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Physical review. B, Solid state

Critical properties of random and constrained dipolar magnets

Amnon Aharony A

Published Aug 1, 1975• 40 citations
Publisher

Abstract

Renormalization-group techniques are used to study a model of $n$-coupled $m$-component spin systems, in the limit of large dipole-dipole interactions. As recently shown by Emery, this model describes the critical behavior of a constrained dipolar system in the limit $n\ensuremath{\rightarrow}\ensuremath{\infty}$ and that of a dipolar system with a quenched random perturbation in the limit $n\ensuremath{\rightarrow}0$. In both cases, the unperturbed dipolar fixed point is unstable, and there is a crossover to a new behavior. For the constrained system, this leads to another dipolar fixed point (if $\ensuremath{\alpha}<0$, $\ensuremath{\alpha}$ being the dipolar specific-heat exponent) with the same thermodynamic critical exponents, or to one with renormalized dipolar exponents (if $\ensuremath{\alpha}>0$). These results are different from those of previous "spherical" dipolar models. For the random case, the crossover is either to a new fixed point, with very different exponents, e.g., $2\ensuremath{\nu}\ensuremath{\simeq}1+1.183\ensuremath{\epsilon}$ for $m=d=4\ensuremath{-}\ensuremath{\epsilon}$, or away from all the fixed points found to order $\ensuremath{\epsilon}$. One of the new fixed points in this case has complex eigenvalues of the linearized recursion relations. This is related to the fact that the recursion-relation flow is not of a gradient type for random systems.

