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Physical Review A

Absorption spectrum of optically bistable systems

Lorenzo M. Narducci, Robert Gilmore, D.H. Feng, G. S. Agarwal

Published Aug 1, 1979• 16 citations
Publisher

Abstract

The quantum-mechanical theory of optical bistability developed in an earlier paper is generalized to calculate the absorption spectrum (gain coefficient) of an optically bistable system in the presence of a weak probe field. The behavior of the gain coefficient on the cooperative branch and the single-atom branch is analyzed in detail.
DOI
10.1103/physreva.20.545

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The purpose of this work is to study the behavior of atomic fluctuations and the spectrum of transmitted light by a nonlinear medium with absorption and dispersion. The authors make use of the system-size expansion and apply it to the quantum-mechanical Langevin's equations for the atomic operators and obtain the characteristic curves for bistable behavior, macroscopic atomic expectation values, and the spectrum of the atomic fluctuations. The calculated spectrum of transmitted light exhibits line narrowing near bistable thresholds, discontinuous formation of bands along the high-transmission bistable branch, and hysteresis effects, etc., for detuning $|\ensuremath{\delta}|$ less than a critical value ${\ensuremath{\delta}}_{c}$. For $|\ensuremath{\delta}|>{\ensuremath{\delta}}_{c}$, the discontinuous character of all the physical variables of the system vanishes; the system no longer exhibits bistable behavior. The system, however, still shows cooperative and single-atom behavior separated by a critical value of the intensity of the incident coherent pump at which a critical slowing down of the medium occurs, exhibiting a phase transition.
The main purpose of this paper is to study the behavior of the atomic fluctuations and the spectrum of the light transmitted by an absorptive bistable device. To this end we develop an approximation scheme based on the so-called system-size expansion and apply it to the quantum-mechanical Langevin equations for the atomic fluctuation operators. The Bonifacio-Lugiato mean-field equations for bistability are derived from the lowest-order approximation to the system-size expansion, while the atomic correlation functions result from the next-higher-order expansion. The calculated spectrum of the transmitted light exhibits line narrowing near the bistable thresholds, discontinuous formation of sidebands along the high-transmission branch of the device, and hysteresis effects.
We specialize the quantum-statistical theory of optical bistability developed in "Optical Bistability. II" to a low-QQQ cavity. From a linearized Fokker-Planck equation derived in the positive PPP representation, the steady-state correlation matrix and spectrum of fluctuations are calculated. Expressions which normally assume a positive-definite diffusion matrix are shown to be valid for nonpositive-definite diffusion. For absorptive bistability we find agreement with results derived previously by quite different methods. More generally we extend previously published results by including atomic and cavity detunings. We compare the transmitted spectrum for dispersive bistability with that for absorptive bistability, and photon antibunching in dispersive bistability is discussed.
The absorption and gain bands of a weak probe signal in the presence of the Bose-Einstein condensation of excitons, which appears under nonequilibrium conditions in a field of coherent laser radiation, are considered. It is shown that the absorption of light is caused by a quantum transition from the ground state of the crystal to the quasiexciton branch of the spectrum. Amplification of the signal occurs as a result of transitions from the quasiexciton branch of the spectrum to the ground state of the crystal.
It is shown theoretically that optical bistability will exist in a material whose optical absorption is more than linearly proportional to the degree to which the material is excited. No cavity or external feedback is required. The underlying principle of this bistability appears to be a generalization of several previous independent discussions of mirrorless bistabilities in specific physical systems. This bistability and associated differential gain are demonstrated experimentally using a thermal nonlinearity in a GaAs/GaAlAs multiple-quantum-well semiconductor. Theory and experiment show good agreement.