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Physical review. B, Condensed matter

Random antiferromagnetic quantum spin chains

Daniel S. Fisher

Published Aug 1, 1994• 651 citations
Publisher

Abstract

The properties of spin-1/2 antiferromagnetic chains with various types of random exchange coupling are studied via an asymptotically exact decimation renormalization-group transformation, which is a generalization of that introduced by Dasgupta and Ma. Random-singlet phases occur in which each spin is paired with one other spin that may be very far away; more exotic phases also occur. The behavior of typical and mean correlation functions is analyzed and found to be very different, with very small sets of spins dominating the latter at long distances as well as the low-temperature thermodynamics. Some of the phase transitions that occur between antiferromagnetically ordered phases and random singlet or other antiferromagnetic phases are also analyzed. For example, if a small uniaxial anisotropy perturbation is added to a random Heisenberg antiferromagnetic chain, a transition occurs from a random-singlet phase to an Ising antiferromagnetic phase, as the anisotropy changes sign from easy plane to easy axis. The staggered magnetization vanishes at the transition with critical exponent \ensuremath{\beta}=8/(1+ \ensuremath{\surd}7 ). Possible implications for the properties of random quantum magnetic systems in higher dimensions are briefly discussed.

DOI
10.1103/physrevb.50.3799

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The properties of spin-1/2 antiferromagnetic chains with various types of random exchange coupling are studied via an asymptotically exact decimation renormalization-group transformation, which is a generalization of that introduced by Dasgupta and Ma. Random-singlet phases occur in which each spin is paired with one other spin that may be very far away; more exotic phases also occur. The behavior of typical and mean correlation functions is analyzed and found to be very different, with very small sets of spins dominating the latter at long distances as well as the low-temperature thermodynamics. Some of the phase transitions that occur between antiferromagnetically ordered phases and random singlet or other antiferromagnetic phases are also analyzed. For example, if a small uniaxial anisotropy perturbation is added to a random Heisenberg antiferromagnetic chain, a transition occurs from a random-singlet phase to an Ising antiferromagnetic phase, as the anisotropy changes sign from easy plane to easy axis. The staggered magnetization vanishes at the transition with critical exponent \ensuremath{\beta}=8/(1+ \ensuremath{\surd}7 ). Possible implications for the properties of random quantum magnetic systems in higher dimensions are briefly discussed.
The zero-temperature phase diagram of the anisotropic, strongly disordered antiferromagnetic quantum spin-1 chain is investigated, within the framework of a real-space renormalization-group approach. In the presence of uniform anisotropy there occurs a phase transition from a random singlet phase to an Ising antiferromagnetic phase controlled by a fixed point that does not have Heisenberg symmetry. We find evidence of a fixed point due to randomness in the anisotropy similar to that which occurs for quantum Heisenberg spin-12\frac{1}{2}21​ chains.
A real-space renormalization-group treatment of random transverse-field Ising spin chains that was introduced previously is developed and extensively analyzed. It yields results that are asymptotically exact in the critical region near the zero-temperature para-to-ferromagnetic quantum phase transition. In particular, the exact scaling function is obtained for the magnetization as a function of a uniform applied magnetic field and the distance to the critical point, and up to the solution of a linear ordinary differential equation whose solution can be exhaustively analyzed, the scaling function of the average spin-spin correlation function is also obtained. Thus more exact information is obtainable about the critical behavior for this random model than is known for the pure version which is equivalent to the two-dimensional Ising model. The basic reason for this is the extremely broad distribution of energy scales that occurs at low energies near the critical point of the random system. For the random chain the distribution of the magnetization of the first spin in a semi-infinite system is also studied and the results found to agree in the scaling limit with results of McCoy obtained from the exact solution of the closely related McCoy-Wu Ising model; this provides strong justification for the validity of the present approach. The singular properties of the weakly ordered and weakly disordered ``Griffiths' phases'' that occur at zero temperature near the critical point are also studied, as well as the behavior at low but nonzero temperature. Possible extensions of the results and general lessons drawn from them for other random systems are briefly discussed.
The low-temperature thermodynamic properties of a spin-\textonehalf{} one-dimensional random anisotropic (Heisenberg-Ising) antiferromagnet described by the Hamiltonian $H=\ensuremath{\Sigma}{i}^{}{J}_{i}({\ensuremath{\sigma}}_{x}^{i}{\ensuremath{\sigma}}_{x}^{i+1}+{\ensuremath{\sigma}}_{y}^{i}{\ensuremath{\sigma}}_{y}^{i+1}+\ensuremath{\gamma}{\ensuremath{\sigma}}_{z}^{i}{\ensuremath{\sigma}}_{z}^{i+1})$ are studied as a function of disorder and anisotropy. The Ji> 0{J}_{i}>~0Ji​> 0 are independent random variables obeying a probability distribution P(J)P(J)P(J), and $0<~\ensuremath{\gamma}<~\ensuremath{\infty}$. The approach used is a numerical implementation of a real-space renormalization-group (RG) method previously introduced. The isotropic Heisenberg case ($\ensuremath{\gamma}=1$), the XY\mathrm{XY}XY case ($\ensuremath{\gamma}=0$). and the Ising case ($\ensuremath{\gamma}=\ensuremath{\infty}$) are fixed points of the RG transformation. It is found that in the XY\mathrm{XY}XY region $\ensuremath{\gamma}<~1$, including the Heisenberg point, the system exhibits singular behavior in the thermodynamic properties for arbitrary probability distributions for the couplings. For the XY\mathrm{XY}XY limit ($\ensuremath{\gamma}=0$) this is in agreement with known exact results. The functional form for the low-temperature susceptibility is found to be $\ensuremath{\chi}\ensuremath{\sim}\frac{1}{(T{\mathrm{ln}}^{m}(\frac{T}{{T}_{0}}))}$ in the entire region $0<~\ensuremath{\gamma}<~1$ for arbitrary probability distributions. In the Ising region ($\ensuremath{\gamma}>1$) the susceptibility shows an approximate power-law divergence for small anisotropy but goes eventually to zero as $T\ensuremath{\rightarrow}0$. Possible relevance of these results to recent experiments on Qn(TCNQ)2{(\mathrm{TCNQ})}_{2}(TCNQ)2​ is discussed.
The low energy properties of the spin-1/2 random Heisenberg chain with ferromagnetic and antiferromagnetic interactions are studied by means of the density matrix renormalization group (DMRG) and real space renormalization group (RSRG) method for finite chains. The results of the two methods are consistent with each other. The deviation of the gap distribution from that of the random singlet phase and the formation of the large-spin state is observed even for relatively small systems. For a small fraction of the ferromagnetic bond, the effect of the crossover to the random singlet phase on the low temperature susceptibility and specific heat is discussed. The crossover concentration of the ferromagnetic bond is estimated from the numerical data.
We introduce variants of the Ma-Dasgupta renormalization-group (RG) approach for random quantum spin chains, in which the energy-scale is reduced by decimation built on either perturbative or non-perturbative principles. In one non-perturbative version of the method, we require the exact invariance of the lowest gaps, while in a second class of perturbative Ma-Dasgupta techniques, different decimation rules are utilized. For the S = 1 random antiferromagnetic Heisenberg chain, both type of methods provide the same type of disorder dependent phase diagram, which is in agreement with density-matrix renormalization-group calculations and previous studies.