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Journal of the Physical Society of Japan

Exactly Soluble Models of Quantum Systems Showing the Second Order Phase Transitions

Masuo Suzuki

Published Nov 1, 1966• 27 citations
Publisher

Abstract

A theorem is given for calculating the partition function of quantum mechanical systems. Using this theorem, it is shown that some sort of long-range interaction is equivalent to an effective field. The exact solution of linear anisotropic Heisenberg model with staggered fields, and consequently the zero field staggered susceptibility are given. Finally, it is shown that due to the effect of the transverse components, the value of the Curie point decreases both in the ferromagnetic and antiferromagnetic cases. The rate of decreases in the antiferromagnetic case is smaller than in the ferromagnetic case.

DOI
10.1143/jpsj.21.2140

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A theorem is given for calculating the partition function of quantum mechanical systems. Using this theorem, it is shown that some sort of long-range interaction is equivalent to an effective field. The exact solution of linear anisotropic Heisenberg model with staggered fields, and consequently the zero field staggered susceptibility are given. Finally, it is shown that due to the effect of the transverse components, the value of the Curie point decreases both in the ferromagnetic and antiferromagnetic cases. The rate of decreases in the antiferromagnetic case is smaller than in the ferromagnetic case.
We present a systematic study of the anisotropic spin-1/2 Heisenberg model in staggered magnetic fields in two dimensions. To mimic real materials, we consider a system of coupled, antiferromagnetic chains, whose interchain interaction can be either ferro- or antiferromagnetic. When the staggered field is commensurate with the magnetic interactions, an energy gap opens immediately and follows a power law as a function of the applied field, similar to the situation in one dimension. When the field competes with the interactions, a quantum phase transition (QPT) occurs from a gapless, magnetically ordered phase at low fields to a gapped, disordered regime. We use a continuous-time Monte Carlo method to compute the staggered moment of the ordered phases and the spin gap of the disordered phases. We deduce the phase diagrams as functions of the anisotropy ratio and the applied field, and calculate the scaling behavior of the models in both quantities. We show that in the competitive case, the staggered field acts to maintain a regime of quasi-1D behavior around the QPT, and we discuss as a consequence the nature of the crossover from one-dimensional (1D) to 2D physics.
Exact expressions for the partition function, spin pair correlation function, and susceptibility of the onedimensional isotropic classical Heisenberg model are obtained in zero external field with cyclic boundary conditions. It is shown that the methods used to derive these results enable the partition functions and susceptibilities of finite clusters of interacting classical spins to be evaluated in terms of the $3n\ensuremath{-}j$ symbols of Wigner. Exact results in one dimension are also obtained for the partition function and susceptibility of a "planar" classical Heisenberg model. In this model the spin vectors interact via a Heisenberg coupling but each spin vector is restricted to lie in a plane.The anisotropic classical Heisenberg model described by the Hamiltonian $\mathcal{H}=\ensuremath{-}\ensuremath{\Sigma}\stackrel{}{(\mathrm{ij})}2({{J}_{\mathrm{ij}}}^{x}{{s}_{i}}^{x}{{s}_{j}}^{x}+{{J}_{\mathrm{ij}}}^{y}{{s}_{i}}^{y}{{s}_{j}}^{y}+{{J}_{\mathrm{ij}}}^{z}{{s}_{i}}^{z}{{s}_{j}}^{z})\ensuremath{-}mH\ensuremath{\Sigma}\stackrel{N}{j=1}{{s}_{i}}^{z},$ where six{{s}_{i}}^{x}si​x, siy{{s}_{i}}^{y}si​y, and siz{{s}_{i}}^{z}si​z are components of the unit vector si{\mathbf{s}}_{i}si​, is also considered. A perturbation series for the zero-field free energy of the anisotropic model in one dimension with nearest-neighbor interactions Jijx=Jijy=J{{J}_{\mathrm{ij}}}^{x}={{J}_{\mathrm{ij}}}^{y}=JJij​x=Jij​y=J and ${{J}_{\mathrm{ij}}}^{z}=\ensuremath{\gamma}J$ is developed in powers of $\ensuremath{\gamma}\ensuremath{-}1$ using the isotropic model as the unperturbed system. Detailed calculations are performed to third order in $\ensuremath{\gamma}\ensuremath{-}1$. It is found that the perturbation series for the energy per spin breaks down as $T\ensuremath{\rightarrow}0$. A high-temperature series expansion for the anisotropic model, which is valid for a general interaction potential and lattice, is derived by generalizing the methods developed by Horwitz and Callen for the Ising model. This series is rearranged to give a simplified diagram expansion. Finally, a practical technique for calculating the high-temperature series expansions of the zero-field free energy and susceptibility of the isotropic classical Heisenberg model is presented.
