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Optics and Spectroscopy

Fluorescence of a two-level atom in a two-dimensional photonic crystal in the vicinity of the saddle point of the photonic band spectrum

E. Yu. Perlin

Published Mar 1, 2005• 1 citation
Publisher

Abstract

The fluorescence of a two-level atom embedded into a two-dimensional photonic crystal is considered under the assumption that the electronic transition frequency ω 10 is close to the photonic mode frequency ω 0 in the saddle critical point of the photonic spectrum. In this case, the density of photonic states has a logarithmic peak, which manifests itself in a considerable rearrangement of the fluorescence spectrum. The Green’s function of the electron-photon system, which contains the description of the dynamics of spectroscopic transitions and the shape of fluorescence spectra, is obtained in the rotating field approximation. Using the Green’s function, the frequency-dependent Lamb shift and the broadening of the atomic transition are calculated. The shape of the fluorescence spectra is studied. At a large oscillator strength of the atomic transition, the fluorescence line splits into two components in the vicinity of the singularity caused by the saddle critical point. This splitting is associated with a specific Fano-type resonance between the discrete spectrum (the atomic states) and the continuum (the dispersion of photons with a saddle critical point). At small detunings δ = ω 10 -ω 0 , the components of the fluorescence line have considerably different intensities. As δ increases, the spectral positions of the strong and weak components tend to the frequencies of the atomic transition and the saddle point, respectively. The results obtained show that two-level atoms (or quantum dots) can be used as specific probes of the band spectra of photonic crystals.

