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Advanced Materials

Time‐frequency domain optical storage in rare‐earth‐doped materials

Ravinder Kachru, Yu Bai, Xiao‐An Shen

Published Oct 1, 1994• 0 citations
Publisher

Abstract

The storage of information in the time domain through the use of spectral hole burning rare‐earth‐doped crystals is described. The technique, which is also known as stimulated echo, makes serial read/write data rates of 100 MHz possible. Applications include high‐speed memory, signal processing, high‐speed optical switching, optical interconnects, image processing, and logic operations.

DOI
10.1002/adma.19940061019

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The storage of information in the time domain through the use of spectral hole burning rare‐earth‐doped crystals is described. The technique, which is also known as stimulated echo, makes serial read/write data rates of 100 MHz possible. Applications include high‐speed memory, signal processing, high‐speed optical switching, optical interconnects, image processing, and logic operations.
We describe a new approach to develop a high-speed, high-density random access cache memory. This new technique is based on a novel approach using, in essence, a hybrid of the time domain stimulated echo (SE) concept and the frequency domain scheme. It has been demonstrated that the rare-earth doped crystals, can at low temperatures store large amounts of information for up to 24 hours using SE. The basic approach we have developed is the partitioning of the absorption frequency domain into smaller bins, so that each frequency bin stores a smaller portion of information independently. The bins are distinguishable by their different absorption frequencies and they are accessed by changing the laser frequency (color). However, information is still stored and retrieved using the time-domain pulse sequency used in SE. Specifically, with the laser frequency set at the particular absorption of a frequency bin, the laser is externally modulated by an acousto-optic modulator to produce amplitude modulated pulses representing the digital data, the write pulse, and the read pulse, during the write and retrieve operation, respectively. The advantages of this approach are that memory can be stored in space, time, and frequency domain, allowing us to tailor a flexible memory architecture to match those of the computational processor.
Unique spectroscopic properties of isolated rare earth ions in solids offer optical linewidths rivaling those of trapped single atoms and enable a variety of recent applications. We design rare-earth-doped crystals, ceramics, and fibers with persistent or transient "spectral hole" recording properties for applications including high-bandwidth optical signal processing where light and our solids replace the high-bandwidth portion of the electronics; quantum cryptography and information science including the goal of storage and recall of single photons; and medical imaging technology for the 700-900 nm therapeutic window. Ease of optically manipulating rare-earth ions in solids enables capturing complex spectral information in 105 to 108 frequency bins. Combining spatial holography and spectral hole burning provides a capability for processing high-bandwidth RF and optical signals with sub-MHz spectral resolution and bandwidths of tens to hundreds of GHz for applications including range-Doppler radar and high bandwidth RF spectral analysis. Simply stated, one can think of these crystals as holographic recording media capable of distinguishing up to 108 different colors. Ultra-narrow spectral holes also serve as a vibration-insensitive sub-kHz frequency reference for laser frequency stabilization to a part in 1013 over tens of milliseconds. The unusual properties and applications of spectral hole burning of rare earth ions in optical materials are reviewed. Experimental results on the promising Tm3+:LiNbO3 material system are presented and discussed for medical imaging applications. Finally, a new application of these materials as dynamic optical filters for laser noise suppression is discussed along with experimental demonstrations and theoretical modeling of the process.
We are developing a high density, high speed optical memory, using rare-earth doped hole- burning materials. These materials are theoretically capable of achieving storage densities of 1000 Gigabits/cm3 at input/output (I/O) rates of several gigabits/sec. One remarkable attribute of this storage concept is that both the temporal and spatial information encoded on a laser beam can be stored. Because both the temporal and spatial information can be stored, digital data can be recorded serially as a data or packet stream as well as holographically using the page format. During the past year we have achieved a breakthrough in demonstrating random access holographic data storage at high frame rates. Five hundred holograms were stored and retrieved with very good fidelity at 30 Hz (video rate). Each holographic image with 512 multiplied by 488 pixels could be randomly accessed during the storage and retrieval process. This frame rate is the highest demonstrated frame rate for any optical technique. This breakthrough was achieved through the invention of a memory architecture that allows multiple holographic frames to be stored without any mechanical beam scanning. In this new architecture multiplexing of 500 holograms was achieved by stepping the laser frequency over a range covered by high speed acousto-optic modulators (AOM).
