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Journal of the Optical Society of America B

Measurement of the calcium ^1P_1−^1D_2 transition rate in a laser-cooled atomic beam

N. Beverini, F. Giammanco, E. Maccioni, F. Strumia, G. Vissani

Published Nov 1, 1989• 56 citations
Publisher

Abstract

The efficiency of laser cooling in a thermal beam of calcium has been investigated under different cooling schemes. Special attention has been paid to analysis of the loss factor represented by the decay of atoms excited by the cooling laser to the 1P1 state into the metastable 1D2 level. The cooling scheme at a fixed laser frequency makes possible a good estimation of the branching ratio R between the decay probability from the 1P1 level to the ground 1S0 state and to the metastable 1D2 state. The measured value of (1.0 ± 0.15) × 105 seems high enough to produce only a small reduction in the cooling efficiency.

DOI
10.1364/josab.6.002188

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The efficiency of laser cooling in a thermal beam of calcium has been investigated under different cooling schemes. Special attention has been paid to analysis of the loss factor represented by the decay of atoms excited by the cooling laser to the 1P1 state into the metastable 1D2 level. The cooling scheme at a fixed laser frequency makes possible a good estimation of the branching ratio R between the decay probability from the 1P1 level to the ground 1S0 state and to the metastable 1D2 state. The measured value of (1.0 ± 0.15) × 105 seems high enough to produce only a small reduction in the cooling efficiency.
We report on a system for atomic beam deceleration and magneto-optical trapping of calcium atoms that uses the 1S0–1P1 transition, in which a single laser is used to trap and slow the atoms. The slower laser beam is focused near the magneto-optical trap’s center, which has a waist size much smaller than the atomic cloud such that its influence on the trapped atoms is greatly reduced. We also investigate the theoretical possibility of cooling by use of a two-photon (4s2)1S0–(4s5s)1S0 transition. Excitation near resonance with the 1P1 level results in an equilibrium temperature seven times smaller than the Doppler limit of the 1S0–1P1 transition.
The optical frequency transitions with long-lifetime spin triplet states produced by the two valence electrons in the outermost layer of alkaline earth atoms make calcium atom a promising quantum frequency reference. Electron-shelving detection improves the signal-to-noise ratio of the clock transition spectrum, enabling a calcium atomic beam optical frequency standard. This scheme employs the 1S0-1P1 transition at 423 nm to detect the 1S0-3P1 transition at 657 nm, emphasizing the importance of 423 nm laser stability. While the performance of these clocks is well-studied, research on the atomic beam itself is limited. This study investigates frequency shifts in neutral calcium atoms’ 1S0-1P1 transition at 423 nm and their 1S0-3P1 transition at 657 nm. We measure the frequency shift caused by temperature, laser power, and laser alignment, providing insights to optimize the design of the calcium beam’s physical apparatus.
Laser excitation of the 4s4p3P2−−4s3d1D24s4p {}^{3}{P}_{2} -- 4s3d {}^{1}{D}_{2}4s4p3P2​−−4s3d1D2​ transition in atomic calcium has been observed and the wavelength determined to 1530.5298(6) nm. The metastable 4s4p3P24s4p {}^{3}{P}_{2}4s4p3P2​ atoms were magnetically trapped in the quadrupole magnetic field of a magneto-optical trap. This state represents the only ``loss'' channel for the calcium atoms when laser cooled on the 4s21S0−−4s4p1P14{s}^{2} {}^{1}{S}_{0} -- 4s4p {}^{1}{P}_{1}4s21S0​−−4s4p1P1​ transition. A rate equation model shows that an order of magnitude more atoms are trapped in this state compared with those taking part in the main cooling cycle. Excitation of the 3P2{}^{3}{P}_{2}3P2​ atoms back up to the 4s3d1D24s3d {}^{1}{D}_{2}4s3d1D2​ state provides a means of accessing these atoms. Efficient repumping is achieved if the 1530-nm laser is used in conjunction with a 672-nm laser driving the 4s3d1D2−−4s5p1P14s3d {}^{1}{D}_{2} -- 4s5p {}^{1}{P}_{1}4s3d1D2​−−4s5p1P1​ transition. In the present experiment, we detected about $4.5\ifmmode\times\else\texttimes\fi{}{10}^{4}$ trapped 3P2{}^{3}{P}_{2}3P2​ atoms, a relatively low atom density, and measured a lifetime of approximately 1 s, which is limited by background collisions.
A thermal atomic beam of dysprosium atoms is cooled using the $4{f}^{10}6{s}^{2}(J=8)\ensuremath{\rightarrow}4{f}^{10}6s6p(J=9)$ transition at 421421421 nm. The cooling is done via a standing light wave orthogonal to the atomic beam. Efficient transverse cooling to the Doppler limit is demonstrated for all observable isotopes of dysprosium. Branching ratios to metastable states are demonstrated to be <<<$5\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}4}$. A scheme for enhancement of the nonzero-nuclear-spin-isotope cooling and a method for direct identification of possible trap states are proposed.