DOI
10.1103/physrevb.12.1049

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Annual Conference on Magnetism and Magnetic Materials (MMM)•Jan 1, 1974•7 citations
Renormalization-group techniques are used to study a model of nnn-coupled mmm-component spin systems, in the limit of large dipole-dipole interactions. As recently shown by Emery, this model describes the critical behavior of a constrained dipolar system in the limit n\ensuremath→\ensuremath∞n\ensuremath{\rightarrow}\ensuremath{\infty}n\ensuremath→\ensuremath∞ and that of a dipolar system with a quenched random perturbation in the limit n\ensuremath→0n\ensuremath{\rightarrow}0n\ensuremath→0. In both cases, the unperturbed dipolar fixed point is unstable, and there is a crossover to a new behavior. For the constrained system, this leads to another dipolar fixed point (if \ensuremathα<0\ensuremath{\alpha}<0\ensuremathα<0, \ensuremathα\ensuremath{\alpha}\ensuremathα being the dipolar specific-heat exponent) with the same thermodynamic critical exponents, or to one with renormalized dipolar exponents (if \ensuremathα>0\ensuremath{\alpha}>0\ensuremathα>0). These results are different from those of previous "spherical" dipolar models. For the random case, the crossover is either to a new fixed point, with very different exponents, e.g., 2\ensuremathν\ensuremath≃1+1.183\ensuremathϵ2\ensuremath{\nu}\ensuremath{\simeq}1+1.183\ensuremath{\epsilon}2\ensuremathν\ensuremath≃1+1.183\ensuremathϵ for m=d=4\ensuremath−\ensuremathϵm=d=4\ensuremath{-}\ensuremath{\epsilon}m=d=4\ensuremath−\ensuremathϵ, or away from all the fixed points found to order \ensuremathϵ\ensuremath{\epsilon}\ensuremathϵ. One of the new fixed points in this case has complex eigenvalues of the linearized recursion relations. This is related to the fact that the recursion-relation flow is not of a gradient type for random systems.
The exact renormalization-group approach of Wilson is used to study the critical behavior for T>TcT>{T}_{c}T>Tc​, H=0H=0H=0, and small $\ensuremath{\epsilon}>0$, of an isotropic ferromagnetic system in $d=4\ensuremath{-}\ensuremath{\epsilon}$ dimensions, with exchange and dipolar interactions between ddd-component spins. Normal isotropic Heisenberg behavior with $\frac{1}{\ensuremath{\gamma}}\ensuremath{\approx}\frac{1}{2\ensuremath{\nu}}\ensuremath{\approx}1\ensuremath{-}\frac{\ensuremath{\epsilon}}{4}$ (to first order in $\ensuremath{\epsilon}$) is retained for $t=(\frac{T}{{T}_{c}})\ensuremath{-}1\ensuremath{\ll}\frac{G}{J{a}^{d}}$, where $G=\frac{{(g{\ensuremath{\mu}}_{B})}^{2}}{2}$ measures the strength of the dipole-dipole interactions, JJJ is the short-range exchange parameter, and aaa is the lattice spacing. When ${t}^{\ensuremath{\varphi}}\ensuremath{\approx}\frac{G}{J{a}^{d}}$, where $\ensuremath{\varphi}\ensuremath{\approx}1+\frac{\ensuremath{\epsilon}}{4}$, crossover occurs to a characteristic dipolar behavior described by a new fixed point of the recursion relations. For $t\ensuremath{\ll}\frac{G}{J{a}^{d}}$ one thus finds $\frac{1}{\ensuremath{\gamma}}\ensuremath{\approx}\frac{1}{2\ensuremath{\nu}}\ensuremath{\approx}1\ensuremath{-}\frac{9\ensuremath{\epsilon}}{34}$ {and, for spins of ndn dnd components, $\frac{1}{\ensuremath{\gamma}}\ensuremath{\approx}\frac{1}{2\ensuremath{\nu}}\ensuremath{\approx}1\ensuremath{-}[\frac{(6n+3)}{2(6n+11)}]\ensuremath{\epsilon}$, which agrees with spherical-model results when $n\ensuremath{\rightarrow}\ensuremath{\infty}$}. In the dipolar regime the spin-correlation function $〈{s}_{q}^{\ensuremath{\alpha}}{s}_{\ensuremath{-}q}^{\ensuremath{\beta}}〉$ has a factor [${\ensuremath{\delta}}_{\ensuremath{\alpha}\ensuremath{\beta}}\ensuremath{-}(\frac{{q}^{\ensuremath{\alpha}}{q}^{\ensuremath{\beta}}}{{q}^{2}})$], which suppresses longitudinal spin fluctuations; the susceptibilities ${\ensuremath{\chi}}^{\ensuremath{\alpha}\ensuremath{\alpha}}$ display the expected demagnetization effects. It is found that dipolar anistropies derving from the lattice structure produce weak instabilities which should be hard to detect although their effects are not fully elucidated. Extensions of the results to nonzero magnetic fields, and to anistropic exchange interactions are indicated; the experimental situation is mentioned briefly.
In quenched random-spin systems, the renormalization group can be used to develop recursion relations for the probability distribution for random potentials. Alternatively, recursion relations for the average values of potentials and their higher cumulants can be obtained. In this paper, the above technique is used to study phase transitions in quenched random nnn-component classical spin systems using the $\ensuremath{\epsilon}$ expansion to second order in $\ensuremath{\epsilon}$. It there are long-range correlations in the random potentials (e.g., all potentials along a line are equal), there are no stable physical fixed points within the $\ensuremath{\epsilon}$ expansion. This is interpreted as a smeared transition. If there are no long-range correlations in the random potentials, there is a sharp transition with pure system exponents if the specific-heat exponent ${\ensuremath{\alpha}}^{H}$ of the pure system is negative. If ${\ensuremath{\alpha}}^{H}>0$ and n>1n>1n>1, there is a sharp transition with new exponents $\ensuremath{\eta}=[\frac{(5{n}^{2}\ensuremath{-}8n)}{256{(n\ensuremath{-}1)}^{2}}]{\ensuremath{\epsilon}}^{2}$ and $\ensuremath{\nu}=\frac{1}{2}+[\frac{3n}{32(n\ensuremath{-}1)}]\ensuremath{\epsilon}+[\frac{n(127{n}^{2}\ensuremath{-}572n\ensuremath{-}32)}{4096{(n\ensuremath{-}1)}^{3}}]{\ensuremath{\epsilon}}^{2}$. For n=1n=1n=1, there is no stable fixed point, which is again interpreted as a smeared transition.
