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Journal de Physique IV (Proceedings)

4He OPTICAL PUMPING WITH POLARIZATION MODULATED LIGHT AND MAGNETOMETRY APPLICATION

H. Gilles, Bernard Cheron, J. Hamel

Published Dec 1, 1991• 3 citations
Publisher

Abstract

In optical pumping experiments using a laser, beam polarization can be modulated with the help of an electrooptic modulator device. This technique has been applied to pump 4He(23S1) metastable atoms. New resonances, never observed before, has been studied theoretically and experimentally versus geometric and modulation parameters and an application to high sensitivity magnetometer is presented.

DOI
10.1051/jp4:19917129

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In optical pumping experiments using a laser, beam polarization can be modulated with the help of an electrooptic modulator device. This technique has been applied to pump 4He(23S1) metastable atoms. New resonances, never observed before, has been studied theoretically and experimentally versus geometric and modulation parameters and an application to high sensitivity magnetometer is presented.
4^44He (2 3^33S1_11​) metastable atoms are optically pumped with intensity modulated light. The use of a single mode diode-pumped LNA laser as the pumping source, allows the study of resonance signals predicted by the optical pumping theory but not yet observed. Resonances are detected on the transmitted pumping beam at the modulation frequency and its harmonics. Application of this method to high sensitivity magnetometers is suggested.
Optical pumping experiments have been performed on helium 4 atoms in the metastable level 2 3 S 1 with the object of studying the modulation of light in absorption in the longitudinal and transverse beams. Magnetic resonance curves were obtained similar to those found in emission in double-resonance experiments. With a particular geometrical arrangement employing circular polarizers, the Bloch magnetic resonance curves were obtained. Modulation at four times the applied frequency was obtained with a linear polarizer in the pumping beam. This modulation is ascribed to the circulation of coherence in the optical pumping cycle. From the behaviour of the resonance signals as a function of the frequency and amplitude of the stimulating field, it is inferred that a substantial part of the signal arises from coherence which has survived two complete cycles. The observations are satisfactorily explained by the theory developed in the previous paper.
Recently a distributed Bragg reflection (DBR) laser diode was commercialised by SDL (USA) for helium optical pumping experiments. An interesting feature of the new device is the possibility of frequency modulation of the diode output by modulating the current intensity, leading to a new pumping scheme called optical pumping with frequency modulated light. We develop this method to induce spin precession and obtain new resonances in 4He atomic gas, simply by modulating the frequency of the pumping light at the Larmor frequency of atomic states in a static magnetic field. These resonances are analysed with a simple model taking into account velocity changing collisions.
We report a laser-pumped 4He atomic magnetometer with light shift suppression through the atomic sensor itself. A linearly polarized light is used to optically align the 4He metastable atoms and we monitor the magneto-optical double resonance (MODR) signals produced by the left- and right-circularly orthogonal components. It is shown that light shift leads to the atomic alignment to orientation conversion effect, and thus, the difference between the two MODR signals. One of these two MODR signals is locked at the Larmor frequency and is used to measure the ambient magnetic field, while the differential signal is, simultaneously, fed back to suppress the light shift. The scheme could be of the advantage to the design of compact magnetometers by reducing the systematic errors due to light shift.
We investigate the polarization modulation between two linear orthogonal states of the laser beam that synchronously pumps time-dependent atomic alignment in caesium atoms exposed to a static magnetic field. Because of the atomic alignment symmetry two independent groups of resonances can be distinguished in the transmitted light: when modulation frequency matches either the Larmor frequency or its second harmonics, ${\ensuremath{\omega}}_{L}$ and $2{\ensuremath{\omega}}_{L}$, respectively. We report on our experiments, and discuss a model that perfectly reproduces the observed spectra. We have observed that the amplitudes and linewidths of resonances at ${\ensuremath{\omega}}_{L}$ and $2{\ensuremath{\omega}}_{L}$ show magnetic-field direction dependence. This peculiar behavior makes our approach interesting for future application to atomic magnetometry, in view of a dead-zone free high-sensitivity magnetometer.
A new optical pumping scheme utilizing selective reflection is proposed and studied for the first time. This method enables us to observe the spin-polarization of atoms even at the high density, at which the pumping beam cannot be transmitted through a sample cell. Theoretical analysis shows that the light reflectivity at the glass-vapor interface is strongly dependent on the direction of the macroscopic magnetic moment of optical pumped atoms. Two types of demonstrating experiments are carried out with Cs and Rb vapors at the temperature ∼ 200°C. In the transverse pumping experiment with a modulated laser beam, asymmetry of the magnetic resonance signal with respect to the inversion of the magnetic field direction is observed as predicted by the theory. In the longitudinal pumping experiment, the transfer of a large amount of the magnetic moment by spin-exchange collisions is directly observed.