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Physical Review A

Mechanically Chopped γ Rays; Quantitative Treatment of the Sideband Intensities

Stanley L. Ruby, Richard S. Preston, C. E. Skov, B. J. Zabransky

Published Jul 1, 1973• 13 citations
Publisher

Abstract

We report the generation of sidebands in the energy spectrum of 14.4-keV $\ensuremath{\gamma}$ rays by a periodic modulation of the properties of the medium between the emitting and absorbing atoms. The observed spectrum agrees in detail with a "chopping" calculation that encompasses both amplitude and phase modulation, although the modulator may equally well be viewed as a moving multislit grating. This is the first experiment in which the observed sidebands in the $\ensuremath{\gamma}$-ray spectrum have been quantitatively understood.

DOI
10.1103/physreva.8.59

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We report the generation of sidebands in the energy spectrum of 14.4-keV \ensuremathγ\ensuremath{\gamma}\ensuremathγ rays by a periodic modulation of the properties of the medium between the emitting and absorbing atoms. The observed spectrum agrees in detail with a "chopping" calculation that encompasses both amplitude and phase modulation, although the modulator may equally well be viewed as a moving multislit grating. This is the first experiment in which the observed sidebands in the \ensuremathγ\ensuremath{\gamma}\ensuremathγ-ray spectrum have been quantitatively understood.
This study provides a detailed theoretical description of periodic γ -ray intensity signals. These signals are generated by the tabletop time coincidence experimental setups which utilize nuclear resonant interaction of γ -photons from a radioactive source with an absorber exhibiting ultrasonic vibrations. Transmission of the γ -radiation field through the absorber is described by semiclassical theory considering arbitrary periodic motion of the absorber. A key aspect of the presented work is the application of the Fourier analysis. A fundamental relation between the Fourier coefficients of the γ -ray intensity signal and the Fourier coefficients of a complex exponential of the absorber motion is derived. Application of this relation is shown on the example of the trapezoid motion, which demonstrates its usability for systematic inspection of the discussed signals. The results of the analysis expand the knowledge of the coherent manipulation of γ -photons and may find usage in a broad range of research fields utilizing γ -ray sources.
A classical optical theory is given for the phenomenon of $\ensuremath{\gamma}$-ray quantum beats observed by Perlow in a study of the M\"ossbauer effect of a frequency-modulated source. The intensity $I({\ensuremath{\omega}}_{0}\ensuremath{-}{\ensuremath{\omega}}_{0}^{\ensuremath{'}},t)$ of the radiation from such a source transmitted through a resonant absorber is obtained as a function of ${\ensuremath{\omega}}_{0}\ensuremath{-}{\ensuremath{\omega}}_{0}^{\ensuremath{'}}$ and ttt, where ${\ensuremath{\omega}}_{0}^{\ensuremath{'}}$ is the frequency of an absorber resonance, ${\ensuremath{\omega}}_{0}$ is the central frequency of the frequency-modulated source, and ttt is the laboratory time. An average is taken over the unobserved initial formation time of the excited nuclear state in the source. When viewed at fixed ${\ensuremath{\omega}}_{0}\ensuremath{-}{\ensuremath{\omega}}_{0}^{\ensuremath{'}}$, the calculated intensity displays beats in the time spectrum, and when viewed at fixed ttt, the intensity shows dispersion at appropriate values of ${\ensuremath{\omega}}_{0}\ensuremath{-}{\ensuremath{\omega}}_{0}^{\ensuremath{'}}$, responsible for the observed enhancement of intensity above background. The harmonic content of the quantum beats is calculated explicitly in the thin-absorber limit, and the observed linear variation about ${\ensuremath{\omega}}_{0}\ensuremath{-}{\ensuremath{\omega}}_{0}^{\ensuremath{'}}=0$ of the ratio of Fourier components D1D2\frac{{D}_{1}}{{D}_{2}}D2​D1​​ is explained. The use of D1D2\frac{{D}_{1}}{{D}_{2}}D2​D1​​ to measure small frequency shifts is analyzed by a statistical comparison with the method of switching between steepest points of the line, as used in gravitational-red-shift measurements. The variances are comparable. The effect on $I({\ensuremath{\omega}}_{0}\ensuremath{-}{\ensuremath{\omega}}_{0}^{\ensuremath{'}},t)$ of line broadening due to sample inhomogeneities is calculated for a Lorentz distribution of center frequencies in source and absorber, and a prescription is given for modifying the various terms in $I({\ensuremath{\omega}}_{0}\ensuremath{-}{\ensuremath{\omega}}_{0}^{\ensuremath{'}},t)$ accordingly. Finally, the effect of a distribution of phase and amplitude of the motion of the vibrating source is discussed.
Temporal light modulation methods which are of great practical importance in optical technology, are emulated with matter waves. This includes generation and tailoring of matter-wave sidebands, using amplitude and phase modulation of an atomic beam. In the experiments atoms are Bragg diffracted at standing light fields, which are periodically modulated in intensity or frequency. This gives rise to a generalized Bragg situation under which the atomic matter waves are both diffracted and coherently shifted in their de Broglie frequency. In particular, we demonstrate creation of complex and non-Hermitian matter-wave modulations. One interesting case is a potential with a time-dependent complex helicity $[V\ensuremath{\propto}\mathrm{exp}(i\ensuremath{\omega}t)],$ which produces a purely lopsided energy transfer between the atoms and the photons, and thus violates the usual symmetry between absorption and stimulated emission of energy quanta. Possible applications range from atom cooling over advanced atomic interferometers to a new type of mass spectrometer.