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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Photon statistics and phonon signatures in the quantum light emission from semiconductor quantum dots

Alexander Carmele, Julia Kabuß, Marten Richter, Andreas Knorr

Published Feb 10, 2011• 0 citations
Publisher

Abstract

We present a microscopic description of the photon statistics and phonon signatures in the quantum light emission from semiconductor quantum dots. Using higher-order Born approximation, time-resolved optical emission and scattering spectra are calculated in the weak coupling regime. In the strong coupling regime, a mathematical induction method is presented to calculate the longitudinal optical (LO) phonon-assisted quantum dot cavity-QED. The phonon interaction at room temperature has a strong impact on the quantum correlation of the cavity field and enhances the non-classicality of the cavity field, initially prepared in a thermal state.

DOI
10.1117/12.876367

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We present a microscopic description of the photon statistics and phonon signatures in the quantum light emission from semiconductor quantum dots. Using higher-order Born approximation, time-resolved optical emission and scattering spectra are calculated in the weak coupling regime. In the strong coupling regime, a mathematical induction method is presented to calculate the longitudinal optical (LO) phonon-assisted quantum dot cavity-QED. The phonon interaction at room temperature has a strong impact on the quantum correlation of the cavity field and enhances the non-classicality of the cavity field, initially prepared in a thermal state.
Electron-phonon coupling in semiconductor quantum dots plays a significant role in determining the optical properties of excited excitons, especially the spectral nature of emitted photons. This paper presents a comprehensive theory and analysis of emission spectra from artificial atoms or quantum dots coupled to structured photon reservoirs and acoustic phonons, when excited with incoherent pump fields. As specific examples of structured reservoirs, we chose a Lorentzian cavity and a slow-light coupled-cavity waveguide, which have both been explored experimentally. For the case of optical cavities, we directly compare and contrast the spectra from three well-known and distinct theoretical approaches to treat electron-phonon coupling, including a Markovian polaron master equation, a non-Markovian phonon correlation expansion technique, and a semiclassical linear susceptibility approach, and we point out the limitations of these models. For the cavity-QED polaron master equation, which treats the cavity-mode operator at the level of a system operator, we give closed form analytical solutions to the phonon-assisted scattering rates in the weak excitation approximation, fully accounting for temperature, cavity-exciton detuning, and cavity-dot coupling. We also show explicitly why the semiclassical linear susceptibility approach fails to correctly account for phonon-mediated cavity feeding. For weakly coupled cavities, we calculate the optical spectra using a more general photon reservoir polaron master-equation approach, and explain its differences from the above approaches in the low-QQQ limit of a Lorentzian cavity. We subsequently use this general reservoir approach to calculate the emission spectra from quantum dots coupled to slow-light photonic crystal waveguides, which demonstrate a number of striking photon-phonon coupling effects.
A microscopic theory to study the combined dynamics of a quantum dot exciton coupled to a single cavity mode as well as acoustic phonons is presented. By considering the phonon subsystem in the coherent state representation, the phonon’s impact on the emitted photons is investigated. The single photon emission probability and phonon effects on this quantity are studied. On the other hand, we illustrate that while a quantum dot interacts with a single cavity mode, the collapse and revival phenomenon will occur. It is demonstrated that acoustic phonons have a pronounced impact on the collapse and revival of the quantum dot exciton. Our finding reveals that at elevated temperatures the phonon interaction decreases the Rabi frequency. Moreover, the cavity mode possesses non-classical features such as sub-Poissonian statistics.
The effect of phonons on a nonlinear optical response of a quantum dot-cavity system in quantum strong coupling regime can be accounted for by a fully analytical treatment, provided that the exciton-phonon dynamics is much faster than the exciton-cavity dynamics. Modern experiments involving semiconductor quantum dots embedded in optical microcavities typically meet this criterion. We find that, for a relatively small exciton-cavity coupling, the effect of phonons is concentrated mainly in the polaron shift of the exciton frequency and reduction of exciton-cavity coupling by the Huang-Rhys factor. We have generalized this result to an arbitrary optical nonlinearity and demonstrated a good agreement with the exact solution in a wide range of temperatures. This generalization provides access to higher rungs of the Jaynes-Cummings ladder, where exact numerical approaches are impractical or even impossible. At larger coupling strengths and low temperatures, our approximation is also in good agreement with the exact solution, which makes it a very useful tool for addressing the phonon contribution to the coherent dynamics of a nonlinear optical system. We demonstrate our results for third-order optical polarization with varying observation time and delay time between excitation pulses in the form of two-dimensional spectra. These spectra provide useful information about the coherent coupling between the exciton and the cavity modes. The presented analytical approach is also compared with another useful approximation, having the form of a matrix product, which is a special case of the asymptotically exact solution in the limit of a short phonon memory time.
The generation of photons in a microcavity coupled to a laser-driven quantum dot interacting with longitudinal acoustic (LA) phonons is studied in the regime of simultaneously strong driving and strong dot-cavity coupling. The stationary cavity photon number is found to depend in a nontrivial way on the detuning between the laser and the exciton transition in the dot. In particular, the maximal efficiency of the cavity feeding is obtained for detunings corresponding to transition energies between cavity-dressed states with excitation numbers larger than one. Phonons significantly enhance the cavity feeding at large detunings. In the strong-driving, strong-coupling limit, the photon statistics is highly non-Poissonian. While without phonons a double-peaked structure in the photon distribution is predicted, phonons make the photon statistics thermal-like with very high effective temperatures $\ensuremath{\sim}{10}^{5}$ K, even for low phonon temperatures $\ensuremath{\sim}4$ K. These results were obtained by numerical calculations where the driving, the dot-cavity coupling, and the dot-phonon interactions are taken into account without approximations. This is achieved by a reformulation of an exact iterative path-integral scheme which is applicable to a large class of quantum-dissipative systems and which in our case reduces the numerical demands by 15 orders of magnitude.
We present a semiconductor master equation technique to study the input/output characteristics of coherent photon transport in a semiconductor waveguide-cavity system containing a single quantum dot. We use this approach to investigate the effects of photon propagation and anharmonic cavity-QED for various dot-cavity interaction strengths, including weakly-coupled, intermediately-coupled, and strongly-coupled regimes. We demonstrate that for mean photon numbers much less than 0.1, the commonly adopted weak excitation (single quantum) approximation breaks down, even in the weak coupling regime. As a measure of the multiphoton correlations, we compute the Fano factor and the correlation error associated with making a semiclassical approximation. We also explore the role of electron--acoustic-phonon scattering and find that phonon-mediated scattering plays a qualitatively important role on the light propagation characteristics. As an application of the theory, we simulate a conditional phase gate at a phonon bath temperature of 20 K in the strong coupling regime.