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Bulletin of the Russian Academy of Sciences Physics

Simulation of coherent responses of resonant media excited by a series of ultrashort laser pulses

Alexey Tiranov, Каримуллин Камиль Равкатович, В. В. Самарцев

Published Mar 1, 2012• 1 citation
Publisher

Abstract

A technique for the numerical simulation of coherent optical responses of the photon echo type formed in resonance media with strong inhomogeneous broadening under the action of femtosecond laser pulses is developed. This approach is based on solving the Maxwell-Bloch equations using the finite-difference time-domain (FDTD) method without application of a fast rotating field and slowly varying envelope approximations. The method can be used to simulate coherent responses in different resonance media with a complex structure of energy levels. The technique was validated using the example of describing experiments on narrowing a photon echo pulse and femtosecond echo processing.

DOI
10.3103/s1062873812030331

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A technique for the numerical simulation of coherent optical responses of the photon echo type formed in resonance media with strong inhomogeneous broadening under the action of femtosecond laser pulses is developed. This approach is based on solving the Maxwell-Bloch equations using the finite-difference time-domain (FDTD) method without application of a fast rotating field and slowly varying envelope approximations. The method can be used to simulate coherent responses in different resonance media with a complex structure of energy levels. The technique was validated using the example of describing experiments on narrowing a photon echo pulse and femtosecond echo processing.
We present a one-dimensional iterative predictor-corrector finite-difference time-domain method for modeling of broadband optical pulse propagation and interaction with inhomogeneously broadened materials. The simulator is used to demonstrate two- and three-pulse photon echoes resulting from bandwidth limited pulse and matched chirp interactions with a material modeled with hundreds of equally spaced, discrete spectral lines of detuning. The results are illustrated as Bloch-sphere evolution movies.
Propagation and amplification of an ultrashort laser pulse in a two-level medium is numerically investigated with the use of the finite-difference time-domain (FDTD) procedure simultaneously solving Maxwell and Schrodinger equations with no assumptions characteristic of slowly varying envelope approximation. Comparison of the results of FDTD numerical simulations with the predictions of the pulse area theorem has demonstrated that the developed numerical procedure provides an adequate description of pulse evolution in a two-level medium. Amplification of ultrashort light pulses in a two-level medium is analyzed. Two methods of improving the gain of ultrashort pulses in a two-level medium by modulating the spatial distribution of dipole moments of resonant transitions and using initially chirped frequency-detuned pulses are explored.
Recent progress in ultrafast technology has led to the generation of optical pulses as short as 8 fs. The propagation of such short pulses in nonlinear optical media requires new computational techniques in which the standard approximations such as the slowly-varying envelope approximation (SVEA) and rotating-wave approximation (RWA) are not made while using the Maxwell-Bloch equations [1]. Previous calculations, which used the finite-difference time-domain (FDTD) method, found that for a a Kerr-like instantaneous nonlinearity [2] significant differences can occur when the full vector Maxwell equations are used instead of the nonlinear Schrodinger equation. Recently, the FDTD method has been extended to the case of a homogeneously broadened two-level atomic system [3].
Important applications in optical information storage and processing based on photon echo have been developed.An accurate and effective numerical method to solve the Maxwell-Bloch equations that are used to describe the optical pulse propagation and interaction with inhomogeneously broadened two-level medium will be introduced.Two-pulse photon echo is calculated then photon echo and multiple-pulse photon echoes are stimulated in optical thin(thick) media by using the method,and the physical properties of those echoes are analyzed.The results show that the approach to storage and retrieval of light using multiple-pulse photon echoes based on stimulated photon echo is an effective mode.
An accurate and effective numerical method is presented to solve the Maxwell-Bloch equations that are used to describe the optical pulse propagation and interaction with inhomogeneously broadened two-level medium.The convergence and stability of this numerical method are proved by comparing with the analytic solutions and area theorem derived under special condition.The simulations of arbitrary conditions is discussed by employing this method and analyze the pulse evolution for different detunings,relaxation times and inhomogeneously broadened linewidthes.The established numerical method provides a good way to have further study about the coherent interaction of short optical pulses with resonant mediums,and can be used to solve the corrections of Maxwell-Bloch equations.
Summary form only given. Coherent optical transients such as photon echo are a versatile method far measurement of the homogeneous absorption spectrum of molecular systems in the presence of strong inhomogeneous broadening. Such experiments require measurement of the decay of the optical coherence, typically accomplished by gradually varying the time delay between the excitation pulses. Time-domain information is then Fourier transformed to frequency domain by a computer. In this paper we demonstrate a new method that yields the homogeneous spectrum in a single shot of femtosecond laser pulse illumination by performing Fourier transformation of coherent optical transient signal with a lens. We apply this method to measure the homogeneous spectrum of dye molecules in a polymer film in a broad range of temperatures.