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The European Physical Journal B

Pressure shift of atomic resonance lines in liquid and solid helium

S. I. Kanorsky, Antoine Weis, Markus Arndt, R. Dziewior, Theodor W. Hänsch

Published Sep 1, 1995• 46 citations
Publisher
DOI
10.1007/bf01338408

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We have measured the pressure broadening and shift of the excitation and emission lines of the 6s2{\mathit{s}}^{2}s2 1^{1}1S0{\mathit{S}}_{0}S0​\ensuremath{\rightarrow}6s6p 1^{1}1P1{\mathit{P}}_{1}P1​ transition of Ba atoms implanted in liquid and solid helium at 1.5 K. The observed spectra are quantitatively explained within the adiabatic line-broadening theory by assuming a bubble structure of the trapping sites for the Ba atoms. The evolution of the bubble shape and size in the optical excitation-deexcitation cycle is modeled theoretically.
We show that for atoms trapped in a liquid He matrix the excitation and emission spectra can be quantit- atively described by the bubble model which treats the matrix as an incompressible continuous medium. Com- parison with experimental results shows that the model also holds for a solid matrix. The model is only valid in the case where the attractive He-He interaction dominates the attractive part of the foreign atom-helium interaction. Its failure in the case of implanted Na atoms is discussed.
The excitation and emission spectra of alkali-metal atoms (Cs and Rb) in liquid helium are studied. The helium pressure is changed from the saturated vapor pressure to about 25 atm at 1.6 K, under which conditions the liquid helium is in a superfluid state. The pressure shift and broadening of the observed spectra corresponding to the D lines are explained qualitatively by a theoretical calculation based on the spherical atomic bubble model. The Cs D2{\mathit{D}}_{2}D2​ excitation spectra are found to have double peaks, indicating the existence of anisotropic oscillations of the bubble surface. The disappearance of the D2{\mathit{D}}_{2}D2​ emission lines and the pressure-dependent quenching of the Rb D1{\mathit{D}}_{1}D1​ emission lines are also discussed.