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Optics Communications

Influence of atomic recoil on power broadened lineshapes in 2-level atoms

Philip Hemmer, F.Y. Wu, Shaoul Ezekiel

Published Jul 1, 1981• 12 citations
Publisher
DOI
10.1016/0030-4018(81)90209-1

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Journal of Physics A Mathematical and General•Apr 1, 1977•12 citations
Previously derived equations describing recoil effects in saturated absorption by a gas of two-level atoms or molecules are solved numerically for the case of standing plane-wave excitation and large Doppler broadening. The numerical techniques and accuracy estimates are discussed briefly. The lineshapes obtained are well approximated by the superposition of two Lorentzian functions whose width, heights, and separation parametrise the lineshape. The dependence of these parameters on saturation, recoil splitting, and relaxation rates is described and compared with corresponding results in the rate equation approximation and in the weak-probe-beam approximation. Saturation broadening depends strongly on these latter approximations, but very little on recoil splitting. When multiphoton processes are retained in the equations, increasing saturation causes a slight decrease in the fitted separation of the peaks. The ratio of the heights of the two Lorentzians is closely related to the ratio of relaxation rates for the level populations.
In the framework of the Jaynes–Cummings model, we investigate how atomic lineshapes are affected by coherently driving the atom–field interaction. We pay particular attention to the two-level atom interaction with a thermal cavity field when both are influenced by external classical fields. Adopting a density matrix formalism, we calculate the average atomic inversion and demonstrate how the corresponding lineshapes vary as a function of the average number of thermal photons and the atom–field classical coupling. Furthermore, we compare these results with those obtained from the standard Jaynes–Cummings model and validate our findings through numerical calculations.
The problem of saturated absorption by a gas of two-level molecules, including recoil effects, is formulated in a new quantum representation for the molecular motion. The relationship to other representations is clarified in a simple chart. The new formulation requires the solution of simultaneous linear differential equations with mixed boundary conditions, instead of linear difference equations in two variables followed by an integration over velocity. Analytic solutions are presented for one running wave with Doppler line broadening, and for a weak probe beam in the Doppler limit. The latter lineshape is analysed to show when power broadening obscures the recoil splitting.