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Physical Review A

Tunneling-time probability distribution

Randall S. Dumont, T. L. Marchioro II

Published Jan 1, 1993• 80 citations
Publisher

Abstract

Localized wave-packet tunneling through a one-dimensional potential barrier is investigated with respect to the distribution of tunneling times. Specifically, we construct a quantity--- termed the ``tunneled flux''---which has properties of a tunneling-time probability distribution. The tunneled flux is determined completely in terms of the time evolution of an initially localized wave packet. The tunneled flux and the corresponding tunneling-time distributions are investigated analytically via a semiclassical approximation. Additionally, numerical studies are performed with both the semiclassical and quantal versions of the tunneled flux. The semiclassical calculation qualitatively reproduces numerical tunneled fluxes, converging quantitatively as \ensuremath{\Elzxh}\ensuremath{\rightarrow}0. It also provides a wealth of insight into the nature of tunneling processes. Our principle conclusions are as follows: (i) There is an essential disparity between the time- and energy-domain pictures of wave-packet tunneling; (ii) the tunneling-time distribution can be modeled as an exponential of a skewed Lorentzian function, with a width governed primarily by the phase-space asymmetry of the initial wave packet; and (iii) tunneling is faster than simple classical motion from one side of the barrier to another, even assuming an instantaneous transit between the turning points. Effectively, the barrier acts as a filter for the high-momentum components of the initial wave packet.

DOI
10.1103/physreva.47.85

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The Journal of Chemical Physics•Oct 27, 2015•0 citations
Localized wave-packet tunneling through a one-dimensional potential barrier is investigated with respect to the distribution of tunneling times. Specifically, we construct a quantity--- termed the ``tunneled flux''---which has properties of a tunneling-time probability distribution. The tunneled flux is determined completely in terms of the time evolution of an initially localized wave packet. The tunneled flux and the corresponding tunneling-time distributions are investigated analytically via a semiclassical approximation. Additionally, numerical studies are performed with both the semiclassical and quantal versions of the tunneled flux. The semiclassical calculation qualitatively reproduces numerical tunneled fluxes, converging quantitatively as \ensuremath{\Elzxh}\ensuremath{\rightarrow}0. It also provides a wealth of insight into the nature of tunneling processes. Our principle conclusions are as follows: (i) There is an essential disparity between the time- and energy-domain pictures of wave-packet tunneling; (ii) the tunneling-time distribution can be modeled as an exponential of a skewed Lorentzian function, with a width governed primarily by the phase-space asymmetry of the initial wave packet; and (iii) tunneling is faster than simple classical motion from one side of the barrier to another, even assuming an instantaneous transit between the turning points. Effectively, the barrier acts as a filter for the high-momentum components of the initial wave packet.
An interesting analytical expression is obtained for the coordinate probability distribution of a wave packet transmitted through a potential barrier. In the large-time asymptotics the distribution is given in terms of the transmission amplitude and the phase-space quasidistribution of the initial (not necessarily pure) state. The distortion of a (broad) wave packet due to the barrier penetration is determined by two timelike parameters, given by the energy derivative of the complex transmission amplitude. The resulting change of the packet shape reveals a dependence on the detector position and incorporates a possible speed-up effect and a negative dispersion.
The precise definition and physical interpretation of a tunneling time is a fundamental problem in quantum mechanics. The lack of a well-defined time operator in quantum theory precludes the calculation of time in terms of an expectation value. Consequently, model calculations and simulation studies have been proposed and used to determine the time for a particle to traverse a quantum-mechanical barrier. The results offer both qualitatively and quantitatively, disparate predictions. One of the more commonly used approaches is the phase method, which we have applied to several one-dimensional model potentials to show that the tunneling time is characterized by the ratio of the typical decay length in the barrier to the incident velocity, τ∼(1/κ)/v0. We also show that the phase and the spin precession methods are equivalent when the magnetic field is applied throughout the space containing the particle wave function and the tunneling barrier. In principle, the spin precession method can be regarded as an operational definition of the tunneling time. It also has been shown that a tunneling time can be defined operationally for a time-dependent barrier, for which the model calculations predict a tunneling time given by the mean barrier width divided by the magnitude of the imaginary velocity of the particle in the barrier, τ∼d/‖v‖. This pseudokinematic result has been inferred by magnetic field dependent tunneling through heterostructures and computer simulation of wave packet tunneling through one-dimensional square barriers. Other tunneling time theories predict one or the other of the above mentioned characteristic times; several theories predict both. We interpret these different results for τ to mean that a tunneling time is not uniquely defined as a function of particle energy and the barrier shape unless the process in which the tunneling is involved is also specified. That is, the tunneling time is a meaningful and unique concept only for particular tunneling processes or definite operational procedures.
The time behavior of a wave packet, transmitted through a potential barrier, is investigated for all times assuming it to be initially located outside the asymmetric barrier. The survival probability of the initial state, which characterizes the decay of the unstable quantum system in three time domains, is discussed. The presence of initial, exponential, and long-time regimes is a general feature of the decay process. We analytically found the three crucial points of time that separate these regimes. These characteristic times are set by simple formulae, including momentum distribution. It is then shown that the radius of convergence of the cumulant expansion for the survival probability is always small. A long-time behavior of survival probability is described by the asymptotic series whose coefficients decrease with increasing particle energy but at different rates. To be specific, we have examined the exactly solvable model of tunneling through a finite range triangular barrier.
The time evolution of the probability and current densities stemming from an initial state of a particle in the form of a wave packet on the left hand side of a square barrier is studied. In particular, the space distribution at a given time of the above densities is given. Furthermore, the evolution in time at the entrance and exit of the barrier is given. The numerical results show repeated reversal in the current density at the barrier entrance, while being unidirectional at the exit. However, the probability entering the barrier over a long time equals the corresponding probability exiting the barrier. Owing to the fact that the wave packet expands on both of its sides, as time goes by, it is possible to have transmission even if the particle’s initial momentum points away from the barrier. The effect, in question, becomes evident in a diagram for the transmission coefficient in terms of the particle initial momentum, over a relatively small region.
The time independent semiclassical treatment of barrier tunneling has been understood for a very long time. Several semiclassical approaches to time dependent tunneling through barriers have also been presented. These typically involve trajectories for which the position variable is a complex function of time. In this paper, a method is presented that uses only real valued trajectories, thus avoiding the complications that can arise when complex trajectories are employed. This is accomplished by expressing the time dependent wave packet as an integration over momentum. The action function in the exponent in this expression is expanded to second order in the momentum. The expansion is around the momentum, p0(*) , at which the derivative of the real part of the action is zero. The resulting Gaussian integral is then taken. The stationary phase approximation requires that the derivative of the full action is zero at the expansion point, and this leads to a complex initial momentum and complex tunneling trajectories. The "pseudo-stationary phase" approximation employed in this work results in real values for the initial momentum and real valued trajectories. The transmission probabilities obtained are found to be in good agreement with exact quantum results.