Spectral hole burning and photon echoes are the techniques for frequency-selective optical memories, which have the potential to increase areal data storage density by a factor 10**7. They also have the capability to perform in-memory data processing. In this thesis, several materials and techniques for optical memories in the frequency- and time domain have been investigated. In the frequency domain, ways to increase the storage density and the working temperature were studied using photon-gated spectral hole burning materials of the metal-tetrabenzoporphyrin derivatives. A selection rule for the electron acceptors in the donor-acceptor electron transfer systems was deduced. By doping the material with two different donors a maximum inhomogeneous line width of more than 30 THz was achieved. A polarization holographic technique was established for the formation and detection of spectral holes. Our results indicate that this technique can provide a better signal-to-noise ratio than that achieved by a conventional holographic technique, in particular for samples of poor optical quality. In the time domain, magnetic field-induced and the intensity-induced dephasing processes were studied in Pr3+ doped in a YAlO3 crystal and a Y2SiO5 crystal, respectively. As a step along the route to make photon echo based optical processing possible, the amplification of photon echo signals by the use of a fiber amplifier (Pr3+-doped ZBLAN) was demonstrated. A gain of 45 was achieved. The erasure of stored data using photon echoes has also been investigated. A technique to diagnose the phase and frequency stability of a light source by the photon echo erasure process was proposed and illustrated. An approach to bit-selective data erasure, that is free from laser phase and frequency fluctuations, is also suggested. A concept for an arbitrary shape pulse generator based on photon echoes and hole-burning was experimentally and theoretically studied. Finally, a comparison between the properties and capabilities of spectral hole burning and photon echoes was made.
Optical data storage has been interested in several decades because of the potential of fast access time and high-density storage. Recently volume holographic data storage technique has drawn much interest as new materials and improved techniques have developed.1 However, the large of hologram storage is restricted by low diffraction efficiency and mainly focused to read only memory because of the material's characteristic difficult to rewrite in short time interval. Another optical memory technique (photon echo optical memory)2 based on time-domain has developed since 1980's and made big progress for the area of real time image processing and dynamic random access memory. In this technique, data pulses interfere with timely separated write pulse (reference), and their interference pattern is written as population gratings. A read pulse (reference) retrieves each data pulse information as a four-wave mixing process. The write and read pulse separations are restricted by phase and population decay times of the material, respectively, and storage density is determined by the ratio of inhomogeneous to homogeneous linewidths. Even though photon echo technique has advantages of fast access time (≥ ns) and high-density (≥ Mbits/laser spot), its operating temperature is kept extremely low around liquid helium temperature. This is because that homogeneous decay time rapidly shortens as temperature increases due to phonon interactions, i.e., the ratio of inhomogeneous to homogeneous decay rates is ~ 1 at liquid nitrogen temperature (77 K) in a rare-earth doped solid, so that restricts its applications.
The photon-echo memory[1], or the time-domain optical data storage, resembles the hole-burning memory [2] in that the inhomogeneous absorption line of a material is employed as a storage medium and the information is stored in it as a frequency-dependent absorption change with the resolution determined by the homogeneous width. Having the common memory capacity N given by the inhomogeneous-to-homogeneous width ratio, both types of memories share common problems like low-temperature operation, spectral diffusion and so on. Although a storage medium is common, storage techniques are definitely different for the two memories. The photon-echo memory utilizes the temporal interference effect between a reference pulse and a data pulse and their interference pattern is stored as a population grating in the frequency domain. In this sense this is a time-domain analog of holography where the spatial interference pattern between a reference beam and a data beam is stored in a medium as a population grating in the real space. Like the spatially diffracted beam from the read beam gives the information stored in the hologram, the “temporally diffracted pulse", or the photon echo, after the read pulse can give the information stored in the inhomogeneous distribution.