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Physical Review Letters

Optical bistability and photon statistics in cavity quantum electrodynamics

Gerhard Rempe, Robert J. Thompson, Robert J. Brecha, W. D. Lee, Harry J. Kimble

Published Sep 23, 1991• 345 citations
Publisher

Abstract

The quantum statistical behavior of a small collection of N two-state atoms strongly coupled to the field of a high-finessse optical cavity is investigated. Input-output characteristics are recorded over the range 3\ensuremath{\lesssim}N\ensuremath{\lesssim}65, with bistability observed for N\ensuremath{\gtrsim}15 intracavity atoms and for a saturation photon number ${\mathit{n}}_{0}$\ensuremath{\simeq}0.8. For weak excitation the transmitted field exhibits photon antibunching as a nonclassical manifestation of state reduction and quantum interference with the magnitude of the nonclassical effects largely independent of N.

DOI
10.1103/physrevlett.67.1727

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Annual Meeting Optical Society of America•Jan 1, 1990•0 citations
The quantum statistical behavior of a small collection of N two-state atoms strongly coupled to the field of a high-finessse optical cavity is investigated. Input-output characteristics are recorded over the range 3\ensuremath{\lesssim}N\ensuremath{\lesssim}65, with bistability observed for N\ensuremath{\gtrsim}15 intracavity atoms and for a saturation photon number n0{\mathit{n}}_{0}n0​\ensuremath{\simeq}0.8. For weak excitation the transmitted field exhibits photon antibunching as a nonclassical manifestation of state reduction and quantum interference with the magnitude of the nonclassical effects largely independent of N.
For the most part, quantum statistical processes in quantum optics are investigated in a weak-coupling regime, but it has become possible recently to realize experimentally optical systems for which the internal coupling coefficient g is comparable to the external dissipative rates. Within, this context, the subject of our investigation is the quantum dynamical processes for a small collection of N two-state atoms strongly coupled to a single mode of a high-finesse optical cavity. For this system, we record input-output characteristics for steady-state operation with 3 ⪝ N ⪝ 65 intracavity atoms and observe optical bistability for N⪞15 atoms.1
The radiative properties of atoms inside an optical cavity can be dramatically changed with respect to those in free space. In the strong-coupling limit, the reversible dipole interaction between an atom and the cavity field dominates the irreversible decay resulting from spontaneous emission and cavity damping. In this limit the atom and field can no longer be regarded as separate quantities but instead form a composite dynamic system. To enhance the dipole coupling constant and increase the photon storage time, our experiments are performed with a small cavity 1 mm long, with a finesse of 8 × 104. On average, 0.4 photons are sufficient to saturate the resonance transition at 852 nm for the cesium atoms used, while the cooperativity parameter for a single atom is 2. Optical bistability is studied in this system over the range 3 < N < 65 atoms inside the cavity, with the semiclassical theory predicting bistability for N > 5. We report observations of manifestly quantum effects in this regime, including photon antibunching and sub-Poissonian photon statistics, with the magnitude of these nonclassical effects observed to be largely independent of the number of intracavity atoms.
We investigate the photon statistics of the light transmitted from a driven optical cavity containing N two-level atoms, with emphasis on the weak driving field limit. This limit is of most interest from the point of view of quantum fluctuations. We find that various types of nonclassical behavior are possible, even with large numbers of atoms in the cavity, under conditions of strong atom-field coupling, which we refer to as the cavity quantum electrodynamics limit. We describe the system with a pure-state formalism valid for weak fields, and also use a Fokker-Planck equation obtained by a small fluctuation linearization. We examine the conditions under which the linearized theory is appropriate, and explore the sensitivity of nonclassical effects in the system to atom number, transit-time broadening, and detunings.
A tutorial review is given on recent experiments performed with 1 ⩽ N ⩽ 110 atoms in a microscopic high-finesse optical cavity. The resonator has length 1 mm and finesse 80 000. The radiative properties of the strongly coupled atom-cavity system differ from those of the individual components. For example, spontaneous emission is reversible, the first excited state of the composite system splits into two levels and the intensity fluctuations of the light transmitted by the resonator are nonclassical. We observe photon-antibunching and sub-Poissonian photon statistics. In terms of practical applications, the system renders possible ( i ) the detection of single atoms with high sensitivity and ( ii ) optical bistability for a few atoms and photons only.
While for the most part quantum statistical processes in quantum optics are investigated in a weak-coupling regime, it has recently become possible to realize experimentally systems for which the internal coupling coefficient g is comparable to the external dissipative rates. Within this context the subject of our investigation is the quantum dynamical processes for a collection of N two-state atoms strongly coupled to a single mode of a high finesse optical cavity. Our particular system consists of a collection of N~20 Cesium atoms (6S 1/2, f = 4– > 6P 3/2, f = 5 transition at 852 nm) interacting with the TEMoo mode of a spherical mirror cavity of finesse 4 × 104. Of principal importance are the single atom cooperativity parameter C1 = g 2/κγ and the saturation photon number no = g2/8γ 2, where (κ,γ) are the cavity and atomic decay rates. For our system, c1~1 and n0~0.5. In measurements of the joint probability of photoelectric detection we observe photon antibunching and sub-Poissonian photon statistics.1,2 An interpretation of our results in terms of quantum state reduction and interference in a dissipative dynamical setting is presented.2 We emphasize the decisive role played by the quantum fluctuations of a single atom (c1~1), which can result in a field of large variance even in the presence of N>1 atoms.
We present analytic results for the photon statistics of a weakly driven optical cavity containing N two-level atoms. The second-order intensity correlation function g(2)() is calculated in the weak field limit for arbitrary atomic and cavity loss rates, and cavity and atomic detunings are included. The transmitted light field may exhibit photon antibunching, sub-Poissonian photon statistics, and other novel nonclassical effects.1,2 The size of these effects depends principally on the single-atom coupling constant C1 = g2/κγ, so these effects persist with many atoms in the cavity. Our results can be interpreted via the collapse of the wave function and quantum interference of probability amplitudes. These phenomena can also be understood in terms of the self-homodyning of the driving field with squeezed polarization fluctuations.2