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Journal of Physics B Atomic and Molecular Physics

Polarisation theory of phase conjugation in resonant non-degenerate four-wave mixing

G. G. Adonts, D G Akopyan

Published Aug 28, 1985• 10 citations
Publisher

Abstract

The theory of polarised light phase conjugation (PC) in non-degenerate four-wave mixing in a resonant medium has been developed in the irreducible tensorial formalism. The theory is applied to a wave with any polarisation in a resonant medium with levels of arbitrary momentum in the absence of pump-induced saturation effects. The formula for the non-linear susceptibility of the medium has been found and it is shown that the change of the polarisation at PC is essentially connected with the relaxation of the atomic multipole momenta (population, orientation and alignment). Wave equations were investigated for different pump-wave polarisations and three different physical mechanisms of the PC are discussed. The influence of the different relaxation rates of the atomic multipole momenta on the PC reflectivity has been investigated. The spectral dependence of the reflectivity and the spectral ranges which depend on the wave polarisation are found. For motionless atoms with small momenta (J 1 = 1 / 2 to J 2 = 1 / 2 , J 1 =1 to J 2 =0), exact formulae for the non-linear susceptibility of the medium as a function of pump intensity were found. The spontaneous decay of higher level to the lower one was taken into account. Because of optical pumping, saturation effects can be shown at considerably smaller intensities than in the usual two-level system. The exact expressions for the PC reflectivity at different polarisations of the pump waves are given.

