Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Journal of Modern Optics

Resonant nonlinearity enhancement in rubidium vapor with additional optical pumping

N. Korneev, Y.M. Torres, Chrystian Gutiérrez Parra, Yolanda Maya Ortega

Published May 14, 2014• 0 citations
Publisher

Abstract

We investigate the enhancement of characteristic nonlinear phase shift in warm rubidium vapor for a signal beam using an additional pump laser at different frequency. A numerical model based on density matrix formalism is used. Experimental results of self-rotation and diffraction in a three-wave mixing process as well as beam amplification are shown. For 87Rb transition D2 line with Fg = 1, the nonlinearity to absorption ratio can be enhanced approximately two times with a pump beam tuned at Fg = 2 transition in a co-propagating scheme, which produces strong nonlinear interaction for Fg = 1 line at signal beam powers of ~10 mW.

DOI
10.1080/09500340.2014.917730

Related papers

Resonant four-wave mixing with co-propagating scheme in rubidium vapor cell

Taek Jeong, Han Seb Moon

We have observed four-wave mixing (FWM) of weak pumping in a resonance double-Λ system for the 5S1/2- 5P1/2transition of87Rb atoms. When three beams (CPT1, CPT2 and pump) were co-propagated in the double-Λ configuration composed of the common excited state 5P1/2(Fe=2) and the two ground state 5S1/2(Fg=1 and 2), we directly measured the generated FWM signal filtering the three beams using polarizer and etalon filters. The spectral width of FWM signal was measured to be ~10 kHz under the condition of coherent population trapping (CPT). Dependence of FWM signals on the intensities of the two beams related CPT and pump beam was investigated in detail.

Conference on Lasers and Electro-Optics Pacific Rim (CLEO-PR)•Aug 1, 2015•0 citations

Three Resonant Nonlinear Optical Processes In Atomic Cesium.

Arlee V. Smith

We have investigated three resonant nonlinear processes in atomic cesium vapor. They are third harmonic generation, two photon absorption, and parametric frequency conversion. Resonant enhancement of each is provided by tuning the ruby laser half the 6S - 9D transition frequency of 28828.90 cm. The parametric process involves, in addition, a resonance with one of the P states. We have studied the variation of each of the three processes with laser intensity and frequency. At exact resonance the THG is found to be proportional to the square of the laser intensity and the TPA is proportional to laser intensity over a large power range. The resonance lineshape for both processes is found to be power dependent. A detailed analysis of these two processes based on steady state density matrix calculations and including A. C. Stark shifts, photoionization, and beam geometry is shown to accurately describe most of our observations.

•Jan 1, 1977•0 citations

Destruction of darkness: Optical coherence effects and multi-wave mixing in rubidium vapor

Alexander S. Zibrov

We describe several novel experimental effects resulting from optical coherences in multilevel atoms driven with coherent laser fields. Four configurations were explored using Rb vapor cells: lambda dark-line resonances, single beam double-lambda oscillations, and cascade two-photon transitions in co- and counter-propagating geometries. Experiments were performed with high spectral-resolution using low-power diode lasers sources and optically thick cells. Two of the most striking effects we observed are: (1) a self-oscillation that occurs at 3.0 GHz on the 85Rb hyperfine frequency when a single laser field pumps the atoms, and (2) a coherent blue-beam emission that we observe in the co-propagating cascade two-photon case. These phenomena lead to complex lineshapes, and the effects sometimes dominate the well-known 3-level coherence effects. Additional higher-order mixing or cascaded interferences are apparent in all four experimental configurations. Many of these can be viewed as multi-wave mixing enhanced by optical coherences around closed-loop paths of atomic energy levels. The effects are particularly strong when four-photon closed-loop paths with resonant energy levels are possible, as in, the double-lambda system or as a four-wave mixing “box.”

AIP conference proceedings•Jan 1, 2001•4 citations

Study of four-wave mixing in the femtosecond laser pulse propagation near the resonance rubidium doublet

A. A. Preobrazhenskaya, Д. Ю. Преображенский, A. A. Pastor +1 more

In this paper, we investigated the coherent degenerate and nondegenerate four-wave interaction in the propagation of a femtosecond laser pulse in atomic rubidium vapor. In the case of degenerate four-wave interaction, the mechanism for optical switching in an optically dense resonant medium is considered. The third-order nonlinear interaction of the laser beams intersecting in the cell at a small angle leads to a nonlinear response in the form of a fourth beam, which occurs as a result of the interaction between the two pump beams and the third signal laser beam.

Russian Journal of Physical Chemistry B•Jul 1, 2015•0 citations

Vortex-beam-induced lensing of off-resonance probe beam in Rb vapor

Andrew G. Truscott, M. E. J. Friese, Halina H. Rubinsztein-Dunlop +1 more

Summary form only given.We investigate nonlinear optical effects in an atomic gas with a LG/sub 03/ donut beam. The LG/sub 03/ donut beam was produced with a Ti:sapphire laser using a computer-generated hologram. The nonlinear medium was Rb atomic vapor in a cylindrical Pyrex cell 10 cm long and 2.5 cm in diameter, heated to approximately 120 C. The power of the donut beam at the cell window was 450 mW. By tuning the laser frequency close to the Rb atomic D/sub 2/ line at 780.1 nm, we obtained resonant enhancement of the nonlinearity. As the laser frequency was tuned through the Rb D/sub 2/ line, we could monitor self-focusing and defocusing on either side of the atomic transition.