A Hamiltonian of a one-dimensional Heisenberg model with ferromagnetic interaction is expressed in terms of fermion operators, and renormalized linked cluster expansion has been carried out. It is shown that the approximation leads to ferromagnetic behaviors similar to the molecular field approximation. A model for which the second- and higher-order terms vanish is presented and regarded as an example of quantum-mechanical systems that shows ferromagnetism rigorously. It is also noted that the model is very much like the Husimi-Temperley model or the van der Waals gas with respect to a long-range character of interaction and the vanishing of higher-order terms.
We study quantum phase transitions in Heisenberg antiferromagnetic chains with a staggered power-law decaying long-range interactions. Employing the density-matrix renormalization group (DMRG) algorithm and the fidelity susceptibility as the criticality measure, we establish more accurate values of quantum critical points than the results obtained from the spin-wave approximation, quantum Monte Carlo, and DMRG in literatures. The deviation is especially evident for strong long-range interactions. We extend isotropic long-range interactions to the anisotropic cases and find that kaleidoscope of quantum phases emerge from the interplay of anisotropy of the long-range exchange interaction and symmetry breaking. We demonstrate nonfrustrating long-range interactions induce the true long-range order in Heisenberg antiferromagnetic chains with a continuous symmetry breaking, lifting the restrictions imposed by the Mermin-Wagner theorem.
We study the phase diagram of the spin-1/2 XXZ Heisenberg chain in a staggered magnetic field. An exact solution is obtained along the phase boundary, where the exchange anisotropy and the staggered-field strength satisfy an exact analytical relation, yielding a highly degenerate manifold of ground states with off-diagonal long-range order. We demonstrate that these exact ground states lie on the boundary between the ferromagnetic phase and a gapless Luttinger liquid phase. Upon further decreasing the anisotropy, the gapless phase eventually gives way to a gapped quantum-disordered phase. Large-scale density-matrix renormalization group calculations confirm this phase structure and indicate that the transition across the exact boundary is of first order. Our results provide an exact benchmark for understanding quantum phase transitions driven by staggered magnetic fields in one-dimensional quantum spin systems.
We study the ground-state phase diagram of an unfrustrated antiferromagnetic Ising chain with longitudinal and transverse fields in the full range of interactions: from all-to-all to nearest-neighbors. First, we solve the model analytically in the strong long-range regime, confirming in the process that a mean-field treatment is exact for this model. We compute the order parameter and the correlations and show that the model exhibits a tricritical point where the phase transition changes from first to second order. This is in contrast with the nearest-neighbor limit where the phase transition is known to be second order. To understand how the order of the phase transition changes from one limit to the other, we tackle the analytically intractable interaction ranges numerically, using a variational quantum Monte Carlo method with a neural-network-based ansatz, the visual transformer. We show how the first-order phase transition shrinks with decreasing interaction range and establish approximate boundaries in the interaction range for which the first-order phase transition is present. Finally, we establish that the key ingredient to stabilize a first-order phase transition and a tricritical point is the presence of ferromagnetic interactions between spins of the same sublattice on top of antiferromagnetic interactions between spins of different sublattices. Tunable-range unfrustrated antiferromagnetic interactions are just one way to implement such staggered interactions.