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Journal of Nonlinear Optical Physics & Materials

QUANTUM NOISE REDUCTION IN TRAVELLING-WAVE QUASI-PHASE-MATCHED SECOND HARMONIC GENERATION

Juan Ariel Levenson, P. Vidaković

Published Oct 1, 1996• 1 citation
Publisher

Abstract

The present calculation on squeezing capabilities of quadratic nonlinear media in which the phase matching condition is achieved artificially by a periodic poling of the nonlinear susceptibility shows that interesting performance can be obtained for highly integrable and nonlinear materials, using technologies already developed. The origin of squeezing in quasi-phase matched (QPM) media is the cascading of two second order nonlinearities, which at small second harmonic conversion rates has properties similar to a more familiar, purely third order nonlinear effect—Kerr effect.

DOI
10.1142/s0218863596000623

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The present calculation on squeezing capabilities of quadratic nonlinear media in which the phase matching condition is achieved artificially by a periodic poling of the nonlinear susceptibility shows that interesting performance can be obtained for highly integrable and nonlinear materials, using technologies already developed. The origin of squeezing in quasi-phase matched (QPM) media is the cascading of two second order nonlinearities, which at small second harmonic conversion rates has properties similar to a more familiar, purely third order nonlinear effect—Kerr effect.
Cascading of quadratic nonlinearity has been attracting great interests for its potential application to parametric devices, such as phase conjugators or effective Kerr media. In most configurations, the device consists of a single nonlinear element with uniform phase-mismatch. Cascading of several elements with different phase-mismatch has been theoretically investigated and predicted to improve performance of the device for classical applications. In this paper, amplitude squeezing in second-harmonic generation using cascaded quadratic nonlinear elements is numerically analyzed. The analyses are based on linearization of nonlinear coupling equations, where interacting fields are approximated as plane waves. Phase-mismatch of each element is varied independently and tolerance of squeezing performance to the fluctuation of the phase-mismatch is also investigated. It is predicted that the performance as a squeezing device can be also superior to that of a single element device, if a proper combination of the phase-mismatch of each element is chosen. For the fundamental wave, the tolerance to the fluctuation of the phase-mismatch will improve by nearly tenfold compared with the single element case. For the harmonic wave, squeezing beyond the limit of perfect phase-matched case (3dB) will be available, though the tolerance to the fluctuation of the phase-mismatch is quite small. These improvements can be attributed to the nonlinear phase rotation that keeps squeezed axis coincided with the amplitude phase in a stable manner.
Cascaded nonlinear phase shifts via second-harmonic generation are theoretically studied for quasi-phase-matched (QPM) structures. Both the effective phase mismatch and the structure itself contribute to the resultant nonlinear phase shift. Depending on the sign of the effective phase mismatch, structural contribution may enhance or depress the nonlinear phase shift. The fundamental wave will experience a nonlinear phase shift even if the effective phase matching is satisfied. By properly designing the effective phase mismatch, QPM structures with large material-based phase mismatch may provide large nonlinear phase shifts before saturation.
Parametric down-conversion of light (PDC) in a quasi-phase-matched (QPM) nonlinear crystal can be spectrally very broad when the spatial frequency of periodical poling is linearly chirped. The present day technology makes possible the fabrication of chirped QPM crystals phase-matched for PDC in all optical spectrum. In the low-gain regime this allows for generation of biphotons with the correlation time of the order of a single optical cycle. A natural next step is the study of the PDC light produced by such a crystal in the high-gain regime, where PDC is widely used as a source of squeezed states of light. Up to now only a classical treatment of this regime was undertaken. In the present work we demonstrate a possibility to generate single-cycle squeezing in a chirped QPM nonlinear crystal with squeezing spectrum covering almost all the optical octave.
We analyze squeezing of both the fundamental and harmonic fields undergoing traveling-wave, second-harmonic generation (SHG) in second-order (${\mathrm{\ensuremath{\chi}}}^{(2)}$) nonlinear media. We take into account depletion of the fundamental field as well as the phase mismatch between the fundamental and harmonic fields. The behavior of the quantum noises on the propagating fields is studied by linearizing the nonlinear operator equations around the mean-field values. We first consider the degenerate case that is applicable to type-I phase-matching geometries, obtaining expressions for squeezing in both the fundamental and harmonic fields under the conditions of perfect phase matching and large phase mismatch. We show that in the case of a large phase mismatch, the intensity-dependent self-phase shift of the fundamental field, arising due to cascading of the ${\mathrm{\ensuremath{\chi}}}^{(2)}$ nonlinearity, is responsible for the squeezing generation. We also numerically solve the linearized quadrature-operator equations together with the nonlinear mean-field equations. We find that in the case of a finite phase mismatch the harmonic field can be highly squeezed. This is in contrast to the perfectly phase-matched case where the maximum squeezing is limited to 50%. Finally, we analyze the nondegenerate case that applies to type-II phase-matching geometries. Here we show that the commonly used type-II phase-matched SHG process with the input harmonic field in the vacuum state is equivalent to a type-I SHG process in parallel with a degenerate optical-parametric process. The latter causes squeezing in the mode that is polarized orthogonal to the fundamental beam. In the perfect phase-matching case, the squeezing in the orthogonally polarized mode follows the simple expression S=1-\ensuremath{\gamma}, where \ensuremath{\gamma} is the harmonic conversion frequency.