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Physical Review A

Statistical mechanics of stationary states. VII. Quantum-mechanical theory with applications to ferromagnets

Isaac Goldhirsch, Itamar Procaccia

Published Oct 1, 1980• 2 citations
Publisher

Abstract

A quantum-statistical-mechanical theory of nonequilibrium stationary states (NESS) is presented. The average of an arbitrary dynamical operator is calculated. The theory is applied to correlation functions in a heat-conducting NESS of the Heisenberg ferromagnet. Significant changes (as compared with equilibrium) are found. Correlation functions that vanish in equilibrium due to symmetry are allowed and are very important for $\stackrel{\ensuremath{\rightarrow}}{\mathrm{k}}$ vectors in the hydrodynamic regime. In the absence of magnetic field, the change with respect to equilibrium is pronounced. A static correlation that depends on $k$ as $\frac{1}{{k}^{7}}$ is found. Such correlations are expected to be seen experimentally when magnon-phonon interactions can be neglected (i.e., $k>{10}^{6}$ ${\mathrm{cm}}^{\ensuremath{-}1}$). The influence on time correlation functions is examined and found to be well within experimental detectability.

DOI
10.1103/physreva.22.1720

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A quantum-statistical-mechanical theory of nonequilibrium stationary states (NESS) is presented. The average of an arbitrary dynamical operator is calculated. The theory is applied to correlation functions in a heat-conducting NESS of the Heisenberg ferromagnet. Significant changes (as compared with equilibrium) are found. Correlation functions that vanish in equilibrium due to symmetry are allowed and are very important for k\ensuremath→\stackrel{\ensuremath{\rightarrow}}{\mathrm{k}}k\ensuremath→​ vectors in the hydrodynamic regime. In the absence of magnetic field, the change with respect to equilibrium is pronounced. A static correlation that depends on kkk as 1k7\frac{1}{{k}^{7}}k71​ is found. Such correlations are expected to be seen experimentally when magnon-phonon interactions can be neglected (i.e., k>106k>{10}^{6}k>106 cm\ensuremath−1{\mathrm{cm}}^{\ensuremath{-}1}cm\ensuremath−1). The influence on time correlation functions is examined and found to be well within experimental detectability.
A statistical theory of the localized model of ferromagnetism is developed by considering the effective density matrices for a single spin, and two nearest-neighbor spins, respectively. The Ising Model and the Heisenberg model, and even the case of the anisotropic exchange interaction, are treated within a unified mathematical scheme. The result is reduced to that of the Bethe approximation in the case of the Ising model, and the constant coupling approximation in the case of the Heisenberg model. The method is generalized to calculate the static spin-correlation function. It is obtained in Ornstein-Zernike type. In the nonequilibrium state, the expectation value of the spin decays by the homogeneous damping as well as the spin-diffusion process. This relaxation equation is different from that by Van Hove because of the existence of the homogeneous damping. The diffusion constant does not vanish even at the Curie point TC, contrary to Van Hove's result, although the damping constant vanishes at TC. The latter fact causes the critical slowing down of the regression of fluctuation. The solution of this relaxation equation gives the time-dependent spin-correlation function. The method can be applied to the antiferromagnetic case, too.
The development of methods of quantum statistical mechanics is considered in light of their applications to quantum solid-state theory. We discuss fundamental problems of the physics of magnetic materials and the methods of the quantum theory of magnetism, including the method of two-time temperature Green’s functions, which is widely used in various physical problems of many-particle systems with interaction. Quantum cooperative effects and quasi-particle dynamics in the basic microscopic models of quantum theory of magnetism: the Heisenberg model, the Hubbard model, the Anderson Model, and the spinfermion model are considered in the framework of novel self-consistent-field approximation. We present a comparative analysis of these models; in particular, we compare their applicability for description of complex magnetic materials. The concepts of broken symmetry, quantum protectorate, and quasi-averages are analyzed in the context of quantum theory of magnetism and theory of superconductivity. The notion of broken symmetry is presented within the nonequilibrium statistical operator approach developed by D.N. Zubarev. In the framework of the latter approach we discuss the derivation of kinetic equations for a system in a thermal bath. Finally, the results of investigation of the dynamic behavior of a particle in an environment, taking into account dissipative effects, are presented.
We use the spin functional renormalization group recently developed by two of us [Krieg and Kopietz, Phys. Rev. B 99, 060403(R) (2019)] to calculate the magnetization M(H,T)M(H,T)M(H,T) and the damping of magnons due to classical longitudinal fluctuations of quantum Heisenberg ferromagnets. In order to guarantee that for vanishing magnetic field $H\ensuremath{\rightarrow}0$, the magnon spectrum is gapless when the spin rotational invariance is spontaneously broken, we use a Ward identity to express the magnon self-energy in terms of the magnetization. In two dimensions, our approach correctly predicts the absence of long-range magnetic order for H=0H=0H=0 at finite temperature TTT. The magnon spectrum then exhibits a gap from which we obtain the transverse correlation length. We also calculate the wave-function renormalization factor of the magnons. As a mathematical byproduct, we derive a recursive form of the generalized Wick theorem for spin operators in frequency space which facilitates the calculation of arbitrary time-ordered connected correlation functions of an isolated spin in a magnetic field.
Starting from the usual formulation of nonequilibrium quantum statistical mechanics, the expectation value of an operator A in a steady state nonequilibrium quantum system is shown to have the form 〈A〉 =Tr{${\mathit{e}}^{\mathrm{\ensuremath{-}}\mathrm{\ensuremath{\beta}}(\mathit{H}\mathrm{\ensuremath{-}}\mathit{Y})}$A} /Tr{${\mathit{e}}^{\mathrm{\ensuremath{-}}\mathrm{\ensuremath{\beta}}(\mathit{H}\mathrm{\ensuremath{-}}\mathit{Y})}$}, where H is the Hamiltonian, \ensuremath{\beta} is the inverse of the temperature, and Y is an operator which depends on how the system is driven out of equilibrium. Because 〈A〉 is not expressed as a sum of correlation functions integrated over real time, one can now consider performing nonperturbative calculations in interacting nonequilibrium quantum problems.
The usual spin-wave theory, when applied to the calculation of rotationally invariant averages in the Heisenberg model, permits exact calculation of static and dynamical correlation functions in one dimension. The results are also believed to be exact in two dimensions, although this has not been show rigorously here. The one-dimensional ferromagnet in the hydrodynamic regime and the two-dimensional ferromagnet at all wave vectors do not satisfy the dynamical scaling hypothesis. There is no characteristic exponent in these cases. The present results contradict the prediction of the mode-coupling theory.
A system of bosons interacting by 2-body forces is treated in momentum space in the Heisenberg representation, assuming a statistically homogeneous and stationary state. The principle of weak statistical dependence of different momentum modes, previously applied to turbulence dynamics, is used to obtain an exact expansion expressing quadrilinear (2-body) time-displaced correlation functions of the second-quantized field variables in terms of bilinear time-displaced correlation functions and average impulse-response functions. The last-named functions are defined in terms of the exact Green's operator, for infinitesimal sources, of the nonlinear Heisenberg equations of motion. A set of coupled integral equations are then obtained which determine both the bilinear correlation functions and the response functions. By retaining in these equations only the lowest terms in the cited expansion, a theory is obtained which includes particle "self-energy" interactions with the medium of all orders. A modification of the theory is briefly outlined which includes, at finite temperatures, all the processes described at absolute zero by the Brueckner approximation and, in addition, 3-body effects, iterated to all orders, which are omitted in that approximation.