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Physical Review A

Motion of atoms in a radiation trap

J. P. Gordon, Arthur Ashkin

Published May 1, 1980• 585 citations
Publisher

Abstract

The force exerted by optical-frequency radiation on neutral atoms can be quite substantial, particularly in the neighborhood of an atomic resonance line. In this paper we derive from quantum theory the optical force, its first-order velocity dependence, and its fluctuations for arbitrary light intensity, and apply the results to the problem of creating a stable optical trap for sodium atoms. New results include the position dependence of the velocity-dependent force, a complete expression for the momentum diffusion constant including the substantial contribution from fluctuations of the dipole force, and an estimate of trapping times in excess of 1 sec even in the absence of effective damping. The paper concludes with a discussion of the prospects and difficulties in providing sufficient damping to stabilize such a trap.

DOI
10.1103/physreva.21.1606

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Atom traps Light forces It is well known that a light beam carries momentum and that the scattering of light by an object produces a force. This property of light was first demonstrated by Frish [139] through the observation of a very small transverse deflection (3 × 10 –5 rad) in a sodium atomic beam exposed to light from a resonance lamp. With the invention of the laser, it became easier to observe effects of this kind because the strength of the force is greatly enhanced by the use of intense and highly directional light fields, as demonstrated by Ashkin [20, 21] with the manipulation of transparent dielectric spheres suspended in water. The results obtained by Frish and Ashkin raised the possibility of using light forces to control the motion of neutral atoms. Although the understanding of light forces acting on atoms was already established by the end of the 1970s, unambiguous demonstration of atom cooling and trapping was not accomplished before the mid 1980s. In this section we discuss some fundamental aspects of light forces and schemes employed to cool and trap neutral atoms. The light force exerted on an atom can be of two types: a dissipative, spontaneous force and a conservative, dipole force. The spontaneous force arises from the impulse experienced by an atom when it absorbs or emits a quantum of photon momentum.

