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Low Temperature Physics

Symmetry and relaxation dynamics of spins = 1 magnets

Mikhail Yurievich Kovalevsky, Anton V. Hlushchenko

Published May 1, 2014• 8 citations
Publisher

Abstract

Pure and mixed quantum states of spin s = 1 magnets are examined by introducing a polarization density matrix. Uniaxial and biaxial quadrupole orderings corresponding to pure magnetic states are found and the degrees of polarization are calculated. The types of normal and degenerate magnetic states associated with subalgebras of Poisson brackets of the magnetic degrees of freedom are established. The spectra of collective magnetic excitations are calculated taking damping in the normal and degenerate states into account.

DOI
10.1063/1.4876536

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Pure and mixed quantum states of spin s = 1 magnets are examined by introducing a polarization density matrix. Uniaxial and biaxial quadrupole orderings corresponding to pure magnetic states are found and the degrees of polarization are calculated. The types of normal and degenerate magnetic states associated with subalgebras of Poisson brackets of the magnetic degrees of freedom are established. The spectra of collective magnetic excitations are calculated taking damping in the normal and degenerate states into account.
We have studied the dynamics of none-quilibrium states of high-spin magnets (s>1/2) in a Weyl and Racah basis. We have established non-linear equations of the dynamics of magnets with arbitrary spin and studied the case of the spin s=1;3/2 in detail. We have found expressions for Casimir invariants in case of pure quantum states and established inequalities that characterize magnetic degrees of freedom for mixed quantum states. We have calculated the explicit form of the polarization density matrix for pure quantum states of magnets with spins s=1 and s=3/2.
We have numerically solved the low-energy excitation spectra of ferromagnetic Bose-Einstein condensates subject to dipolar interparticle interactions. The system is assumed to be harmonically confined by purely optical means, thereby maintaining the spin degree of freedom of the condensate order parameter. Using a zero-temperature spin-1 model, we solve the Bogoliubov excitations for different spin textures, including a spin-vortex state in the absence of external magnetic fields and a rapidly rotating polarized spin texture in a finite homogeneous field. In particular, we consider the effect of dipolar interactions on excitations characteristic of ferromagnetic condensates. The energies of spin waves and magnetic quadrupole modes are found to increase rapidly with the dipolar coupling strength, whereas the energies of density oscillations change only slightly.
The ground states and collective excitations of trapped Fermion gases consisting of atoms with magnetic dipole moment are studied using a time-dependent density-matrix approach. The advantages of the density-matrix approach are that one-body and two-body observables are directly calculated using one-body and two-body density matrices and that it has a clear relation to the Hartree-Fock (HF) and time-dependent HF theory. The HF calculations show the magnetization of the gases when the dipole-dipole interaction is strong. It is shown that the tensor properties of the dipole-dipole interaction are revealed in the excitation modes associated with spin degrees of freedom.
The excitation spectrum of the one-dimensional spin-orbital model in a magnetic field is studied, using a recently developed dynamical density-matrix renormalization-group technique. The method is applied to chains with up to 80 sites, and examined for test cases such as the one-dimensional spin-1/2 Heisenberg antiferromagnet whose excitation spectrum is known exactly from the Bethe ansatz. In the spin-orbital chain, the characteristic dynamical response depends strongly on the model parameters and the applied magnetic field. The coupling between the spin and orbital degrees of freedom is found to influence the incommensuration at finite magnetizations. In the regions of the phase diagram with only massive spin and orbital excitations, a finite field is required to overcome the spin gap. An orbital mode is found to become massless in this partially spin-polarized regime, indicating a strong coupling between the two degrees of freedom. In the critical region with three elementary gapless excitations, a prominent particle-hole excitation is observed at higher energies, promoted by the biquadratic term in the model Hamiltonian of the spin-orbital chain.
This thesis investigates exotic phases of matter in magnetic materials that present anisotropic properties in two dimensions. Using the microscopic spin Hamiltonians, the study addresses two problems: (i) the appearance of a novel class of magnetic excitations in the spectra of anisotropic magnets at zero temperature, and (ii) the quantum-to-classical correspondence of spins for the description of magnetic solids in the disordered phase above the critical temperature. Different analytical and numerical means are used to this purpose.In the first part, motivated by experimental observations of multipolar excitations in afamily of strongly-anisotropic van der Waals antiferromagnets, we have developed ageneral theory for these excitations as a distinct type of quasi-particles. We called themlongitudinal magnons. They appear in easy-axis magnetic materials, and are characterized by the quantum number Sz = ±2S. They can exist as coherent long-lived excitations for D ≥ |J|, where D and J are the typical single-ion and exchange coupling constants, respectively. Starting with the strong-coupling limit, this work presented different approaches to compute the dispersion of longitudinal magnons. First, a mapping to an effective spin-1/2 model was performed and illustrated for several lattice spin models: the honeycomb-lattice zigzag antiferromagnet and the square-lattice ferro- and antiferromagnet. The excitation energy was derived for different spin values S = 1, 3/2, 2and 5/2. Second, a thorough study explored the S = 1 anisotropic square-lattice, wherethe analytical results of the effective model are compared to the multi-boson spin-wavetheory, the linked-cluster calculations in antiferromagnetic coupling J > 0, and the exactsolution of the two-magnon problem in ferromagnetic coupling J < 0. In the limit of largeJ/D, the longitudinal magnons start to overlap with the multi-magnon continuum, andtheir finite lifetime can be computed using the multi-boson theory, which is specificallyshown for two-magnon decay processes in S = 1. Moreover, critical values of J/D forthe stability of longitudinal magnons are obtained along high-symmetry lines of the Brillouin zone. Third, we investigated the appearance and condensation of the longitudinal magnons in triangular S = 1 antiferromagnets under high magnetic field. As suggested by recent experiments on a candidate material, a spin nematic phase may appear upon condensation of the multipolar excitations, opening the way for realizations of new phases of matter in classically-ordered magnets.In the second part, the correspondence between quantum and classical spins is investigated for spin Hamiltonians at finite temperature. Given a model of quantum spins, it is useful to determine the classical model that best describes its thermodynamics, which is of interest for semi-classical analyses, e.g. by classical Monte Carlo methods. Based on high-temperature series expansions, we established the scaling laws of the different microscopic constants in a quantum spin model, involving quadratic and biquadratic exchange interactions, single-ion anisotropy and the Zeeman energy. We showed that quantum corrections to the thermodynamic quantities are power series in S(S + 1). Subsequently, the findings were applied to numerically determine the phase transition temperature in several ferro- and antiferromagnetic compounds, using classical Monte Carlo simulations. To this aim, the lattice spin models were constructed with microscopic coupling constants from the literature, and the transition temperatures were compared to the experimental values.This illuminates complex collective magnetic behaviors in different models and materials.