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Physical Review Letters

Phase Transfer in Time-Delayed Interferometry with Nuclear Resonant Scattering

Yuji Hasegawa, Yoshitaka Yoda, Koichi Izumi, Tetsuya Ishikawa, S. Kikuta, X. W. Zhang, Masami Ando

Published Sep 11, 1995• 13 citations
Publisher

Abstract

In x-ray interferometry accompanying nuclear resonant scattering with some time delay, interference was observed under the condition that a phase shifter was set in front of a nuclear scatterer. The observed interference pattern clarified that the phase information is transferred to the reemitted beam through the intermediate state in nuclear resonance. A storing of phase information in time-delayed scattering is discussed in a system consisting of a quantized radiation field combined with a nucleus state.

DOI
10.1103/physrevlett.75.2216

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In x-ray interferometry accompanying nuclear resonant scattering with some time delay, interference was observed under the condition that a phase shifter was set in front of a nuclear scatterer. The observed interference pattern clarified that the phase information is transferred to the reemitted beam through the intermediate state in nuclear resonance. A storing of phase information in time-delayed scattering is discussed in a system consisting of a quantized radiation field combined with a nucleus state.
The time-delayed scattering in 14.4 keV Mossbauer resonance at 57 Fe has been intensively studied using pulsed synchrotron radiation source and delayed coincidence technique. Here, results of x-ray interferometric experiments are shown, which were obtained at KEK with this nuclear resonance. There, the interference arises from the beams re-emitted by different nuclei with some time interval after the absorption of a single incident photon. High visibility interference oscillations verified the coherent superposition as well as the complete coincidence in the time domain of the beams after the nuclear resonance. The collective nuclear excitations from a single photon are discussed with regard to the no-reduction of the detection probability. In addition, the phase information transfer in successive absorption and re-emission with time-delay, and the dispersion effect at the nuclear resonance are shown.
The temporal dynamics of stimulated emission is studied, with particular emphasis on stimulated emission induced by x-ray pulses interacting with nuclei. In typical nuclear forward scattering experiments, the short incident x-ray pulse is accompanied by a huge number of off-resonant background photons. This prompts the question of whether stimulated emission can be observed in the delayed nuclear scattering signal which is emitted after the incident pulse has passed. We find that the stimulated photons essentially overlap with the stimulating pulse. To overcome this problem, we identify the reduction of the delayed scattered light intensity as an alternative signature for the stimulated emission. We further study a phase-sensitive variant of stimulated emission in the low-excitation regime, which provides convenient control parameters to facilitate the detection. Finally, we analyze the possibility of observing stimulated emission in nuclei driven by free electron lasers or synchrotron radiation sources.
The so-called gamma-echo effect has been observed experimentally and analyzed using the semiclassical optical theory. Here the effect is reinterpreted using a new 1D quantum mechanical model. This leads to a different interpretation of the effect as a π phase-shift induced transparency. In the basic time-differential Mössbauer spectroscopic technique the forward-scattered recoil-free radiation is observed, in delayed coincidence, after passing through a nuclear-resonant absorber. The effect in question is produced most efficiently when the source of recoil-free radiation is moved abruptly causing a π phase shift of the source radiation during its radiative lifetime. Using the 1D model the effect is seen to arise from the constructive interference between the source radiation at a later time, and the radiation coming from the absorber excited at an earlier time. The exact form of the source modulation and the nuclear-resonant thickness of the resonant absorber determines the shape of the time-differential resonant gamma ray transmission spectrum. Numerical results are given using the familiar 57Fe recoil-free resonant transition. The π phase-shift-induced transparency allows the resonant gamma radiation, incident on the resonant absorber, to be transmitted through the absorber without appreciable attenuation.
A quantum-eraser setup exploiting the time-energy complementarity relation in the x-ray regime is investigated theoretically. The starting point is the interference process between x-ray quanta driving two nuclear hyperfine transitions in a nuclear forward-scattering setup. We show that which-way information can be obtained by marking the scattering paths with orthogonal polarization states, thus leading to the disappearance of the interference pattern. In turn, erasure of the which-way information leads to the reappearance of the interference fringes. We put forward two schemes using resonant scattering off nuclear targets and design which-way marking procedures to realize the quantum-eraser setup for x-ray quanta.
Means to coherently control single x-ray photons in resonant scattering of light off nuclei by electric or magnetic fields are investigated theoretically. In order to derive the time response in nuclear forward scattering, we adapt the Maxwell–Bloch equations known from quantum optics to describe the resonant light pulse propagation through a nuclear medium. Two types of time-dependent perturbations of nuclear forward scattering are considered for coherent control of the resonantly scattered x-ray quanta. Firstly, the simultaneous coherent propagation of two pulses through the nuclear sample is addressed. We find that the signal of a weak pulse can be enhanced or suppressed by a stronger pulse simultaneously propagating through the sample in counter-propagating geometry. Secondly, the effect of a time-dependent hyperfine splitting is investigated and we put forward a scheme that allows parts of the spectrum to be shifted forward in time. This is the inverse effect of coherent photon storage and may become a valuable technique if single x-ray photon wavepackets are to become the information carriers in future photonic circuits.