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Physical Review A

Hanle fluorescence spectra of an atom with a Jg =0⇆ Je =1 transition

Peng Zhou, S. Swain

Published Jan 1, 1997• 1 citation
Publisher

Abstract

We have investigated the two basic types of Hanle fluorescence spectra, distinguished by the direction of observation, from a V-type atom with a ${\mathrm{J}}_{\mathrm{g}}$ =0\ensuremath{\leftrightarrows}${\mathrm{J}}_{\mathrm{e}}$ =1 transition excited by a linearly polarized laser. In the absence of a magnetic field to lift the Zeeman degeneracy of the sublevels, the incoherent fluorescence spectrum ${\mathrm{G}}_{\mathrm{X}}^{\mathrm{inc}}$(\ensuremath{\omega}) is dark for all Rabi frequencies, while the incoherent fluorescence spectrum ${\mathrm{G}}_{\mathrm{Y}}^{\mathrm{inc}}$(\ensuremath{\omega}) exhibits a single peak for small Rabi frequencies and a Mollow-like triplet for large Rabi frequencies. However, if a magnetic field is applied, the incoherent spectra are composed, in general, of five peaks. When ${\mathrm{\ensuremath{\omega}}}_{\mathrm{B}}$ \ensuremath{\ll}\ensuremath{\Omega}, the incoherent spectrum ${\mathrm{G}}_{\mathrm{X}}^{\mathrm{inc}}$(\ensuremath{\omega}) has four peaks, while ${\mathrm{G}}_{\mathrm{Y}}^{\mathrm{inc}}$(\ensuremath{\omega}) has a Mollow-like triplet, and the integrated area (i.e., the fluorescence intensity) under the spectrum ${\mathrm{G}}_{\mathrm{X}}^{\mathrm{inc}}$(\ensuremath{\omega}) is much less than that of ${\mathrm{G}}_{\mathrm{Y}}^{\mathrm{inc}}$(\ensuremath{\omega}). When ${\mathrm{\ensuremath{\omega}}}_{\mathrm{B}}$ \ensuremath{\gg}:\ensuremath{\Omega}, both incoherent spectra have a two-peak structure similar to that of a two-level atom far off resonance, but the integrated area under the spectrum ${\mathrm{G}}_{\mathrm{X}}^{\mathrm{inc}}$(\ensuremath{\omega}) is much greater than that of ${\mathrm{G}}_{\mathrm{Y}}^{\mathrm{inc}}$(\ensuremath{\omega}). When ${\mathrm{\ensuremath{\omega}}}_{\mathrm{B}}$ =\ensuremath{\Omega}\ensuremath{\gg}:\ensuremath{\gamma}, both spectra have a similar five-peak structure, and the same integrated area. The results obtained are interpreted in the dressed atomic state representation. In the strong-field limit, the secular approximation is invoked, and analytical expressions of the resonance fluorescence spectra are derived which demonstrate the dependence of the peak heights and widths of the resonance fluorescence spectra on the intensities of the magnetic and linear polarized laser fields in a more transparent way.

DOI
10.1103/physreva.55.717

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Constantine Mavroyannis, K.J. Woloschuk, D. A. Hutchinson +1 more

We have numerically calculated the excitation spectra arising from the 3rd order mixing of the frequencies ωa and ωb of two laser fields interacting with a three-level atom, where each laser field resonantly couples the ground state with each excited state of the atom, respectively. In the limit of high photon densities, the excitation spectra near the reduced frequency X = (ω−ωa + 2ωb)/γ0 ≈ 0 are considered as a function of the reduced Rabi frequencies ηa and ηb of the two laser fields, respectively and γ0 is the spontaneous emission probability. For ηa < ηb the spectra consist of a doublet peaked at [Formula: see text] and its intensity is constant. When ηa = ηb, the spectra are composed of five pairs of bands peaked at [Formula: see text], and [Formula: see text]. When ηa < ηb the computed spectra consist of five pairs of bands, where the intensities of the peaks at [Formula: see text] and [Formula: see text] are positive indicating absorption, those at [Formula: see text] are negative implying amplification, and the two pairs of peaks at [Formula: see text] have positive and negative components describing the mixed process of absorption–amplification. The intensities of these bands are found to vary as (ηa/ηb)2 for (ηa/ηb) > 1 and, therefore, the intensities of the bands are immensely enhanced as the value of the ratio (ηa/ηb) increases. The computed spectra for a wide selection of Rabi frequencies are graphically presented and compared with those derived by analytical methods.

