ensuremath{\sim}100 msec, indicating that the atoms are exposed on average only to \ensuremath{\sim}1/700 of the maximal light intensity in the trap. The use of a single laser beam allows for simple dynamical changes of the potential and large adiabatic compressions, while keeping the atoms mainly in the dark.
We have confined up to 10{sup 4} {sup 85}Rb atoms in an optical dipole force trap operating up to 65 nm from atomic resonance. For detunings greater than 16 nm, we obtained long confinement times, limited only by background gas collisions, without additional cooling. However, for trapping laser tunings between 4 nm and 16 nm to the red of the lowest Rb (D1) resonance, we observed a novel trap loss mechanism which results in much shorter-trap lifetimes. The trap loss rate is very sensitive to the laser wavelength, and exhibits a complex spectrum. This trap loss may arise from a photo-associative collisional process in which an initially free pair of colliding ground state atoms is promoted to a bound molecular excited state. The bound excited molecule could then be lost from the trap by photoionization, or by spontaneous decay to an untrapped ground state. The results of our preliminary experiments and of further experiments to clarify this novel trap loss process will be presented.
We confine 85Rb^{85}\mathrm{Rb}85Rb atoms in an optical dipole force trap with a very large detuning from resonance of up to 65 nm. Confinement times of 200 ms, limited only by background-gas collisions, are obtained without additional cooling. A typical trap contains 1300 atoms at a temperature of 0.4 mK and a peak density of 8\ifmmode\times\else\texttimes\fi{}1011{10}^{11}1011 ${\mathrm{cm}}^{\mathrm{\ensuremath{-}}3}$. We measure spontaneous photon scatter rates of the trapped atoms to be less than 1.6\ifmmode\times\else\texttimes\fi{}103{10}^{3}103 ${\mathrm{s}}^{\mathrm{\ensuremath{-}}1}$, corresponding to recoil heating rates below 0.6 mK/s. The far-detuned trap confines atoms with a strong, nearly conservative optical force and negligible atomic excitation.
Optical dipole traps can provide strong, state-independent confinement of atoms. Unfortunately, the spatially dependent light shifts of optical transitions in dipole traps can interfere with conventional laser cooling techniques. These limitations may be overcome by cooling trapped atoms with stimulated Raman transitions. In particular, the lights shifts of ground state sublevels can be equal, so that the Raman cooling transition is unperturbed. Cooling in the sideband limit, to the quantum ground state of motion, should be possible. We have confined {sup 85}Rb atoms in a far-detuned optical dipole trap, and indirectly measured extremely low heating rates of the trapped atoms. We have also driven velocity-sensitive stimulated Raman transitions of the trapped atoms. The high resolution of these stimulated Raman resonances should allow us to resolve the motional sidebands and to directly cool the trapped atoms.
We perform spectroscopy on the hyperfine splitting of 85^{85}85Rb atoms trapped in far-off-resonance optical traps. The existence of a spatially dependent shift in the energy levels is shown to induce an inherent dephasing effect, which causes a broadening of the spectroscopic line and hence an inhomogeneous loss of atomic coherence at a much faster rate than the homogeneous one caused by spontaneous photon scattering. We present here a number of approaches for reducing this inhomogeneous broadening, based on trap geometry, additional laser fields, and novel microwave pulse sequences. We then show how hyperfine spectroscopy can be used to study quantum dynamics of optically trapped atoms.