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Journal of Applied Physics

Dynamical effects and the critical behavior of random-field systems (invited)

Yonathan Shapir

Published Apr 15, 1985• 22 citations
Publisher

Abstract

A variety of phenomena is observed experimentally in random-field (RF) systems realized by the application of an external field to diluted antiferromagnets. At low temperatures, infinitely long hysteretic effects are manifested by the history dependence of the final states: long-range order is observed if the field is applied after cooling, while domain states are reached when field cooled. While no indications for critical fluctuations are detected in 2-D systems, scaling behavior, for both the correlation length and the specific heat, is observed in 3-D systems over an intermediate range of temperatures. The related critical properties seem to be well described by the corresponding ones in the 2-D pure Ising model. The renormalization-group approach, which yields for the equilibrium critical exponents their values of the pure model in d−2 dimensions, is reviewed. A generalization of the dimensional-reduction approach, which accounts self-consistently for renormalized responses of the RF system, is presented. The dynamical effects are implicitly incorporated through the variation in the critical response between the local and the global regimes, associated with short- and long-time scales, respectively. In both regimes the lower critical dimension is found to be d=2 in accordance with stability arguments. The short-time critical behavior indicates a dimensional reduction by one for the 3-D thermal exponents, in agreement with the experimental results.

DOI
10.1063/1.335124

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A variety of phenomena is observed experimentally in random-field (RF) systems realized by the application of an external field to diluted antiferromagnets. At low temperatures, infinitely long hysteretic effects are manifested by the history dependence of the final states: long-range order is observed if the field is applied after cooling, while domain states are reached when field cooled. While no indications for critical fluctuations are detected in 2-D systems, scaling behavior, for both the correlation length and the specific heat, is observed in 3-D systems over an intermediate range of temperatures. The related critical properties seem to be well described by the corresponding ones in the 2-D pure Ising model. The renormalization-group approach, which yields for the equilibrium critical exponents their values of the pure model in d−2 dimensions, is reviewed. A generalization of the dimensional-reduction approach, which accounts self-consistently for renormalized responses of the RF system, is presented. The dynamical effects are implicitly incorporated through the variation in the critical response between the local and the global regimes, associated with short- and long-time scales, respectively. In both regimes the lower critical dimension is found to be d=2 in accordance with stability arguments. The short-time critical behavior indicates a dimensional reduction by one for the 3-D thermal exponents, in agreement with the experimental results.
The critical behavior of random-field systems is characterized by exponentially long relaxation times. They may differ by orders of magnitude and slow modes have to be considered quenched with respect to the faster ones. This requires a drastic modification of the renormalization process in which the degrees of freedom are integrated out. A new replica-space renormalization procedure, to carry out the coarse-graining of the time intervals, is presented. We relate by recursion-relations the effective reduced dimensions of consecutive time scales. Their stable fixed-points yield the apparent dimensionalities for the longest and shortest time scales, which are insensitive to the exact behavior on intermediate scales. For Ising systems we find that d = 2 is the lower critical dimension in both regimes. The thermal exponents for d = 3, in the short-time observable regime, are related to those of the pure system in d = 2. This is consistent with the observations in field-cooled random antiferromagnets of the correlation length exponent nu approx. = 1 (by neutron scattering) and of the symmetric logarithmic divergence in the specific-heat (by linear birefringence). 17 refs., 3 figs.
The thermal critical properties of random-field systems in the observable, linear, local-response regime are considered. A consistent nonperturbative approach yields an effective reduced dimension $\overline{d}=\frac{[d+\frac{1}{\ensuremath{\nu}(\overline{d})}]}{2}$ for the thermal exponents if $\ensuremath{\alpha}(\overline{d})<~0$. The consequences for Ising systems are particularly reliable at the upper and lower critical dimensions (du.c.d.=6{d}_{\mathrm{u}.\mathrm{c}.\mathrm{d}.}=6du.c.d.​=6 and dl.c.d.=2{d}_{\mathrm{l}.\mathrm{c}.\mathrm{d}.}=2dl.c.d.​=2, respectively) as well as at d=3d=3d=3 where $\ensuremath{\alpha}=0$ (logarithmic divergence). The results are in agreement with measurements on random antiferromagnets of the specific heat (by linear birefringence) and the correlation length (by neutron scattering).
Spin-models in random fields (RFs) are good representations of many impure materials. Their macroscopic collective behaviour is dominated by the fluctuations in the random fields which accumulate on large scales even if the local field is arbitrarily small. This feature is shared by other weakly disordered models, like flux lines or domain walls in random media. We review some of the main theoretical attempts to describe such systems. A modification of Harris’ argument demonstrates that at the critical point the RF disorder is relevant and that (hyper)scaling must be changed. A domain argument invented by Imry and Ma shows that long-range order is not destroyed by weak RFs in more than d=2 dimensions. This result is supported both by a more refined treatment of the domain argument and by considering the roughness of an isolated domain wall due to the randomness. The wall (or flux line) becomes rough due to disorder but if d>2 the wall remains a well-defined object in RF systems. Different approaches are used to calculate the roughness exponent ζ for walls and lines. Some applications of ζ for the description of type-II superconductors and incommensurate systems are given. More detailed calculations are possible for one-dimensional, Bethe-lattice or the hierarchical Dyson model systems, which confirm as a rule the more approximate treatment of the other sections. In one dimension there is an interesting relation between the statistical mechanics of these models and nonlinear dynamics. Non-classical critical behaviour occurs in RF systems for d<6 and is determined in general by three independent exponents which fulfil certain inequalities. The new exponent θ≡yJ>0 is related to the violation of conventional hyperscaling and is determined by the energy ~H0ξ0 of a correlated region of size ξ. In a renormalization group treatment, the temperature T turns out to be a (dangerous) irrelevant variable which is the most prominent property of the systems considered in this review. The irrelevance of thermal fluctuations on large scales produces metastability and hysteresis effects both in the transition region and in the ordered phase, only briefly considered here. These features occur also in other systems with a disordered T=0 fixed point like in the ordered phase of a spin-glass.
