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Journal of Physics A Mathematical and Theoretical

Exactly soluble two-state quantum models with linear couplings

Boyan T. Torosov, Nikolay V. Vitanov

Published Apr 2, 2008• 18 citations
Publisher

Abstract

A class of exact analytic solutions of the time-dependent Schrödinger equation is presented for a two-state quantum system coherently driven by a nonresonant external field. The coupling is a linear function of time with a finite duration and the detuning is constant. Four special models are considered in detail, namely the shark, double-shark, tent and zigzag models. The exact solution is derived by rotation of the Landau–Zener propagator at an angle of π/4 and is expressed in terms of Weber's parabolic cylinder function. Approximations for the transition probabilities are derived for all four models by using the asymptotics of the Weber function; these approximations demonstrate various effects of physical interest for each model.

DOI
10.1088/1751-8113/41/15/155309

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A class of exact analytic solutions of the time-dependent Schrödinger equation is presented for a two-state quantum system coherently driven by a nonresonant external field. The coupling is a linear function of time with a finite duration and the detuning is constant. Four special models are considered in detail, namely the shark, double-shark, tent and zigzag models. The exact solution is derived by rotation of the Landau–Zener propagator at an angle of π/4 and is expressed in terms of Weber's parabolic cylinder function. Approximations for the transition probabilities are derived for all four models by using the asymptotics of the Weber function; these approximations demonstrate various effects of physical interest for each model.
We present an analytically exactly solvable two-state quantum model, in which the coupling has a hyperbolic-tangent temporal shape and the frequency detuning is constant. The exact solution is expressed in terms of associated Legendre functions. An interesting feature of this model is that the excitation probability does not vanish, except for zero pulse area or zero detuning; this feature is attributed to the asymmetric pulse shape. Two limiting cases are considered. When the coupling rises very slowly, it is nearly linear and the tanh model reduces to the shark model introduced earlier. When the coupling rises very quickly, the tanh model reduces to the Rabi model, which assumes a rectangular pulse shape and hence a sudden switch on. Because of its practical significance, we have elaborated the asymptotics of the solution in the Rabi limit, and we have derived the next terms in the asymptotic expansion, which deliver the corrections to the amplitude and the phase of the Rabi oscillations due to the finite rise time of the coupling.
An exact analytic solution to the time-dependent Schrödinger equation is presented for a two-state quantum system coherently driven by a nonresonant pulsed external field. The pulse has a hyperbolic-secant shape, with a sign jump (i.e. a phase step of π) at its maximum, which nullifies the overall pulse area. It is shown that off resonance, for detunings larger than the pulse bandwidth, the transition probability approaches unity as the field intensity increases. The population inversion is robust against small-to-moderate variations in the detuning and the intensity, a feature reminiscent of adiabatic passage. The population inversion, however, is not of adiabatic nature; it is induced by δ-function-shaped nonadiabatic coupling with an area of nearly π. An estimate of the required experimental resources shows that implementation with shaped femtosecond pulses is feasible.
Exact solution to the driven quantum system with an explicitly time-dependent Hamiltonian is not only an issue of fundamental importance to quantum mechanics itself, but also a ubiquitous problem in the design for quantum control. In particular, the nonadiabatic transition induced by the time-dependent external field is often involved in order to target the quantum state for the atomic and molecular systems. In this paper we investigate the exact dynamics and the associated nonadiabatic transition in a typical driven model, the Rosen-Zener model and its multi-level extension, by virtue of the algebraic dynamical method. Previously, this kind of driven models, especially of the two-level case, were solved by converting the corresponding Schrödinger equation to a hypergeometric equation. The property of the dynamical transition of the system was then achieved by the asymptotic behavior of the yielded hypergeometric function. A critical drawback related to such methods is that they are very hard to be developed so as to treat the multi-level extension of the driven model. Differing from the above mentioned method, we demonstrate that the particular kind of the Rosen-Zener model introduced here could be solved analytically via a canonical transformation or a gauge transformation approach. In comparison, we show that the present method at least has two aspects of advantages. Firstly, the method enables one to describe the evolution of the wavefunction of the system analytically over any time interval of the pulse duration. Moreover, we show that the method could be exploited to deal with the multi-level extensions of the model. The explicit expression of the dynamical basis states, including the three-level system and the four-level system, is presented and the transition probabilities induced by the nonadiabatic evolution among different levels are then characterized for the model during the time evolution. In addition, our study reveals further that the dual model of the driven system can be constructed. Since the dynamical invariant of a solvable system can always be obtained within the framework of the algebraic dynamical method, the general connection between the dual model and the original one, including the solvability and their dynamical invariants, are established and characterized distinctly.
This work presents an analytic description of the coherent excitation of a two-state quantum system by an external field with a Lorentzian temporal shape and a constant frequency. An exact analytical solution for the differential equation of the model is derived in terms of Confluent Heun functions. Also a very accurate analytic approximation to the transition probability is derived by using the Dykhne-Davis-Pechukas approach. This approximation provides analytic expressions for the frequency and amplitude of the probability oscillations.
The non-stationary Schrödinger equation in a finite basis of states is considered for the Hamiltonian matrix linearly depending on time. Exact analytical solutions of asymptotic transition probabilities are obtained for a bow-tie model, in which an arbitrary number of linear time-dependent diabatic potential curves cross at one point and only a particular horizontal curve has interactions with the others. Based on the contour integral method used, some mathematical aspects such as a possible generalization of the Whittaker functions are also briefly discussed.
Exact analytical solutions to the dissipative time-dependent Schrödinger equation are obtained for a decaying two-state system with decay rates Γ1 and Γ2 for the levels with extremal spin projections. The system is coherently driven with a pulse whose detuning is made up of two parts: a time-dependent part (chirp) of hyperbolic-tangent shape and a static part with real and imaginary terms. This gives us a wide range of possibilities to arbitrarily select the interaction terms. We considered two versions which led to decaying Demkov-Kunike (DK) models; the version in which the Rabi frequency (interaction) is a time-dependent hyperbolic-secant function (called decaying DK1 model) and the case when it is constant in time and never turns off (decaying DK2 model). Our analytical solutions account for all possible initial moments instead of only t0 = 0 or t0 = − ∞ as for non-decaying models and may be useful for the experiments on level crossings. Two complementary limits of the pulse detuning are considered and explored: the limit of fast (i) and slow rise (ii). In the case (i), the coupling between level positions in the first DK model collapses, while the second DK model reduces to a Rabi model (constant Hamiltonian), in the case (ii), both DK models reduce to the LZ model. In both cases (i) and (ii), analytical approximated solutions which conveniently approach the exact solutions are derived.