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Nano Letters

Tunneling-Induced Spectral Broadening of a Single Atom in a Three-Dimensional Optical Lattice

Wookrae Kim, Changwon Park, Jung-Ryul Kim, Youngwoon Choi, Sungsam Kang, Sooin Lim, Yea‐Lee Lee, Jisoon Ihm, Kyungwon An

Published Dec 31, 2010• 10 citations
Publisher

Abstract

We have investigated the spectral broadening in the near-resonance fluorescence spectrum of a single rubidium atom trapped in a three-dimensional (3D) optical lattice in a strong Lamb-Dicke regime. Besides the strong Rayleigh peak, the spectrum exhibited weak Stokes and anti-Stokes Raman sidebands. The line width of the Rayleigh peak for low potential depths was well explained by matter-wave tunneling between the first-two lowest vibrational states of 3D anisotropic harmonic potentials of adjacent local minima of the optical lattice.

DOI
10.1021/nl103858x

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We have investigated the spectral broadening in the near-resonance fluorescence spectrum of a single rubidium atom trapped in a three-dimensional (3D) optical lattice in a strong Lamb-Dicke regime. Besides the strong Rayleigh peak, the spectrum exhibited weak Stokes and anti-Stokes Raman sidebands. The line width of the Rayleigh peak for low potential depths was well explained by matter-wave tunneling between the first-two lowest vibrational states of 3D anisotropic harmonic potentials of adjacent local minima of the optical lattice.
We form a 1D optical lattices for Cs atoms using light tuned a few thousand linewidths below the 6S1/2(F equals 4) yields 6P3/2(F' equals 5) transition at 852 nm. In this far-off- resonance lattice the time scale for damping of motional coherences and kinetic energy can be orders of magnitude longer than the vibrational oscillation period for atoms trapped in the lattice potential wells. Atoms are loaded directly into deeply bound states, by adiabatic transfer from a superimposed, near-resonance optical lattice. This yields a mean vibrational excitation n approximately equals 0.3, and localization (Delta) z approximately (lambda) /20 deep in the Lamb-Dicke regime. Light scattering subsequently heats the atoms, but the initial rate is only of order 10-3 vibrational quanta per oscillation period. Low vibrational excitation, localization in the Lamb-Dicke regime and low heating rates make these atoms good candidates for resolved- sideband Raman cooling, and for the generation and study of non-classical states of center-of-mass motion. We propose a scheme for resolved-sideband Raman cooling and quantum state preparation; the scheme employs Raman coupling between magnetic sublevels induced by the lattice light field itself.
We have observed quantized motion of rubidium atoms spatially confined by dipole forces inside microscopic light traps. A cubic lattice of such traps is formed by three mutually orthogonal standing waves. We compare 2D and 3D confinement in the same experiment by observing the absorption of a weak probe laser beam. In both cases we observe Raman transitions between vibrational levels and a central Rayleigh resonance. When we switch to 3D confinement the line width of this Rayleigh resonance dramatically decreases to values below 1 kHz.
We investigate theoretically the spectrum of resonance fluorescence of a harmonically trapped atom, whose internal transitions are $\ensuremath{\Lambda}$ shaped and driven at two-photon resonance by a pair of lasers, which cool the center-of-mass motion. For this configuration, photons are scattered only due to the mechanical effects of the quantum interaction between light and atom. We study the spectrum of emission in the final stage of laser cooling, when the atomic center-of-mass dynamics is quantum mechanical and the size of the wave packet is much smaller than the laser wavelength (Lamb-Dicke limit). We use the spectral decomposition of the Liouville operator of the master equation for the atomic density matrix and apply second-order perturbation theory. We find that the spectrum of resonance fluorescence is composed of two narrow sidebands---the Stokes and anti-Stokes components of the scattered light---while all other signals are in general orders of magnitude smaller. For very low temperatures, however, the Mollow-type inelastic component of the spectrum becomes visible. This exhibits novel features which allow further insight into the quantum dynamics of the system. We provide a physical model that interprets our results and discuss how one can recover temperature and cooling rate of the atom from the spectrum. The behavior of the considered system is compared with the resonance fluorescence of a trapped atom whose internal transition consists of two levels.
We investigate the resonance fluorescence emission and absorption spectra for a one-dimensional harmonically trapped two-level ion. The master equation is used to generate the atomic polarizations from which the spectra are derived. Because of their size, the final density matrix equations are investigated numerically. The calculations are carried out in the Lamb-Dicke limit of tight localization of the ion. Sharp peaks are found to appear in the spectra at frequencies detuned from line centre by steps of the trap frequency. The frequency of the peaks and their superposition with Rabi sidebands above saturation are analysed for a variety of parameter ranges. Moreover, new features of the absorption spectra of a weak probe such as sharp gain regions around the trap sidebands are also discussed.
The possibility of using ultracold atoms to observe strong localization of matter waves is now a subject of great interest, as undesirable decoherence and interactions can be made negligible in these systems. It was proposed that a static-disordered potential can be realized by trapping atoms of a given species in randomly chosen sites of a deep three-dimensional (3D) optical lattice with no multiple occupation. We analyze in detail the prospects of this scheme for observing localized states in 3D for a matter wave of a different atomic species that interacts with the trapped particles and that is sufficiently far detuned from the optical lattice to be insensitive to it. We demonstrate that at low energy a large number of 3D strongly localized states can be produced for the matter wave, if the effective scattering length describing the interaction of the matter wave with a trapped atom is of the order of the mean distance between the trapped particles. Such high values of the effective scattering length can be obtained by using a Feshbach resonance to adjust the free-space interspecies scattering length and by taking advantage of confinement-induced resonances induced by the trapping of the scatterers in the lattice.