Molecular crystals and liquid crystals science technology. Section A, Molecular crystals and liquid crystals/Molecular crystals and liquid crystals science and technology. Section A, Molecular crystals and liquid crystals

Single Molecule Spectroscopy and Spectral Hole-Burning

Hermann Bach, Thomas Irngartinger, Alois Renn, Urs P. Wild

Published Dec 1, 1996• 4 citations

Publisher

Abstract

Spectral hole-burning in the Shpol'skii system terrylene in n-octane has been investigated on the single molecule level. Fluorescence microscopy provides a link between the two methods of spectral hole-burning and single molecule spectroscopy. Information about many different individual molecules can be obtained simultaneously under identical experimental conditions allowing the determination of statistical properties. From a single frequency scan after spectral hole-burning, the ground state population function and an average hole-width, as well as the single molecule linewidth distribution of 700 molecules have been determined.

DOI: 10.1080/10587259608042735

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