"Renorma1ization-group methods have been applied in the study of quenched random magnetic systems in recent years. We begin with a brief review of second-order phase transitions in pure, homogeneous systems and also of the .. renorma1ization group framework. Then we provide an introduction to quenched random magnetic systems. Next, momentum-space methods and position-space techniques as applied to quenched random magnets are outlined and compared. Grinstein and Luther applied the Wilson-Fisher E-expansion to random n-vector models; Khme1'nitsky discovered that the random Ising model (n = 1) possessed a ""random"" fixed point of 0(squareroot(e)). This fixed point was found to have one marginal and one irrelevant operator. We have investigated the stability of this fixed point using Ca11an-Symanzik equations and renorma1ized perturbation theory. We find the fixed point stable in the next order; we have also obtained critical exponents to one higher order. Next, position-space techniques are used to study some simple model systems. In addition to critical exponents, global thermodynamic properties are determined. These calculations are based on the Migda1-Kadanoff approximate recursion relations suitably generalized to the inhomogeneous case. Firstly we study the randomly bond-dilute two-dimensional nearest- neighbor Ising model on a square lattice. Calculations give both thermal and magnetic exponents associated with the percolative fixed point. Differential recursion relations yield a phase diagram which is in quantitative agreement with all known results. Curves for the specific heat, percolation probability, and magnetization are displayed. The critical region of the specific heat becomes unobservably narrow well above the percolation threshold Pc. This provides a possible explanation for the apparent specific-heat rounding in certain experiments. We then study the Edwards-Anderson model of a spin glass. The current theoretical situation, which is far from satisfactory at present, is briefly reviewed. We treat the spin-l/2 Ising model with independently random nearestneighbor interactions in dimensionalities d = 2, 3, and 4. The phase diagram, which is in qualitative agreement with mean-field results, exhibits paramagnetic, ferromagnetic, antiferromagnetic, and spin-glass phases. The spinglass and paramagnetic phases meet along an extended second-order phase boundary, which terminates in two tricritical points. Critical and tricritical exponents are calculated. The spin-glass specific-heat exponent turns out to be large and negative, compatibly with recent experiments which show a rounded specific heat anomaly. Global specific-heat curves are also displayed for d = 2."
Critical behaviors in quenched random-spin systems with N-spin component are studied in the limit M → 0 of the non-random MN-component models by means of the renormalization group theory. As the static critical phenomena the stability of the fixed points is investigated and the critical exponents η[~ O(ε3); ε ≡ 4 – d], γ, α, and crossover index [Formula: see text] and the equation of state [~ O(ε)] are obtained. Within the approximation up to the order ε2, even the random-spin systems with N = 2 or 3 are unstable in the three dimensions and the pure systems are stable there.
The zero-field critical behavior of ferromagnets above Tc{T}_{c}Tc​, with both isotropic exchange coupling and dipolar interactions, is studied by renormalization-group techniques in $d=4\ensuremath{-}\ensuremath{\epsilon}$ dimensions with n(=d)n (=d)n(=d) component spins. The critical exponents are calculated to order ${\ensuremath{\epsilon}}^{2}$, and are found to be numerically very close to their nondipolar analogs. In particular the correlation length exponent is given by $2\ensuremath{\nu}=1+(\frac{9}{34})\ensuremath{\epsilon}+(\frac{7013}{58956}){\ensuremath{\epsilon}}^{2}+O({\ensuremath{\epsilon}}^{3})$. The value of the specific-heat exponent ${\ensuremath{\alpha}}_{s} (=2\ensuremath{-}d\ensuremath{\nu})$ seems inconsistent with experimental data (at d=3d=3d=3, $\ensuremath{\epsilon}=1$). The critical scattering function is shown to have the form ${\ensuremath{\Gamma}}^{\ensuremath{\alpha}\ensuremath{\beta}}(\stackrel{\ensuremath{\rightarrow}}{\mathrm{q}})=C{t}^{\ensuremath{-}\ensuremath{\gamma}}\stackrel{^}{D}({\ensuremath{\xi}}^{2}{q}^{2})({\ensuremath{\delta}}_{\ensuremath{\alpha}\ensuremath{\beta}}\ensuremath{-}\frac{{q}^{\ensuremath{\alpha}}{q}^{\ensuremath{\beta}}}{{q}^{2}})$ to all orders in $\ensuremath{\epsilon}$. The exponents related to the leading correction to scaling, to crossovers to anisotropic exchange behavior, and to cubic dipolar behavior, are also calculated, and are found to differ significantly from their nondipolar counterparts.
Studies of magnetic critical behavior using the recursion relation approach will be reviewed. For a Hamiltonian including both (anisotropic) exchange and dipole‐dipole interactions many fixed points arise, each representing distinct asymptotic critical behavior. Various non‐dipolar fixed points, for degree of isotropy m, describe the critical behavior of (rotationally invariant) antiferromagnets, except for additional, slowly decaying terms, which can lead to “effective critical exponents”. In addition one finds a series of “dipolar” fixed points. For m>1, these yield exponents which deviate slightly more from the classical values than those for the non‐dipolar fixed points. When m=1 the dipolar fixed point has classical exponents for dimension d>3, plus logarithmic corrections at d=3, but non‐classical behavior for d<3. The dipolar spin‐spin correlation functions always develop a characteristic angular dependence. Spatially anisotropic interactions, antisymmetric exchange interactions, terms of cubic symmetry, etc. may lead to still further fixed points, and hence to new critical behavior.