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Optica Acta International Journal of Optics

Amplitude Self-modulation of Intracavity Second-harmonic Generation

Paul Mandel, Thomas Erneux

Published Jan 1, 1982• 49 citations
Publisher

Abstract

We consider second-harmonic generation by a non-linear crystal placed in an empty resonant cavity and pumped by an external coherent field. It was recently predicted that the stationary state loses its stability through a Hopf bifurcation when the input intensity reaches a critical value. A new amplitude self-modulated state then arises. We construct explicitly this new time-periodic solution and prove its stability in the vicinity of the transition point. As the input intensity is further increased, numerical investigations indicate a new transition to another time-periodic solution; this transition involves an hysteresis cycle. The two periodic solutions differ by the number of maxima in one period: at low input intensity, there is one maximum per period, whereas at high input intensity there are two.

DOI
10.1080/713820743

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arXiv:0808.3122•Physical Review A•Jan 13, 2009•41 citations
We consider second-harmonic generation by a non-linear crystal placed in an empty resonant cavity and pumped by an external coherent field. It was recently predicted that the stationary state loses its stability through a Hopf bifurcation when the input intensity reaches a critical value. A new amplitude self-modulated state then arises. We construct explicitly this new time-periodic solution and prove its stability in the vicinity of the transition point. As the input intensity is further increased, numerical investigations indicate a new transition to another time-periodic solution; this transition involves an hysteresis cycle. The two periodic solutions differ by the number of maxima in one period: at low input intensity, there is one maximum per period, whereas at high input intensity there are two.
We analyse the problem of intracavity second harmonic generation to determine properties of the antiphased states that have been observed in this system. We study the time-periodic solutions by means of a perturbation expansion in powers of a small parameter which is the ratio of the cavity lifetime to the population inversion relaxation time. We prove that each mode intensity is characterized by two oscillation frequencies though the total intensity oscillates with only one of these frequencies. In first approximation, we find that the bifurcation from the steady state to the periodic state remains vertical. We resolve this singularity by a complementary numerical analysis. We show that there are at least four distinct types of antiphase dynamics, including partial clustering of the oscillating modes into subsets of antiphasing states. Finally, we analyse the scaling exponent of the oscillation amplitudes near the bifurcation point and determine that the generic 1/2 exponent is the rule for only two of four types of antiphasing. The exponents of the other two cases depend on the mode number and partition.
Second-harmonic generation (SHG) in doubly resonant optical resonators (resonant for the pump and for the harmonic wave) is a subject rich in outstanding challenges: the demonstration of self-pulsing, in which the intracavity field amplitudes undergo a Hopf bifurcation to a stable limit cycle,1 and chaos; the generation of near-perfect squeezing near but below the self-pulsing threshold; the generation of squeezed radiation in the self-pulsing regime; and the demonstration of quantum nondemolition measurements.
The interaction between two cavity resonant nonlinear processes in an intracavity ${\mathrm{\ensuremath{\chi}}}^{(2)}$ medium is studied, namely frequency doubling of a pump field of frequency ${\mathrm{\ensuremath{\omega}}}_{1}$ and subsequent down-conversion of the second harmonic to a pair of photons of frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$\ifmmode\pm\else\textpm\fi{}\ensuremath{\Delta}. A closed set of semiclassical equations of motion for appropriately chosen quantities of the full system is derived and an explicit stationary solution is given. Its features and stability are discussed, the most striking being a stable plateau in the second harmonic, i.e., the field of frequency ${\mathrm{\ensuremath{\omega}}}_{2}$=2${\mathrm{\ensuremath{\omega}}}_{1}$ becomes independent of the pump field scrE1{\mathit{scrE}}_{1}scrE1​, provided scrE1{\mathit{scrE}}_{1}scrE1​ is larger than a certain threshold value. It is demonstrated that undamped self-pulsing can only prevail, if the ratio of the rates of second harmonic generation over and parametric down-conversion exceeds a value which depends solely on the relative damping rates of the second harmonic and fundamental, which yields a tentative theoretical explanation of the experimentally observed quenching of the self-pulsing.
We consider the process of second-harmonic generation (SHG) in a cavity that is resonant for both the fundamental- and second-harmonic modes. It has been previously shown that such a system displays a phase instability leading to self-pulsing and that one gets important intensity squeezing on both the fundamental- and second-harmonic mode for pump intensities close to but below, this instability threshold. Such a squeezing has been recently observed. We have analytically calculated the intensity-noise spectrum of the frequency-doubled field above such an instability threshold, using a semiclassical input-output technique for the treatment of quantum fluctuations.1 Such a method, introduced to deal with fluctuations around a stable solution, has been generalized to the self-pulsing domain. As expected, the instability brings excess noise to the output beams, especially around the zero-frequency, the self-oscillation frequency, and its harmonics. Remarkably, some regions exist in which where the noise increase is small; squeezing still occurs in this frequency range far in the instability domain.
We consider three nonlinear optical models that display a two-photon process and exhibit a Hopf bifurcation corresponding to a phase instability. The three models describe second-harmonic generation, two-photon optical bistability, and degenerate four-wave mixing in resonant cavities. In all three cases we consider only the resonant configuration and analyze the attractors which emerge when the driving field is increased beyond the Hopf bifurcation threshold. At a finite distance from threshold, we find a hysteresis domain that involves a pair of periodic attractors. For all three models, each of the two solutions has the same ``field portrait'' i.e., the same representation in a plane whose axes are the imaginary and the real parts of the electric field. This suggests that the scenario is generic for this class of systems. On the other hand, the models for two-photon optical bistability and degenerate four-wave mixing in resonant cavities exhibit additional nongeneric attractors when the driving field is further increased.
We describe a theoretical analysis of the nonlinear dynamics of third-harmonic generation $(\ensuremath{\omega}\ensuremath{\rightarrow}3\ensuremath{\omega})$ via Kerr $({\ensuremath{\chi}}^{(3)})$ nonlinearities in a resonant cavity with resonances at both $\ensuremath{\omega}$ and $3\ensuremath{\omega}$. Such a doubly resonant cavity greatly reduces the required power for efficient harmonic generation, by a factor of $\ensuremath{\sim}V∕{Q}^{2}$, where VVV is the modal volume and QQQ is the lifetime, and can even exhibit 100% harmonic conversion efficiency at a critical input power. However, we show that it also exhibits a rich variety of nonlinear dynamics, such as multistable solutions and long-period limit cycles. We describe how to compensate for self- and cross-phase modulation (which otherwise shifts the cavity frequencies out of resonance), and how to excite the different stable solutions (and especially the high-efficiency solutions) by specially modulated input pulses.