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Physical Review A

Effects of field-induced quantum coherence on the absorptive line shape of a four-level system with three closely spaced upper levels

Saswata Ghosh, Swapan Mandal

Published Aug 19, 2004• 16 citations
Publisher

Abstract

The optical Bloch equations of a four-level atomic system with three closely spaced upper levels irradiated by a single mode of the electromagnetic radiation field are constructed. Under the rotating wave approximation and by using the slowly varying envelope approximation, we obtain the analytical solution to these optical Bloch equations. These solutions, which are obtained perturbatively, are used to calculate the polarization and hence the absorptive line shape. In particular, we examine the effects of the field-induced coherence arising from the interference between the probability amplitudes of the levels participating in dipole-allowed transitions. We obtain the shifts of the resonance peak positions due to two different reasons. The first is due to the nonlinear effects arising from the closely spaced nature of the peaks. The second is attributed to the field-induced coherence alone. It is found that the shifts of the positions of the resonance peaks due to field-induced coherence may be in the blue or in the red region.

DOI
10.1103/physreva.70.023407

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The optical Bloch equations of a four-level atomic system with three closely spaced upper levels irradiated by a single mode of the electromagnetic radiation field are constructed. Under the rotating wave approximation and by using the slowly varying envelope approximation, we obtain the analytical solution to these optical Bloch equations. These solutions, which are obtained perturbatively, are used to calculate the polarization and hence the absorptive line shape. In particular, we examine the effects of the field-induced coherence arising from the interference between the probability amplitudes of the levels participating in dipole-allowed transitions. We obtain the shifts of the resonance peak positions due to two different reasons. The first is due to the nonlinear effects arising from the closely spaced nature of the peaks. The second is attributed to the field-induced coherence alone. It is found that the shifts of the positions of the resonance peaks due to field-induced coherence may be in the blue or in the red region.
Under the Doppler free condition, a four-level system with three coherently prepared closely spaced upper levels coupled to a single electromagnetic field is being investigated for the absorptive and dispersive lineshapes. By using a perturbation method, the optical Bloch equations for the present four-level system are solved analytically to obtain the induced polarization and hence the spectral lineshapes. The field induced and field independent coherences appear automatically in the analytical expressions of the imaginary and real parts of the complex polarization. These field independent and field dependent coherences are the outcome of the quantum interference between the probability amplitudes of finding the atom in those energy levels. The phase sensitive field induced polarizations are extensively studied for two special conditions of the ground level populations. The influence of the closely spaced transitions on the quantum coherence and hence the subsequent effects on absorption despite inversion, electromagnetically induced transparency and on the ultrahigh index of refraction are discussed.
A single electromagnetic field interacting with a V-type three-level system having two closely spaced upper levels is studied for the Doppler-free absorptive lineshape. The usual optical Bloch equations are constructed. Quantum interference between the probability amplitudes of the levels participating in a dipole allowed transition is taken into consideration. The quantum interference is manifested through the phase angle. It appears that these phases are significant only if the applied electromagnetic field is strong. The absorptive lineshape calculations are revisited in the light of such field induced coherence. The lineshape exhibits pushing between two spectral lines in addition to the usual pulling between them. It is found that the pushing of the spectral lines depends solely on the coherence induced by the strong field. The complete cancellation of field dependent shifts for the resonance peaks is possible by the suitable adjustment of the phase angles arising from the strong field induced coherence.