DOI
10.1088/0022-3700/18/16/023

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•Jan 1, 1982•0 citations
The theory of polarised light phase conjugation (PC) in non-degenerate four-wave mixing in a resonant medium has been developed in the irreducible tensorial formalism. The theory is applied to a wave with any polarisation in a resonant medium with levels of arbitrary momentum in the absence of pump-induced saturation effects. The formula for the non-linear susceptibility of the medium has been found and it is shown that the change of the polarisation at PC is essentially connected with the relaxation of the atomic multipole momenta (population, orientation and alignment). Wave equations were investigated for different pump-wave polarisations and three different physical mechanisms of the PC are discussed. The influence of the different relaxation rates of the atomic multipole momenta on the PC reflectivity has been investigated. The spectral dependence of the reflectivity and the spectral ranges which depend on the wave polarisation are found. For motionless atoms with small momenta (J 1 = 1 / 2 to J 2 = 1 / 2 , J 1 =1 to J 2 =0), exact formulae for the non-linear susceptibility of the medium as a function of pump intensity were found. The spontaneous decay of higher level to the lower one was taken into account. Because of optical pumping, saturation effects can be shown at considerably smaller intensities than in the usual two-level system. The exact expressions for the PC reflectivity at different polarisations of the pump waves are given.
The optical-pumping theory of the passage of polarised radiation through a resonant medium was developed in the irreducible tensorial formalism. Transitions with arbitrary momenta J 1.2 are considered in the cubic approximation. For transitions with small values of momenta (J 1 =1 to J 2 =0; J 1 = 1 / 2 to J 2 = 1 / 2 ) the vector form of the equation system in density-matrix notation allows the problem to be solved exactly for light intensity. In the general case of an elliptically polarised wave, the equation systems for the interaction between circular components of polarisation of light in a resonant medium are obtained. Numerical calculations for deformation and rotation of the polarisation ellipse in a medium subject to saturation effects are also carried out. Irrespective of the initial state the polarisation tends either to a linear or to a circular form as it propagates, depending on times of collisional relaxation of orientation and alignment. The polarisation of linearly and circularly polarised waves does not change as the waves propagate, but the values of the saturation power for these polarisations differ considerably.
We present the theory of resonant backward degenerate four-wave mixing in gaseous media for Doppler-broadened degenerate two-level systems. The degeneracy of the atomic levels as well as the influence of the polarization of the incident fields are taken into account within the framework of a tensorial formalism. The amplitude, line shape, and polarization of the reemitted phase-conjugate field are calculated up to the third order in the incident fields. The velocity average is performed in the approximation of large Doppler linewidths. One considers in detail the influence of depolarizing relaxation processes and the effects of pump-probe angular separation. In particular, the importance of the residual Doppler effect (shortening of the lifetime of the optically induced gratings by the atomic motion) associated with the pump-probe angle is emphasized. We show that the polarization of the reemitted fields is governed by very simple laws as soon as the residual Doppler effect overcomes the lifetimes of the atomic levels. Phase-conjugate mirrors can be simply characterized by a linear dichroism (parallel pump polarizations) or a birefringence (cross-polarized pumps). Vectorial phase conjugation is also analyzed, in the case of counter-rotating circular polarizations of the pumps. Finally, the case of two-photon transition is studied and compared with the case of a resonant transition.
Current experimental studies of degenerate four-wave mixing in saturable absorbers1,2 have shown that the dependence of the reflectivity on the pump intensity exhibits a double maxima. This phenomenon can arise from the fact that the medium approximates a set of four-level quantum systems. We have carried out a detailed analysis of the nonlinear processes of degenerate four-wave mixing in a four-level system. Because resonant saturable absorbers are being considered for systems applications, e.g., optical phase conjugation and wide FOV filters, the results presented are relevant to various optical phase conjugation devices. There are two distinct regimes which are of interest. The first case is when the intramolecular relaxation is very weak or absent. The second is when the intramolecular relaxation is strong. For the weak case the medium behaves like a set of two distinct dipole radiation sources which can generate interference effects.
Considers phase conjugation through degenerate four-wave mixing in a Λ-type three-level system under certain simplifying assumptions, the most restrictive among them being the assumption of symmetrical detuning of the pump from the two lower lying sublevels. When compared to an absorbing resonant two-level system, it is found that significantly higher values of the phase-conjugate reflectivity are possible at pump intensities well below saturation provided the sublevel splitting is less than a homogeneous linewidth. The physical mechanism responsible for phase conjugation is coherent population trapping arising from two-photon-induced atomic coherence between the two sublevels.
The representation of irreducible tensor operators is used to develop a theory of wavefront reversal (WFR) in the absence of saturation effects. This theory deals with arbitrarily polarized waves in a two-level resonant medium having arbitrary angular momenta. It is shown that there are three different physical reversal mechanisms associated with a nonuniform population and with the coherence of the magnetic sublevels in the field. An investigation is made of the influence of the decay times of the polarization moments of the system (the total population, orientation, alignment) on WFR. In particular, it is shown that, subject to specific relationships between the decay times, new collision-induced reversal processes can occur in the presence of deorienting collisions. An investigation is made of the spectral composition of the reflection coefficient of the reversed wave and it is shown that there are various spectral ranges of efficient reversal which in general depend on the polarizations of the interacting waves.
This thesis describes the theoretical solution and experimental verification of phase conjugation via nondegenerate four-wave mixing in resonant media. The theoretical work models the resonant medium as a two-level atomic system with the lower state of the system being the ground state of the atom. Working initially with an ensemble of stationary atoms, the density matrix equations are solved by third-order perturbation theory in the presence of the four applied electro-magnetic fields which are assumed to be nearly resonant with the atomic transition. Two of the applied fields are assumed to be non-depleted counterpropagating pump waves while the third wave is an incident signal wave. The fourth wave is the phase conjugate wave which is generated by the interaction of the three previous waves with the nonlinear medium. The solution of the density matrix equations gives the local polarization of the atom. The polarization is used in Maxwell's equations as a source term to solve for the propagation and generation of the signal wave and phase conjugate wave through the nonlinear medium. Studying the dependence of the phase conjugate signal on the various parameters such as frequency, we show how an ultrahigh-Q isotropically sensitive optical filter can be constructed using the phase conjugation process. In many cases the pump waves may saturate the resonant medium so we also present another solution to the density matrix equations which is correct to all orders in the amplitude of the pump waves since the third-order solution is correct only to first-order in each of the field amplitudes. In the saturated regime, we predict several new phenomena associated with degenerate four-wave mixing and also describe the ac Stark effect and how it modifies the frequency response of the filtering process. We also show how a narrow bandwidth optical filter with an efficiency greater than unity can be constructed. In many atomic systems the atoms are moving at significant velocities such that the Doppler linewidth of the system is larger than the homogeneous linewidth. The latter linewidth dominates the response of the ensemble of stationary atoms. To better understand this case the density matrix equations are solved to third-order by perturbation theory for an atom of velocity v. The solution for the polarization is then integrated over the velocity distribution of the macroscopic system which is assumed to be a gaussian distribution of velocities since that is an excellent model of many real systems. Using the Doppler broadened system, we explain how a tunable optical filter can be constructed whose bandwidth is limited by the homogeneous linewidth of the atom while the tuning range of the filter extends over the entire Doppler profile. Since it is a resonant system, sodium vapor is used as the nonlinear medium in our experiments. The relevant properties of sodium are discussed in great detail. In particular, the wavefunctions of the 3S and 3P states are analyzed and a discussion of how the 3S-3P transition models a two-level system is given. Using sodium as the nonlinear medium we demonstrate an ultrahigh-Q optical filter using phase conjugation via nondegenerate four-wave mixing as the filtering process. The filter has a FWHM bandwidth of 41 MHz and a maximum efficiency of 4 x 10-3. However, our theoretical work and other experimental work with sodium suggest that an efficient filter with both gain and a narrower bandwidth should be quite feasible.