Cambridge University Press eBooks•Dec 4, 2003•0 citations
The force exerted by optical-frequency radiation on neutral atoms can be quite substantial, particularly in the neighborhood of an atomic resonance line. In this paper we derive from quantum theory the optical force, its first-order velocity dependence, and its fluctuations for arbitrary light intensity, and apply the results to the problem of creating a stable optical trap for sodium atoms. New results include the position dependence of the velocity-dependent force, a complete expression for the momentum diffusion constant including the substantial contribution from fluctuations of the dipole force, and an estimate of trapping times in excess of 1 sec even in the absence of effective damping. The paper concludes with a discussion of the prospects and difficulties in providing sufficient damping to stabilize such a trap.
We report on the stable effective trapping of cold rubidium atoms by a method for a single optical trap in the near-optical resonant regime. An optical trap with the near-optical resonance condition consists of not only the dipole but also the radiative forces, while a trap using a far-off resonance dominates only the dipole force. We measure the spatial behaviors of the center-of-mass positions and the loading efficiencies of the trapped atoms in the near-optical resonant trap, by changing the detuning over the range of $\ensuremath{-}0.373$ to $\ensuremath{-}2.23$ THz from the D2{\mathrm{D}}_{2}D2​ resonance. The time dependence of the spatial behavior in the trap indicates that the suitable positions for stably holding atoms are altered because the equilibrium condition between the optical dipole and the radiative forces depends on the trap laser detuning. The stable position, which is not a primary position of focus in the Gaussian beam optics, depends only on the laser detuning due to the change in the radiative force, while it is independent of the change in the laser intensity, which results in a balance between the radiative and dipole forces.
The usual form of electromagnetic forces is given by but for neutral atoms q = 0. The next order of force is the dipole term, but this also vanishes because neutral atoms have no inherent dipole moment. However, a dipole moment can be induced by a field, and this is most efficient if the field is alternating near the atomic resonance frequency. Since these frequencies are typically in the optical range, dipole moments are efficiently induced by shining nearly resonant light on the atoms. Laser cooling and trapping rely on the interaction between laser light and atoms to exert a controllable force on the atoms, and many sophisticated schemes have been developed using the special properties of the interaction. This chapter begins with the simplest schemes for exerting optical forces on atoms, namely a single-frequency light field interacting with a two-level atom. Although this is the simplest possible scheme, it is pedagogically valuable because it shows many of the features that will be encountered further on. The ultimate temperature using such a scheme is limited, but lower temperatures can be achieved with multilevel atoms. This topic is addressed later in the chapter. Two kinds of optical forces When an atom absorbs nearly resonant light, it makes a transition to the excited state, and its subsequent return to the ground state can be either by spontaneous or by stimulated emission. The nature of the optical force that arises from these two different processes is quite different, and will be described separately [1]. The spontaneous emission case is different from the familiar quantum mechanical calculations using state vectors to describe the state of the system, because spontaneous emission causes the state of the system to evolve from a pure state into a mixed state (see Exercise 6.9). Spontaneous emission is an essential ingredient for the dissipative nature of the optical forces in monochromatic light, and the density matrix is needed to describe it (see Chap. 6). When an atom absorbs light, its energy excites the atom and its angular momentum changes the electron's orbit. Both of these are internal atomic properties. However, the linear momentum of the light, can change only the external, translational motion of the atom.
The effect of field fluctuations on the motion of a two-level atom in resonant laser radiation is investigated theoretically. The internal motion of the atom is treated quantum mechanically (optical Bloch equations); the translational motion, which is coupled to the internal motion, is treated classically (Ehrenfest's theorem); and the fluctuating radiation is treated as a classical electromagnetic wave with stochastic phase (phase-diffusion model). An expression for the radiation force and equations of motion for the ensemble-averaged Bloch vector are derived and used to calculate (i) the radiation force in a plane running wave, (ii) the steady-state radiation force in a general standing wave, and (iii) the dissipative force in a plane standing wave in the limit of strong phase fluctuations. In case (iii) it is found that the atomic velocity is damped when the radiation is tuned above resonance, which is opposite to the case of a weak coherent standing wave, in which damping occurs for radiation tuned below resonance. It is shown that fluctuations have a substantial effect on the radiation force only when the spectral width of the radiation approaches or exceeds the spontaneous emission rate.
We present a simple review of the basic physical processes allowing one to control, with laser beams, the velocity and the position of neutral atoms. The control of the velocity corresponds to a cooling of atoms, that is, a reduction of the atomic velocity spread around a given value. The control of the position means a trapping of atoms in real space. The best present performances will be given, in terms of the lowest temperatures and the highest densities. The corresponding highest quantum degeneracy will also be estimated. It is imposed by fundamental limits, which will be described briefly. We also give the general trends in this field of research and outline the new directions which look promising for observing quantum statistical effects in laser cooled atomic samples, but which are for the moment restricted by unsolved problems. Introducing the Simple Schemes The radiative forces acting on atoms in a light field can be split into two parts, a reactive one and a dissipative one. The dissipative force (radiation pressure), which basically involves scattering processes, is velocity dependent. We will see that this dependence leads to the Doppler cooling scheme and to the concept of optical molasses, and we will give the corresponding minimal achievable temperature. The dissipative force can be made position dependent, through a gradient of the magnetic field, so that the atoms are also trapped in the so-called magneto-optical trap.
We demonstrate feedback on the motion of a single neutral atom trapped in the light field of a high-finesse cavity. Information on the atomic motion is obtained from the transmittance of the cavity. This is used to implement a feedback loop in analog electronics that influences the atom's motion by controlling the optical dipole force exerted by the same light that is used to observe the atom. In spite of intrinsic limitations, the time the atom stays within the cavity could be extended by almost 30% beyond that of a comparable constant-intensity dipole trap.
Atom traps Light forces It is well known that a light beam carries momentum and that the scattering of light by an object produces a force. This property of light was first demonstrated by Frish [139] through the observation of a very small transverse deflection (3 × 10 –5 rad) in a sodium atomic beam exposed to light from a resonance lamp. With the invention of the laser, it became easier to observe effects of this kind because the strength of the force is greatly enhanced by the use of intense and highly directional light fields, as demonstrated by Ashkin [20, 21] with the manipulation of transparent dielectric spheres suspended in water. The results obtained by Frish and Ashkin raised the possibility of using light forces to control the motion of neutral atoms. Although the understanding of light forces acting on atoms was already established by the end of the 1970s, unambiguous demonstration of atom cooling and trapping was not accomplished before the mid 1980s. In this section we discuss some fundamental aspects of light forces and schemes employed to cool and trap neutral atoms. The light force exerted on an atom can be of two types: a dissipative, spontaneous force and a conservative, dipole force. The spontaneous force arises from the impulse experienced by an atom when it absorbs or emits a quantum of photon momentum.