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We have investigated the two basic types of Hanle fluorescence spectra, distinguished by the direction of observation, from a V-type atom with a Jg{\mathrm{J}}_{\mathrm{g}}Jg​ =0\ensuremath{\leftrightarrows}Je{\mathrm{J}}_{\mathrm{e}}Je​ =1 transition excited by a linearly polarized laser. In the absence of a magnetic field to lift the Zeeman degeneracy of the sublevels, the incoherent fluorescence spectrum GXinc{\mathrm{G}}_{\mathrm{X}}^{\mathrm{inc}}GXinc​(\ensuremath{\omega}) is dark for all Rabi frequencies, while the incoherent fluorescence spectrum GYinc{\mathrm{G}}_{\mathrm{Y}}^{\mathrm{inc}}GYinc​(\ensuremath{\omega}) exhibits a single peak for small Rabi frequencies and a Mollow-like triplet for large Rabi frequencies. However, if a magnetic field is applied, the incoherent spectra are composed, in general, of five peaks. When \ensuremathωB{\mathrm{\ensuremath{\omega}}}_{\mathrm{B}}\ensuremathωB​ \ensuremath{\ll}\ensuremath{\Omega}, the incoherent spectrum GXinc{\mathrm{G}}_{\mathrm{X}}^{\mathrm{inc}}GXinc​(\ensuremath{\omega}) has four peaks, while GYinc{\mathrm{G}}_{\mathrm{Y}}^{\mathrm{inc}}GYinc​(\ensuremath{\omega}) has a Mollow-like triplet, and the integrated area (i.e., the fluorescence intensity) under the spectrum GXinc{\mathrm{G}}_{\mathrm{X}}^{\mathrm{inc}}GXinc​(\ensuremath{\omega}) is much less than that of GYinc{\mathrm{G}}_{\mathrm{Y}}^{\mathrm{inc}}GYinc​(\ensuremath{\omega}). When \ensuremathωB{\mathrm{\ensuremath{\omega}}}_{\mathrm{B}}\ensuremathωB​ \ensuremath{\gg}:\ensuremath{\Omega}, both incoherent spectra have a two-peak structure similar to that of a two-level atom far off resonance, but the integrated area under the spectrum GXinc{\mathrm{G}}_{\mathrm{X}}^{\mathrm{inc}}GXinc​(\ensuremath{\omega}) is much greater than that of GYinc{\mathrm{G}}_{\mathrm{Y}}^{\mathrm{inc}}GYinc​(\ensuremath{\omega}). When \ensuremathωB{\mathrm{\ensuremath{\omega}}}_{\mathrm{B}}\ensuremathωB​ =\ensuremath{\Omega}\ensuremath{\gg}:\ensuremath{\gamma}, both spectra have a similar five-peak structure, and the same integrated area. The results obtained are interpreted in the dressed atomic state representation. In the strong-field limit, the secular approximation is invoked, and analytical expressions of the resonance fluorescence spectra are derived which demonstrate the dependence of the peak heights and widths of the resonance fluorescence spectra on the intensities of the magnetic and linear polarized laser fields in a more transparent way.
We analyze the fluorescence and absorption spectra of a two-level atom driven by a bichromatic field with frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$ and ${\mathrm{\ensuremath{\omega}}}_{2}$, separated by ${\mathrm{\ensuremath{\omega}}}_{2}$-${\mathrm{\ensuremath{\omega}}}_{1}$=2\ensuremath{\delta}, and Rabi frequencies (at resonance) 2${\mathrm{\ensuremath{\Omega}}}_{1}$ and 2${\mathrm{\ensuremath{\Omega}}}_{2}$ such that their ratio \ensuremath{\alpha}=${\mathrm{\ensuremath{\Omega}}}_{2}$/${\mathrm{\ensuremath{\Omega}}}_{1}$1. We focus on the case of ${\mathrm{\ensuremath{\omega}}}_{1}$ close to the atomic frequency ${\mathrm{\ensuremath{\omega}}}_{0}$ and ${\mathrm{\ensuremath{\omega}}}_{2}$ near the Rabi sideband frequency ${\mathrm{\ensuremath{\omega}}}_{1}$+2${\mathrm{\ensuremath{\Omega}}}_{1}$; the detunings are denoted by ${\mathrm{\ensuremath{\Delta}}}_{1}$=${\mathrm{\ensuremath{\omega}}}_{0}$-${\mathrm{\ensuremath{\omega}}}_{1}$ and ${\mathrm{\ensuremath{\Delta}}}_{2}$=${\mathrm{\ensuremath{\omega}}}_{1}$+2${\mathrm{\ensuremath{\Omega}}}_{1}$-${\mathrm{\ensuremath{\omega}}}_{2}$. We find that the spectra depend critically on the detuning ${\mathrm{\ensuremath{\Delta}}}_{2}$: For large ${\mathrm{\ensuremath{\Delta}}}_{2}$, the fluorescence spectrum consists of the well known Mollow triplet, centered at ${\mathrm{\ensuremath{\omega}}}_{1}$; for smaller (but nonzero) ${\mathrm{\ensuremath{\Delta}}}_{2}$, the spectrum is composed of a triplet at ${\mathrm{\ensuremath{\omega}}}_{1}$ together with doublets near the sideband frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$\ifmmode\pm\else\textpm\fi{}2${\mathrm{\ensuremath{\Omega}}}_{1}$. However, when ${\mathrm{\ensuremath{\Delta}}}_{2}$=0 (and \ensuremath{\alpha}\ensuremath{\ll}1), the spectrum consists of a doublet centered at ${\mathrm{\ensuremath{\omega}}}_{1}$ and triplets at ${\mathrm{\ensuremath{\omega}}}_{1}$\ifmmode\pm\else\textpm\fi{}2${\mathrm{\ensuremath{\Omega}}}_{1}$: