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Physical Review Letters

Nonclassical States: An Observable Criterion

W. Vogel

Published Feb 28, 2000• 139 citations
Publisher

Abstract

An observable criterion is derived that allows one to distinguish nonclassical states of the harmonic oscillator from those having a classical counterpart. A quantum state is shown to have no classical counterpart if and only if the characteristic functions of the quadrature distributions or the s-parametrized phase-space distributions exhibit a slower decay than for the ground state of the oscillator. This renders it possible to experimentally check the failure of the P function to be a probability measure.

DOI
10.1103/physrevlett.84.1849

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An observable criterion is derived that allows one to distinguish nonclassical states of the harmonic oscillator from those having a classical counterpart. A quantum state is shown to have no classical counterpart if and only if the characteristic functions of the quadrature distributions or the s-parametrized phase-space distributions exhibit a slower decay than for the ground state of the oscillator. This renders it possible to experimentally check the failure of the P function to be a probability measure.
Necessary and sufficient conditions are derived that allow one to completely characterize the nonclassicality of an arbitrary quantum state of a harmonic oscillator. Starting from a theorem by Bochner we derive an infinite hierarchy of conditions for the characteristic functions of the quantum state. Following the hierarchy step by step, the nonclassicality can be classified with respect to increasing orders. The full hierarchy of conditions is completely equivalent to the most commonly accepted criterion for nonclassicality: the failure of the Glauber–Sudarshan P -function to be a probability density. Our reformulated version of the criterion is directly related to measurable quantities that can be observed in phase-sensitive measurements such as homodyne detection. It directly generalizes a criterion for nonclassicality (Vogel 2000 Phys. Rev. Lett. 84 1849) that has already been applied in experiments (Lvovsky and Shapiro 2002 Phys. Rev. A 65 033830). Examples of phase-insensitive quantum states are considered that exhibit no first-order nonclassical effects, but that are nonclassical in second order.
Criteria for the nonclassicality of a quantum state of the harmonic oscillator are formulated in terms of normally ordered moments of quadratures. Inequalities are obtained that are equivalent to the failure of the Glauber-Sudarshan PPP function to be a probability density. A possibility to measure the required moments is proposed.
The characterization of nonclassicality of quantum states in terms of measurable quadrature distributions is studied, on the basis of recently derived necessary and sufficient conditions for the failure of the Glauber–Sudarshan P -function to be a probability density. When the noise-subtracted quadrature distribution, that is the marginal of the P -function, is not a probability density, the same is true for the Glauber–Sudarshan P -function. Inversely, for a complete characterization of a nonclassical P -function one needs phase-sensitive criteria that connect quadrature distributions for different phases. Even for phase-insensitive quantum states, phase-sensitive nonclassicality conditions are needed, as is illustrated for one-photon added thermal states.
The definition of nonclassical states in quantum optics by the nonpositivity of their Glauber–Sudarshan quasiprobability is investigated and it is shown that it hides some serious problems. It leads to a subdivision of squeezed thermal states into classical and nonclassical states which is difficult to interpret physically by some qualitatively different behaviour of the states. Nonclassical states are found in arbitrarily small neighbourhoods of every classical state that is illustrated by a very artificial modified thermal state. The observability of the criterion in comparison to that for nonclassicality of states determined by the nearest Hilbert–Schmidt distance to a class of reference states is discussed. The behaviour of the nonclassicality of states in models of phase-insensitive processes of damping and amplification is investigated and it is found that every nonclassical state eventually makes a transition to a classical state. However, this is not specific for the negativities or singularities of the Glauber–Sudarshan quasiprobability and is found in similar form for other quasiprobabilities, for example, for the Wigner quasiprobability. We discuss in quite general form some defects of the Glauber–Sudarshan quasiprobability if compared with classical distribution functions over the phase space, in particular the failure of an earlier advertised superposition formula.
“The word ‘classical’ means only one thing in science: it's wrong!” We have previously emphasized the fact that all states of light are quantum mechanical and are thus nonclassical, deriving some quantum features from the discreteness of the photons. Of course, in practice, the nonclassical features of light are difficult to observe. (We shall use “quantum mechanical” and “nonclassical” more or less interchangeably here.) Already we have discussed what must certainly be the most nonclassical of all nonclassical states of light – the single-photon state. Yet, as we shall see, it is possible to have nonclassical states involving a very large number of photons. But we need a criterion for nonclassicality. Recall that in Chapter 5 we discussed such a criterion in terms of the quasi-probability distribution known as the P function, P (α). States for which P (α) is positive everywhere or no more singular than a delta function, are classical whereas those for which P (α) is negative or more singular than a delta function are nonclassical. We have shown, in fact, that P (α) for a coherent state is a delta function, and Hillery has shown that all other pure states of the field will have functions P (α) that are negative in some regions of phase space and are more singular than a delta. It is evident that the variety of possible nonclassical states of the field is quite large.