A V-type three level system with two closely spaced upper levels interacting with a single mode of the electromagnetic field is studied for the absorptive and dispersive lineshapes. A semiclassical description for the atom-field interaction is being adopted to obtain the usual optical Bloch equations. The approximate analytical solutions for the density matrix elements are obtained by solving coupled optical Bloch equations. Through the off-diagonal density matrix elements, the introduction of phase angles between the levels participating in dipole allowed transitions are automatic. It is shown that these phases are appreciable if the applied electromagnetic field is strong. These field dependent phases (coherence) are responsible for the reduction of the inversionless gain and the absorptionless dispersion. For large decay constants, it is found that the energy gap between the upper two levels has no role to play on the laser without inversion and on the absorptionless dispersion. However, for large population per unit decay, a significant increase of the absorptionless dispersion and the inversionless gain is obtained. The condition for large population decay and a possible experimental realization of the field dependent phases are discussed.
The interaction of a four-level atomic system with two electromagnetic radiations has been studied. The two intermediate levels are closely spaced such that a single radiation frequency can induce transitions from the ground state to both of them. In a cascade-type double resonance, the pump electric-field amplitude is much stronger than the amplitude of the signal field, which can induce transitions from both of the intermediate levels to the upper state. The 15 optical Bloch equations obtained from the Liouville equations are solved analytically to obtain the Doppler-free signal line shape. The computed signals, exhibiting two Lorentzian line profiles, are presented for different pump frequencies. In addition to these one-photon transitions, we obtain a weak two-photon resonance peak. The two-photon resonance becomes weaker when the detuning of the pump frequency from a resonance frequency is increased. When the pump frequency ${\mathrm{\ensuremath{\Omega}}}_{\mathit{p}}$ is intermediate between the pump resonance frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$ and ${\mathrm{\ensuremath{\omega}}}_{2}$, the two-photon resonance is very weak and almost vanishes when ${\mathrm{\ensuremath{\Omega}}}_{\mathit{p}}$=(${\mathrm{\ensuremath{\omega}}}_{1}$+${\mathrm{\ensuremath{\omega}}}_{2}$)/2. When the pump frequency is on resonance with one of the transition frequencies, the Rabi splitting of the signal shows asymmetry because of the presence of a close-lying transition which is pumped off resonance. The intensity-dependent shifts of the transitions are such that they repel each other more and more as the intensity of the pump field is increased. These shifts arise from the nonresonant interaction between the atom and the field.
In the domain of semiclassical formulation and for the Doppler-free atom–field interaction, we construct the optical Bloch equations involving an M-type six-level system coupled to two pump fields and a probe field. The response of the system is probed for different pump-induced transitions in double and triple-resonance situations. In order to obtain the coherent lineshapes (absorptive and dispersive), we use the usual perturbation method for obtaining the approximate analytical solutions to these coupled optical Bloch equations for the density matrix elements. The interferences between the probability amplitudes for different energy levels (dipole allowed and dipole forbidden) are taken care of. For off-resonance pump positions, the linewidths of the three probe transitions are insensitive to the pump Rabi frequencies. On the other hand, the shifts of the three resonance peaks are extremely sensitive to the pump Rabi frequencies. However, for on-resonance pump conditions, the sensitivities of pump Rabi frequencies on the linewidths of the resonance peaks and on the shifts of the resonance peak positions are opposite to those of their off-resonance counterparts. In particular, we have shown the asymmetric and symmetric Rabi splittings under different physical conditions, for non-zero and near-zero probe detuning, respectively. The Rabi splitting under triple-resonance conditions, significantly, modifies the dispersive lineshape at the centre of the absorption line. The two- and three-photon absorptions are also reported for different off-resonant pump positions.
Two electromagnetic fields (the stronger called the pump and the weaker called the signal) are allowed to interact with a four-level double λ-type system with two pairs of closely spaced levels. The present four-level system could also be viewed as an example of a double resonant system. Under the Doppler-free condition and using a semiclassical formulation of atom–field interaction, we derive the optical Bloch equations involving the said four-level system coupled to two external fields. These coupled optical Bloch equations are unsolvable in closed analytical form. In order to obtain the absorptive lineshapes, we use the usual perturbation method for getting the approximate analytical solution to the coupled optical Bloch equations for the density matrix elements. Through the off-diagonal complex density matrix elements, the introduction of phase angles between the levels participating in dipole-allowed transitions is automatic. It is shown that these phases are appreciable if the applied electromagnetic field is strong. For on-resonance pump conditions, we obtain the usual Rabi splitting. The effects of two-photon resonances are clearly shown for off-resonance pump conditions.