there is then no fluorescence at ${\mathrm{\ensuremath{\omega}}}_{1}$. As \ensuremath{\alpha} increases, additional triplet structures appear in the spectrum at frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$\ifmmode\pm\else\textpm\fi{}2n${\mathrm{\ensuremath{\Omega}}}_{1}$ with intensities proportional to ${\mathrm{\ensuremath{\alpha}}}^{2(\mathit{n}\mathrm{\ensuremath{-}}1)}$, n\ensuremath{\gtrsim}1, and a line reappears at ${\mathrm{\ensuremath{\omega}}}_{1}$, with intensity proportional to ${\mathrm{\ensuremath{\alpha}}}^{4}$. The absorption by the system of a weak probe beam is also strongly dependent on the detuning, and the spectrum is composed of emission-dispersion-absorption features located near ${\mathrm{\ensuremath{\omega}}}_{1}$ and ${\mathrm{\ensuremath{\omega}}}_{1}$\ifmmode\pm\else\textpm\fi{}2n${\mathrm{\ensuremath{\Omega}}}_{1}$. An analysis in the dressed-atom picture is presented which explains the physical origin of all these features, in both fluorescence and absorption. \textcopyright{} 1996 The American Physical Society.
We examine the radiative properties of a two-level atom driven by a strong bichromatic field with frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$=${\mathrm{\ensuremath{\omega}}}_{0}$-${\mathrm{\ensuremath{\delta}}}_{1}$ and ${\mathrm{\ensuremath{\omega}}}_{2}$=${\mathrm{\ensuremath{\omega}}}_{0}$+${\mathrm{\ensuremath{\delta}}}_{2}$, which can be asymmetrically placed about the atomic transition frequency ${\mathrm{\ensuremath{\omega}}}_{0}$ and can have different Rabi frequencies ${\mathrm{\ensuremath{\Omega}}}_{1}$ and ${\mathrm{\ensuremath{\Omega}}}_{2}$. Applying the optical Bloch equations for the bichromatic excitation, we derive an infinite set of equations of motion for the time evolution of the atomic variables. The equations are solved numerically by matrix inversion and Laplace transforms. Using the quantum regression theorem, we then solve for the steady-state total fluorescence intensity, and the resonance-fluorescence and absorption spectra. The spectra are found to depend on the frequency difference 2\ensuremath{\delta}=${\mathrm{\ensuremath{\delta}}}_{1}$+${\mathrm{\ensuremath{\delta}}}_{2}$, the average detuning \ensuremath{\Delta}=${\mathrm{\ensuremath{\omega}}}_{0}$-1/2(${\mathrm{\ensuremath{\omega}}}_{1}$+${\mathrm{\ensuremath{\omega}}}_{2}$), and the Rabi frequencies of the driving fields. For ${\mathrm{\ensuremath{\Omega}}}_{1}$=${\mathrm{\ensuremath{\Omega}}}_{2}$=\ensuremath{\Omega}, the total fluorescent intensity displays a series of maxima for \ensuremath{\Delta}=\ifmmode\pm\else\textpm\fi{}n\ensuremath{\delta}\ensuremath{\mp}${\mathrm{\ensuremath{\Omega}}}^{2}$/4\ensuremath{\delta}, where the n are the odd integers. The intensity-dependent shift from the resonances n\ensuremath{\delta} is explained as an analog of the generalized Bloch-Siegert shift. The resonance-fluorescence spectrum for \ensuremath{\Delta}\ensuremath{\ne}0 appears to contain more peaks than that for \ensuremath{\Delta}=0.This is due to the splitting of the central peak and the even sidebands into doublets. The absorption spectrum of a weak-probe beam for \ensuremath{\Delta}=0 and equal Rabi frequencies consists of a symmetric series of dispersionlike sidebands separated from ${\mathrm{\ensuremath{\omega}}}_{0}$ by integer multiples of \ensuremath{\delta}, together with a central absorption peak at ${\mathrm{\ensuremath{\omega}}}_{0}$, whose amplitude oscillates with \ensuremath{\Omega}. For \ensuremath{\Delta}\ensuremath{\ne}0 and/or ${\mathrm{\ensuremath{\Omega}}}_{1}$\ensuremath{\ne}${\mathrm{\ensuremath{\Omega}}}_{2}$, the odd sidebands remain dispersionlike, while the central peak and the even sidebands split into absorption-emission doublets. A simple physical interpretation of the spectral features is given in terms of the dressed-atom model.
An experiment was performed recently [Y. Zhu, A. Lezama, Q. Wu, and T. W. Mossberg (unpublished)] in which a two-level atom of transition frequency \ensuremath{\Omega} was placed in a bichromatic laser field with frequencies \ensuremath{\Omega}\ifmmode\pm\else\textpm\fi{}\ensuremath{\delta}, of sufficient intensity to produce dynamic Stark splitting. The observed fluorescence spectrum differed qualitatively in almost all its details from the well-known Mollow triplet [B. R. Mollow, Phys. Rev. 188, 1969 (1969)]. In this article, we use a dressed-atom model to explain the observed results.
