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Il Nuovo Cimento D

Picosecond laser pulse correlation by using a molecular dye

F. Giammanco, M. L. Ciampi, Francesco Maccarrone, F. Papoff

Published Apr 1, 1996• 0 citations
Publisher
DOI
10.1007/bf02451805

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This thesis covers an in-depth analysis of the pulsed laser system to be used in the developing a linear technique for the time domain study of the change in coherence of atomic superposition states for the Ytterbrium atom due to phase-interrupting collisions. The hybrid synchronously pumped dye laser yielded optimally shaped sub-picosecond pulses at the 555.6 nanometer wavelength. Comparison of the results for the experimental trials at the 576 and 555.6 nanometer wavelengths yielded an experimental value for the dephasing time, T sub 2 = 621 picoseconds, of the DMETCI dye used as a saturable absorber dye for the first time.
An image-converter streak camera with picosecond time resolution was used in a study of the kinetics of formation of pulses in a traveling-wave laser in which molecular dye solutions were subjected to two-photon optical pumping. An analytic expression was obtained for the lasing threshold of a nonresonator traveling-wave laser in the case of pulsed (τp τe) and quasicontinuous (τp > τe) pumping. Satisfactory agreement was obtained between the calculated and experimental lasing threshold. The kinetics of the compression of output pulses, determined as a function of the pump radiation intensity, was described by rate equations. At pumping rates up to 10 times the threshold a qualitative agreement between the experimental and calculated results was obtained employing a two-band energy model of the dye with a short (compared with the duration of the pump pulses τp) vibrational relaxation time τe. At rates of excitation well above the threshold the kinetics of compression and delay changed, and the output pulses were split into two components, which was interpreted (in the specific case of rhodamine 6G) using a four-band energy scheme. A practical conclusion of this investigation was in the form of recommendations on the use of the proposed approach as a simple method for generating high-intensity single picosecond superradiance pulses of duration τsr with frequency up-con version and a compression coefficient τp/τsr ~ 10.