The random-field Ising model shows an extreme critical slowdown that has been described by activated dynamic scaling: The characteristic time of relaxation toward equilibrium diverges exponentially with the correlation length $ln\ensuremath{\tau}\ensuremath{\sim}{\ensuremath{\xi}}^{\ensuremath{\psi}}/T$, with $\ensuremath{\psi}$ an a priori unknown barrier exponent. Through a nonperturbative functional renormalization group, we show that for spatial dimensions ddd less than a critical value ${d}_{\text{DR}}\ensuremath{\simeq}5.1$, also associated with dimensional-reduction breakdown, $\ensuremath{\psi}=\ensuremath{\theta}$ with $\ensuremath{\theta}$ the temperature exponent near the zero-temperature fixed point that controls the critical behavior. For d>dDRd>{d}_{\text{DR}}d>dDR​, on the other hand, $\ensuremath{\psi}=\ensuremath{\theta}\ensuremath{-}2\ensuremath{\lambda}$, where $\ensuremath{\theta}=2$ and $\ensuremath{\lambda}>0$ an additional exponent. At the upper critical dimension $d=6,\ensuremath{\lambda}=1$, so that $\ensuremath{\psi}=0$, and activated scaling gives way to conventional scaling. We give a physical interpretation of the results in terms of collective events in real space, avalanches, and droplets. We also propose a way to check the two regimes by computer simulations of long-range one-dimensional systems.
The nonequilibrium dynamics of classical random Ising spin chains with nonconserved magnetization are studied using an asymptotically exact real space renormalization group (RSRG). We focus on random field Ising model (RFIM) spin chains with and without a uniform applied field, as well as on Ising spin glass chains in an applied field. For the RFIM we consider a universal regime where the random field and the temperature are both much smaller than the exchange coupling. In this regime, the Imry-Ma length that sets the scale of the equilibrium correlations is large and the coarsening of domains from random initial conditions (e.g., a quench from high temperature) occurs over a wide range of length scales. The two types of domain walls that occur diffuse in opposite random potentials, of the form studied by Sinai, and domain walls annihilate when they meet. Using the RSRG we compute many universal asymptotic properties of both the nonequilibrium dynamics and the equilibrium limit. We find that the configurations of the domain walls converge rapidly toward a set of system-specific time-dependent positions that are independent of the initial conditions. Thus the behavior of this nonequilibrium system is pseudodeterministic at long times because of the broad distributions of barriers that occur on the long length scales involved. Specifically, we obtain the time dependence of the energy, the magnetization, and the distribution of domain sizes (found to be statistically independent). The equilibrium limits agree with known exact results. We obtain the exact scaling form of the two-point equal time correlation function <S0(t)Sx(t)> and the two-time autocorrelations <S0(t('))S0(t)>. We also compute the persistence properties of a single spin, of local magnetization, and of domains. The analogous quantities for the +/-J Ising spin glass in an applied field are obtained from the RFIM via a gauge transformation. In addition to these we compute the two-point two-time correlation function <S0(t)Sx(t)><S0(t('))Sx(t('))> which can in principle be measured by experiments on spin-glass-like systems. The thermal fluctuations are studied and found to be dominated by rare events; in particular all moments of truncated equal time correlations are computed. Physical properties which are typically measured in aging experiments are also studied, focusing on the response to a small magnetic field which is applied after waiting for the system to equilibrate for a time t(w). The nonequilibrium fluctuation-dissipation ratio X(t,t(w)) is computed. We find that for (t-t(w)) approximately t(alpha)(w) with alpha;<1, the ratio equal to its equilibrium value X=1, although time translational invariance does not hold in this regime. For t-t(w) approximately t(w) the ratio exhibits an aging regime with a nontrivial X=X(t/t(w)) not equal to 1, but the behavior is markedly different from mean field theory. Finally the distribution of the total magnetization and of the number of domains is computed for large finite size systems. General issues about convergence toward equilibrium and the possibilities of weakly history-dependent evolution in other random systems are discussed.
We investigate dimensional reduction, the property that the critical behavior of a system in the presence of quenched disorder in dimension ddd is the same as that of its pure counterpart in $d\ensuremath{-}2$, and its breakdown in the case of the random-field Ising model in which both the interactions and the correlations of the disorder are long ranged, i.e., power-law decaying. To some extent the power-law exponents play the role of spatial dimension in a short-range model, which allows us to probe the theoretically predicted existence of a nontrivial critical value separating a region where dimensional reduction holds from one where it is broken, while still considering the physical dimension d=3d=3d=3. By extending our recently developed approach based on a nonperturbative functional renormalization group combined with a supersymmetric formalism, we find that such a critical value indeed exists, provided one chooses a specific relation between the decay exponents of the interactions and of the disorder correlations. This transition from dimensional reduction to its breakdown should therefore be observable in simulations and numerical analyses, if not experimentally.