We have considered the fluorescence spectra arising from the interaction of a three-level atom in the ‘‘V’’ configuration with two strong electromagnetic fields whose initially populated modes ωa and ωb are equal to the two atomic transition frequencies, respectively. The excitation spectra are calculated by making use of the Green function formalism where the hierarchy of the Green functions is truncated by a decoupling scheme which takes into account photon–photon correlations from each laser field in the limit of high photon densities. The excitation spectra consist of the central peak of the excitation frequency ωa and four pairs of sidebands, which are peaked at the frequencies ωa±η1(2)1/2, ωa±η2/(2)1/2, ωa±(η21+η22)1/2/(2)1/2, and ωa±2(η21+η22)1/2/(2)1/2, where η1 and η2 are the Rabi frequencies of the two laser fields, respectively. Similar spectra are exhibited near the excitation frequency ωb. Numerical calculations for selected values of the Rabi frequencies are graphically presented and compared with those known in the literature. In the Appendix expressions for the excitation spectra are derived first when the two laser fields are treated classically, and second, when the fields are quantized but photon–photon correlations are neglected. It is shown that when the two laser fields are treated classically, the derived results are identical to those obtained when the fields are quantized only when photon–photon correlations arising from each laser field are discarded. The derived results when the fields are quantized but without photon–photon correlations taken into account are also identical to those obtained by the use of the dressed-atom approach. The appearance of the new sidebands reveals the boson character of the photon fields in question. The merit of the method is that it yields results describing both the classical as well as the quantum nature of the photon fields involved.
We have numerically calculated the excitation spectra arising from the 3rd order mixing of the frequencies ωa and ωb of two laser fields interacting with a three-level atom, where each laser field resonantly couples the ground state with each excited state of the atom, respectively. In the limit of high photon densities, the excitation spectra near the reduced frequency X = (ω−ωa + 2ωb)/γ0 ≈ 0 are considered as a function of the reduced Rabi frequencies ηa and ηb of the two laser fields, respectively and γ0 is the spontaneous emission probability. For ηa < ηb the spectra consist of a doublet peaked at [Formula: see text] and its intensity is constant. When ηa = ηb, the spectra are composed of five pairs of bands peaked at [Formula: see text], and [Formula: see text]. When ηa < ηb the computed spectra consist of five pairs of bands, where the intensities of the peaks at [Formula: see text] and [Formula: see text] are positive indicating absorption, those at [Formula: see text] are negative implying amplification, and the two pairs of peaks at [Formula: see text] have positive and negative components describing the mixed process of absorption–amplification. The intensities of these bands are found to vary as (ηa/ηb)2 for (ηa/ηb) > 1 and, therefore, the intensities of the bands are immensely enhanced as the value of the ratio (ηa/ηb) increases. The computed spectra for a wide selection of Rabi frequencies are graphically presented and compared with those derived by analytical methods.
The calculation is given of the spectral distribution of resonance fluorescence from an atom that is driven near a j=12j=\frac{1}{2}j=21​ to j=12j=\frac{1}{2}j=21​ transition by a monochromatic, xxx-polarized electric field and that is subject to radiation damping only. In accordance with Mollow's results for a two-level system, the power spectrum of the scattered radiation corresponding to the xxx component of the dipole moment contains a coherent part for all driving-field intensities. The coherent part is absent in the fluorescence radiation corresponding to the yyy and zzz components of the dipole moment. For weak driving fields all power scattered by these latter components is present in a narrow Lorentzian. Consistent with energy conservation, the width of the Lorentzian corresponds to the probability of excitation of the atom out of its ground level due to the presence of the driving field. For strong driving fields the power spectra corresponding to the xxx component and to the yyy or zzz component mainly differ in the heights and widths of their central incoherent band and their Rabi-precession-frequency-shifted side bands.