The cross sections for singly stimulated two-photon emission and anti-Stokes Raman scattering from the 21S0 metastable state of helium care calculated by a variational procedure for incident photon wavelengths in the range from 5000 AA to 50 mu m.
Multipole interference effects are predicted in the generalized cross sections, and in the ratio $\frac{{\stackrel{^}{\ensuremath{\sigma}}}_{C}}{{\stackrel{^}{\ensuremath{\sigma}}}_{L}}$ of the cross sections for circularly and linearly polarized laser light for the case of the two-photon ionization of the n=2 singlet metastable helium atoms in the wavelength range 5036-5050 \AA{}.
This paper is an extension of a previous one and discusses the theory of the quenching of the metastable 2S state of atomic hydrogen by means of optical radiation, for example by the light from a ruby laser. The case discussed is that for which the incident intensity is sufficiently weak for the usual quantum-electrodynamical perturbation theory to be valid. A procedure developed by Schwartz and others is used to carry out the sum over intermediate states without explicit enumeration. The results are given for a range of incident wavelengths from 5000 \AA{} to 5\ensuremath{\mu}. For unpolarized light from a ruby laser (6934 \AA{}), the total cross section for quenching is found to be ${\ensuremath{\sigma}}_{Q}=1.27\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}22}$ cm2. The cross section for coherent scattering has also been calculated for the same range of wavelengths; for ruby laser light, the total cross section for scattering is found to be ${\ensuremath{\sigma}}_{S}=1.03\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}23}$ cm2.
INTERACTION OF LASER LIGHT WITH THE 2sup1Ssub0 METASTABLE STATE OF HELIUM.