DOI
10.1134/1.1890506

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The fluorescence of a two-level atom embedded into a two-dimensional photonic crystal is considered under the assumption that the electronic transition frequency ω 10 is close to the photonic mode frequency ω 0 in the saddle critical point of the photonic spectrum. In this case, the density of photonic states has a logarithmic peak, which manifests itself in a considerable rearrangement of the fluorescence spectrum. The Green’s function of the electron-photon system, which contains the description of the dynamics of spectroscopic transitions and the shape of fluorescence spectra, is obtained in the rotating field approximation. Using the Green’s function, the frequency-dependent Lamb shift and the broadening of the atomic transition are calculated. The shape of the fluorescence spectra is studied. At a large oscillator strength of the atomic transition, the fluorescence line splits into two components in the vicinity of the singularity caused by the saddle critical point. This splitting is associated with a specific Fano-type resonance between the discrete spectrum (the atomic states) and the continuum (the dispersion of photons with a saddle critical point). At small detunings δ = ω 10 -ω 0 , the components of the fluorescence line have considerably different intensities. As δ increases, the spectral positions of the strong and weak components tend to the frequencies of the atomic transition and the saddle point, respectively. The results obtained show that two-level atoms (or quantum dots) can be used as specific probes of the band spectra of photonic crystals.
Steady state resonance fluorescence spectra from a two-level atom embedded in a photonic bandgap crystal and resonantly driven by a classical pump light are calculated. The photonic crystal is considered to be with a small bandgap which is in the order of magnitude of the Rabi frequency and is modeled by the anisotropic two-band dispersion relation. Non-Markovian noises caused by the non-uniform distribution of photon density states near the photonic bandgap are taken into account by a new approach which linearizes the optical Bloch equations by using the Liouville operator expansion. Fluorescence spectra that only exhibit sidebands of the Mollow triplet are found, indicating that there is no coherent Rayleigh scattering process.
The effect of atomic position on the spontaneous emission and optical spectra of a three-level atom embedded in a photonic crystal was studied by considering the coherent two-band photonic-band-gap (PBG) reservoir. With the definite phase difference between the fields of the air band and dielectric band in this coherent PBG reservoir, we found that this coherent property grows stronger and results in the spectrum shift and the appearance of dark lines and kinks as the width of band gap gets smaller; and the variation of the atomic position leads to large shift of spectral peak. The averaged spectra of the system with an ensemble of atoms embedded in the dielectric region are blueshifted while those of atoms in the air region are redshifted. The spectra peaks can even shift more than 75% of the half width at half maximum. The feasible experimental systems composed of an ensemble of molecules (quantum dots or fluorescence dye) in photonic crystals are discussed.
In contrast to the situation in free space where the Markovian approximation and the quantum regression theorem are valid, the atom-photon interaction in photonic bandgap materials is in general nonMarkovian. In the present paper we treat the photonic crystals as background reservoirs and introduce the nonuniform noise operators caused by such nonuniform DOS distributions near the band edge. The steady state fluorescence spectrum of a two-level atom embedded in a three-dimensional photonic bandgap crystal and driven by a monochromatic classical electrical field is calculated theoretically for the first time as we known. With the help of the Liouville operator expansion, we can calculate the stationary two-time correlation functions of the atomic operators as well as the spectral distribution of the resonance fluorescence. We also use various dispersion relations to model this nonuniform DOS distribution near the bandgap. We find that if the atomic energy level is far from the bandgap, fluorescence spectra with Mollow triplets are observed.
The spontaneous emission field and spectrum of a two-level atom, located in an isotropic photonic crystal with dynamic band edges, are investigated by means of numeric calculation. The investigation is expected to help comprehend the characteristics of the atomic spontaneous emission in the dynamic photonic crystal, and provide a possible way to control dynamically the spontaneous emission in photonic crystal. The expression of the spontaneous radiation field is obtained without using the far-zone approximation and the Weisskopf-Wigner approximation, and expected to be applicable in other relevant researches. In the investigation, the spontaneous radiation field and spectrum are calculated when the band edge frequency is unmodulated, or modulated by a step function or triangle function. In the unmodulated situation, the radiation field intensity tends to a constant which is equal to the intensity of the localized field component. The radiation field pulse presents a wave packet behavior as propagation distance increases. The components of the radiation field correspond one-to-one to the peaks in the spontaneous radiation spectrum. When the band edge frequency is modulated by step function, the radiation field intensity tends to a steady-state value after the modulation has happened. And the steady-state intensity is affected by the time when the modulation happens. The components of the non-localized field and the frequency of the localized field after modulation depend on the atomic transition frequency and the band edge frequency, and are identical to those in the unmodulated situation with the same parameters. When the band edge frequency is modulated by a triangle function, the field intensity presents a decaying quasi-periodic oscillation after a long enough time. The modulation frequency determines the frequency of the oscillation, and influences the decay rate. The radiation energy becomes sharp peaks around a set of the discrete frequencies which are evenly spaced with the modulation frequency. The central frequency of these frequencies depends on the atomic transition frequency and the value range of the band edge frequency. The modulation initial phase affects the intensity of the radiation field emitted in an initial period of time.
We describe the spectral characteristics of the radiation scattered by two-level atoms (quantum dots) driven by a strong external field, and coupled to a photonic crystal radiation reservoir. We show that in the presence of strong variations with the frequency of the photonic reservoir density of states, the atomic, Mollow, sideband components of the scattered intensity can be strongly modified. Consequently, a weak optical probe field experiences a substantial differential gain in response to slight variations in the intensity of an optical driving field. We suggest that these effects may be of relevance to all-optical transistor action in photonic crystals. Using a specific photonic crystal heterostructure, we suggest that an all-optical microtransistor based on photonic crystals may operate at less than 100nW100\phantom{\rule{0.3em}{0ex}}\text{nW}100nW switching threshold power. Collective NNN-atom effects substantially enhance this optical switching effect. Near the switching threshold intensity, collective effects are manifest in the N2{N}^{2}N2 scaling of the intensity spectrum (reminiscent of superradiance). Above and below this critical region, the gain spectrum widens (linearly with NNN). This correspondingly reduces the switching time scales of the atomic system in response to external fields. Furthermore, the quantum degree of second-order coherence exhibits unusual features. Scattered photons display a variable degree of antibunching as function of driving laser field intensity and the photonic density of states discontinuity. We analyze the effects of the inhomogeneous atomic line broadening on the amplification process. We show, using suitable photonic density of states engineering, that it is possible to select a narrow spectral range around the central frequency of the atomic frequency distribution over which amplification and switching occur. This is done either by spectral decoupling of the active elements from the electromagnetic field (through the introduction of band gaps at specified spectral locations) or through incoherent pumping to selectively saturate atoms outside the spectral region chosen for amplification.
We investigate spontaneous emission from a two-level atom embedded in a photonic crystals with three-dimensional dispersion relation, where the dependence of wave vectors on direction is taken into account. Due to the difference of the density of states of electromagnetic modes between a three-dimensional and a one-dimensional photonic crystal (lack of singularity), the dynamics of the population in the excited state and the emitted field are quite different from those of a one-dimensional photonic crystal. There is no quasi-oscillation for the population evolution. The localized field and the propagating field cannot coexist. When the upper level moves from the gap to the band, the emitted field changes from a localized field to a diffusion field and then to a propagating field. The energy of the diffusion and propagating fields propagates out incoherently and coherently, respectively. An analytical expression for the Lamb shift is obtained. The Lamb shift for the current case is smaller than that in an ordinary vacuum or in one-dimensional photonic crystals.