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Physical Review A

Path-integral analysis of the time delay for wave-packet scattering and the status of complex tunneling times

D. Sokolovski, J. N. L. Connor

Published Dec 1, 1990• 74 citations
Publisher

Abstract

The wave-packet simulation (WPS) method for calculating the time a tunneling particle spends inside a one-dimensional potential barrier is reexamined using the Feynman path-integral technique. Following earlier work by Sokolovski and Baskin [Phys. Rev. A 36, 4604 (1987)], the tunneling (or traversal) time ${\mathit{t}}_{\mathrm{pack}}^{\mathit{T}}$ is defined as a matrix element of a classical nonlocal functional between two states that represent the initial and transmitted wave packets. These states do not lie on the same orbit in Hilbert space; as a result, ${\mathit{t}}_{\mathrm{pack}}^{\mathit{T}}$ is complex-valued. It is shown that Re${\mathit{t}}_{\mathrm{pack}}^{\mathit{T}}$ reduces to the standard WPS result, ${\mathit{t}}_{\mathrm{phase}}^{\mathit{T}}$, for conditions similar to those employed in the conventional WPS analysis. Similarly, Im${\mathit{t}}_{\mathrm{pack}}^{\mathit{T}}$ is shown to contain information about the energy dependence of the transmission probability. Under semiclassical conditions, Im${\mathit{t}}_{\mathrm{pack}}^{\mathit{T}}$ reduces to the well-known Wentzel-Kramers-Brillouin expression for the tunneling time. It is shown there are different definitions for the traversal time of a classical moving object, whose size is comparable to the width of the region of interest. In the quantum case, these different definitions correspond to different ways of analyzing the WPS experiment. The path-integral approach demonstrates that the tunneling-time problem is one of understanding the physical significance of complex-valued off-orbit matrix elements of an operator or functional. The physical content of complex-valued tunneling times is discussed. It is emphasized that the use of complex tunneling times includes real-time approaches as a special case. Nevertheless, there is a limitation in the description of tunneling experiments using tunneling times, whether real or complex. The path-integral approach does not supply a universal traversal time, analogous to a classical time, that can be used in quantum situations. It is demonstrated that the often expressed hope of finding a well-defined and universal real tunneling time is erroneous.