Conference on Lasers and Electro-Optics•Nov 27, 2002•0 citations

Experimental study on laser pattern formation by strong nonlinear effects in rubidium atomic hot vapor

Guoxing Lu, Wei Dong, Haixia Chen +4 more

There are abundant nonlinear effects in atomic vapor. In this paper, the phenomenon of laser breaking up into filaments is studied in the near-resonant rubidium atomic vapor,which is induced by the strong nonlinear Kerr effect. When the continuous-wave laser beam with transverse Gaussian distribution passes through the atomic vapor, the pattern arising from the coherent superposition of the diffraction patterns of filaments is observed. We also investigated the influence on the mode pattern by input power of laser, the temperature of the vapor cell and the frequency detuning of pump light. Due to the hyperfine structure of rubidium atoms, the four-wave mixing effect exists in hot rubidium atomic vapor, which is related to the third-order nonlinear effect closely. The Raman gain of the Stokes and anti-Stokes photons is observed by scanning the frequency of the probe beam.

Acta Physica Sinica•Jan 1, 2008•0 citations
We investigate the enhancement of characteristic nonlinear phase shift in warm rubidium vapor for a signal beam using an additional pump laser at different frequency. A numerical model based on density matrix formalism is used. Experimental results of self-rotation and diffraction in a three-wave mixing process as well as beam amplification are shown. For 87Rb transition D2 line with Fg = 1, the nonlinearity to absorption ratio can be enhanced approximately two times with a pump beam tuned at Fg = 2 transition in a co-propagating scheme, which produces strong nonlinear interaction for Fg = 1 line at signal beam powers of ~10 mW.
We have observed four-wave mixing (FWM) of weak pumping in a resonance double-Λ system for the 5S1/2- 5P1/2transition of87Rb atoms. When three beams (CPT1, CPT2 and pump) were co-propagated in the double-Λ configuration composed of the common excited state 5P1/2(Fe=2) and the two ground state 5S1/2(Fg=1 and 2), we directly measured the generated FWM signal filtering the three beams using polarizer and etalon filters. The spectral width of FWM signal was measured to be ~10 kHz under the condition of coherent population trapping (CPT). Dependence of FWM signals on the intensities of the two beams related CPT and pump beam was investigated in detail.
We have investigated three resonant nonlinear processes in atomic cesium vapor. They are third harmonic generation, two photon absorption, and parametric frequency conversion. Resonant enhancement of each is provided by tuning the ruby laser half the 6S - 9D transition frequency of 28828.90 cm. The parametric process involves, in addition, a resonance with one of the P states. We have studied the variation of each of the three processes with laser intensity and frequency. At exact resonance the THG is found to be proportional to the square of the laser intensity and the TPA is proportional to laser intensity over a large power range. The resonance lineshape for both processes is found to be power dependent. A detailed analysis of these two processes based on steady state density matrix calculations and including A. C. Stark shifts, photoionization, and beam geometry is shown to accurately describe most of our observations.
We describe several novel experimental effects resulting from optical coherences in multilevel atoms driven with coherent laser fields. Four configurations were explored using Rb vapor cells: lambda dark-line resonances, single beam double-lambda oscillations, and cascade two-photon transitions in co- and counter-propagating geometries. Experiments were performed with high spectral-resolution using low-power diode lasers sources and optically thick cells. Two of the most striking effects we observed are: (1) a self-oscillation that occurs at 3.0 GHz on the 85Rb hyperfine frequency when a single laser field pumps the atoms, and (2) a coherent blue-beam emission that we observe in the co-propagating cascade two-photon case. These phenomena lead to complex lineshapes, and the effects sometimes dominate the well-known 3-level coherence effects. Additional higher-order mixing or cascaded interferences are apparent in all four experimental configurations. Many of these can be viewed as multi-wave mixing enhanced by optical coherences around closed-loop paths of atomic energy levels. The effects are particularly strong when four-photon closed-loop paths with resonant energy levels are possible, as in, the double-lambda system or as a four-wave mixing “box.”
In this paper, we investigated the coherent degenerate and nondegenerate four-wave interaction in the propagation of a femtosecond laser pulse in atomic rubidium vapor. In the case of degenerate four-wave interaction, the mechanism for optical switching in an optically dense resonant medium is considered. The third-order nonlinear interaction of the laser beams intersecting in the cell at a small angle leads to a nonlinear response in the form of a fourth beam, which occurs as a result of the interaction between the two pump beams and the third signal laser beam.
Summary form only given.We investigate nonlinear optical effects in an atomic gas with a LG/sub 03/ donut beam. The LG/sub 03/ donut beam was produced with a Ti:sapphire laser using a computer-generated hologram. The nonlinear medium was Rb atomic vapor in a cylindrical Pyrex cell 10 cm long and 2.5 cm in diameter, heated to approximately 120 C. The power of the donut beam at the cell window was 450 mW. By tuning the laser frequency close to the Rb atomic D/sub 2/ line at 780.1 nm, we obtained resonant enhancement of the nonlinearity. As the laser frequency was tuned through the Rb D/sub 2/ line, we could monitor self-focusing and defocusing on either side of the atomic transition.
There are abundant nonlinear effects in atomic vapor. In this paper, the phenomenon of laser breaking up into filaments is studied in the near-resonant rubidium atomic vapor,which is induced by the strong nonlinear Kerr effect. When the continuous-wave laser beam with transverse Gaussian distribution passes through the atomic vapor, the pattern arising from the coherent superposition of the diffraction patterns of filaments is observed. We also investigated the influence on the mode pattern by input power of laser, the temperature of the vapor cell and the frequency detuning of pump light. Due to the hyperfine structure of rubidium atoms, the four-wave mixing effect exists in hot rubidium atomic vapor, which is related to the third-order nonlinear effect closely. The Raman gain of the Stokes and anti-Stokes photons is observed by scanning the frequency of the probe beam.