Manipulating Entanglement with atoms and photons in a box

S. Haroche

S. Haroche

Introduction: about quanta, atoms, photons, and cats Experiments which manipulate and study isolated quantum systems have come of age. We can now trap single atoms or photons in a box, entangle them together, observe directly their quantum jumps, and realize in this way some of the thought-experiments imagined by the founding fathers of quantum physics. Schrödinger, who believed that observing an atom so to speak in vivo would remain forever impossible (Schrödinger 1952), would have been amazed, could he have seen what experimenters now achieve by manipulating atoms with lasers. These experiments are not just textbook illustrations of quantum concepts. They are considered by many as first steps towards harnessing the quantum world and realizing classically impossible tasks A quantum computer, for instance, would be a machine using quantum interference effects at a macroscopic scale in order to perform massive parallelism in computation (Nielsen and Chuang 2000). It would achieve an exponential speed-up to solve some problems such as the factoring of large numbers (Shor 1994). Such a machine would manipulate large ensembles of “quantum bits” made of atoms, molecules, or photons. Each bit would evolve in a superposition of two states labeled as “0” and “1”. These bits would be entangled together by quantum gates exploiting electromagnetic interactions between them. The behavior of this machine would be strange and counterintuitive. It would be a system made of thousands of two-level particles following during the calculation a huge number of different routes among which it remains coherently suspended.

Hacker, B., Stephan Welte, Daiss, S. +4 more

Quantum physics allows for entanglement between microscopic and macroscopic objects, described by discrete and continuous variables, respectively. As in Schrödinger's famous cat gedanken experiment, a box enclosing the objects can keep the entanglement alive. For applications in quantum information processing, however, it is essential to access the objects and manipulate them with suitable quantum tools. Here we reach this goal and deterministically generate entangled light-matter states by reflecting a coherent light pulse with up to four photons on average from an optical cavity containing one atom. The quantum light propagates freely and reaches a remote receiver for quantum state tomography. We produce a plethora of quantum states and observe negative-valued Wigner functions, a characteristic sign of non-classicality. As a first application, we demonstrate a quantum-logic gate between an atom and a light pulse, with the photonic qubit encoded in the phase of the light field.

S. Haroche

Wenyu Jiang, Gregory Armstrong, Lulu Han +10 more

Multiphoton light-matter interactions invoke a so-called "black box" in which the experimental observations contain the quantum interference between multiple pathways. Here, we employ polarization-controlled attosecond photoelectron metrology with a partial wave manipulator to deduce the pathway interference within this quantum 'black box" for the two-photon ionization of neon atoms. The angle-dependent and attosecond time-resolved photoelectron spectra are measured across a broad energy range. Two-photon phase shifts for each partial wave are reconstructed through the comprehensive analysis of these photoelectron spectra. We resolve the quantum interference between the degenerate p→d→p and p→s→p two-photon ionization pathways, in agreement with our theoretical simulations. Our approach thus provides an attosecond time-resolved microscope to look inside the "black box" of pathway interference in ultrafast dynamics of atoms, molecules, and condensed matter.

Dik Bouwmeester