DOI
10.1103/physreva.42.6512

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The wave-packet simulation (WPS) method for calculating the time a tunneling particle spends inside a one-dimensional potential barrier is reexamined using the Feynman path-integral technique. Following earlier work by Sokolovski and Baskin [Phys. Rev. A 36, 4604 (1987)], the tunneling (or traversal) time tpackT{\mathit{t}}_{\mathrm{pack}}^{\mathit{T}}tpackT​ is defined as a matrix element of a classical nonlocal functional between two states that represent the initial and transmitted wave packets. These states do not lie on the same orbit in Hilbert space; as a result, tpackT{\mathit{t}}_{\mathrm{pack}}^{\mathit{T}}tpackT​ is complex-valued. It is shown that RetpackT{\mathit{t}}_{\mathrm{pack}}^{\mathit{T}}tpackT​ reduces to the standard WPS result, tphaseT{\mathit{t}}_{\mathrm{phase}}^{\mathit{T}}tphaseT​, for conditions similar to those employed in the conventional WPS analysis. Similarly, ImtpackT{\mathit{t}}_{\mathrm{pack}}^{\mathit{T}}tpackT​ is shown to contain information about the energy dependence of the transmission probability. Under semiclassical conditions, ImtpackT{\mathit{t}}_{\mathrm{pack}}^{\mathit{T}}tpackT​ reduces to the well-known Wentzel-Kramers-Brillouin expression for the tunneling time. It is shown there are different definitions for the traversal time of a classical moving object, whose size is comparable to the width of the region of interest. In the quantum case, these different definitions correspond to different ways of analyzing the WPS experiment. The path-integral approach demonstrates that the tunneling-time problem is one of understanding the physical significance of complex-valued off-orbit matrix elements of an operator or functional. The physical content of complex-valued tunneling times is discussed. It is emphasized that the use of complex tunneling times includes real-time approaches as a special case. Nevertheless, there is a limitation in the description of tunneling experiments using tunneling times, whether real or complex. The path-integral approach does not supply a universal traversal time, analogous to a classical time, that can be used in quantum situations. It is demonstrated that the often expressed hope of finding a well-defined and universal real tunneling time is erroneous.
The precise definition and physical interpretation of a tunneling time is a fundamental problem in quantum mechanics. The lack of a well-defined time operator in quantum theory precludes the calculation of time in terms of an expectation value. Consequently, model calculations and simulation studies have been proposed and used to determine the time for a particle to traverse a quantum-mechanical barrier. The results offer both qualitatively and quantitatively, disparate predictions. One of the more commonly used approaches is the phase method, which we have applied to several one-dimensional model potentials to show that the tunneling time is characterized by the ratio of the typical decay length in the barrier to the incident velocity, τ∼(1/κ)/v0. We also show that the phase and the spin precession methods are equivalent when the magnetic field is applied throughout the space containing the particle wave function and the tunneling barrier. In principle, the spin precession method can be regarded as an operational definition of the tunneling time. It also has been shown that a tunneling time can be defined operationally for a time-dependent barrier, for which the model calculations predict a tunneling time given by the mean barrier width divided by the magnitude of the imaginary velocity of the particle in the barrier, τ∼d/‖v‖. This pseudokinematic result has been inferred by magnetic field dependent tunneling through heterostructures and computer simulation of wave packet tunneling through one-dimensional square barriers. Other tunneling time theories predict one or the other of the above mentioned characteristic times; several theories predict both. We interpret these different results for τ to mean that a tunneling time is not uniquely defined as a function of particle energy and the barrier shape unless the process in which the tunneling is involved is also specified. That is, the tunneling time is a meaningful and unique concept only for particular tunneling processes or definite operational procedures.
Quantum tunneling, a quintessential quantum phenomenon, challenges classical intuitions by allowing particles to pass through seemingly insurmountable barriers. This study delves into the intricate dynamics of electron tunneling, focusing on the critical role of sub-barrier interactions and complex time processes. Through a combination of experimental measurements and simulations based on Feynman’s path integral of complex time trajectories, we reveal that the sub-barrier potential interaction introduces an asymmetric electron wave packet probability distribution along the real time axis and a marked delay at the tunneling exit. The energy-dependent behavior of this delay in electronic tunneling agrees with that observed in the previous atomic tunneling studies, suggesting a universal mechanism underlying quantum tunneling across different scales. Our findings underscore the necessity of incorporating both the wave and particle aspects of quantum entities to fully comprehend tunneling dynamics, which holds promise for an intuitive interpretation of complex-number quantum processes.
The quantum traversal time ${t}_{\ensuremath{\Omega}}$ is obtained as a matrix element of the classical functional in Feynman path-integral technique. The properties of ${t}_{\ensuremath{\Omega}}$ and its relation to the observables in scattering experiments are investigated. The general expression for the tunneling time is found in the one-dimensional case. Various traversal times of previous works are shown to be simply related to ${t}_{\ensuremath{\Omega}}$ as Re${t}_{\ensuremath{\Omega}}$, Im${t}_{\ensuremath{\Omega}}$, or \ensuremath{\Vert}${t}_{\ensuremath{\Omega}}$\ensuremath{\Vert}. Other possible constructions of time parameters describing the motion of a quantum particle are discussed.
An alternative model for near-field propagation and optical tunneling is proposed following the lines of the path-integral method developed by Feynman, and in particular by using a transition-elements analysis. Such a model was able to account for the frequency dependency of delay-time results of an experiment involving microwave propagation in the near field using two horn antennas [A. Ranfagni et al., Phys. Rev. E 66, 036111 (2002)]. Furthermore, this approach is also capable of interpreting delay-time results as a function of the barrier width in a frustrated total internal reflection experiment performed at the microwave scale and in the optical region.
A new variant of the packet analysis to solve the tunneling time problem for the so-called completed elastic scattering (a potential barrier of an arbitrary form is located in the finite spatial interval) is presented. In particular, we propose an explanation of the "paradoxes" of wave packet tunneling, and elaborate a rule enabling one to extract the tunneling times for a particle from the analysis of tunneling the corresponding wave packet. It is shown that the quantum ensembles of transmitted and reflected particles are statistically independent not only after the scattering but also before this event. We find the corresponding counterparts for the transmitted and reflected packets, which describe separately both scattering channels at early times, and define the expectation values of delay times for each channel. Besides, to describe jointly all particles at the stage when they cannot be divided into two independent subensembles, we find the scattering time taking into account broadening the packets. We derive the condition to be satisfied for the completed scattering. The times above are defined in terms of the well-known quantum-mechanical averages for the position and wave-number operators.