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Physical review. B, Condensed matter

Dynamic spin susceptibility in the resonant-valence-bond state in high- Tc superconductors

K. P. Jain, D. K. Ray

Published Mar 1, 1989• 1 citation
Publisher

Abstract

An approximate expression has been derived for the wave number and frequency-dependent spin susceptibility \ensuremath{\chi}(q,\ensuremath{\omega}) for a system of strongly interacting electrons when the charge and spin degrees of freedom can be separated. This expression has contributions from particle-hole excitations across the pseudo-Fermi surface of the quantum spin fluids as well as from pair excitations.

DOI
10.1103/physrevb.39.4339

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Physical Review B•Aug 31, 2005•23 citations
An approximate expression has been derived for the wave number and frequency-dependent spin susceptibility \ensuremath{\chi}(q,\ensuremath{\omega}) for a system of strongly interacting electrons when the charge and spin degrees of freedom can be separated. This expression has contributions from particle-hole excitations across the pseudo-Fermi surface of the quantum spin fluids as well as from pair excitations.
We consider the slave-fermion--Schwinger-boson decomposition of a t-J model for a two-dimensional antiferromagnet in which the next-nearest-neighbor hopping is taken into account by an explicit t' term. This technique is particularly suitable to describe systems with low hole density, as in the parent phases of high-Tc{\mathit{T}}_{\mathit{c}}Tc​ superconducting (HTSC) materials, and we examine the experimental consequences of the model. Using mean-field states which admit finite spiral and off-diagonal order, we compute first the dynamic susceptibility \ensuremath{\chi}(q,\ensuremath{\omega}) from fluctuations in the boson (spin) degrees of freedom, and investigate a selected parameter regime for the model to seek features consistent with inelastic neutron scattering experiments on underdoped HTSC crystals. We find peaks in the scattered intensity at incommensurate wave vectors (\ensuremath{\pi}\ifmmode\pm\else\textpm\fi{}2k0{\mathit{k}}_{0}k0​,\ifmmode\pm\else\textpm\fi{}\ensuremath{\pi}) and (\ensuremath{\pi},\ifmmode\pm\else\textpm\fi{}\ensuremath{\pi}\ifmmode\pm\else\textpm\fi{}2k0{\mathit{k}}_{0}k0​), but within our approximation the q-integrated susceptibility as a function of frequency and temperature resembles that from spin-wave theory, which does not contain the scaling behavior over all values of \ensuremath{\omega}/T found experimentally. We show also the form of the nuclear magnetic resonance relaxation time ${\mathit{T}}_{1}^{\mathrm{\ensuremath{-}}1}$(T), which measures the zero-frequency limit of the susceptibility. The imaginary part of the physical electron Green function is a convolution of both fermionic (hole) and bosonic Green functions, and so incorporates the effect of spin dynamics on the charge motion. We calculate the photoemitted intensity, a direct experimental measurement of this quantity, focusing on its behavior near the hole pockets at (\ifmmode\pm\else\textpm\fi{}\ensuremath{\pi}/2,\ifmmode\pm\else\textpm\fi{}\ensuremath{\pi}/2) which characterize this type of model. The peak photocurrent occurs not at the hole Fermi surface, but at points separated from it by k0{\mathbf{k}}_{0}k0​ due to the boson incommensuration.
The t–J model with a prohibition of “doubles” (doubly occupied sites) in the lower Hubbard band and holes in the upper band is considered in the regime of strong electron correlations. The specific features of the electronic states are described. An expression is obtained for the transverse dynamic susceptibility χ as a function of wave vector q and frequency ω in the random phase approximation (RPA) in the metallic state of the system, and the static susceptibility (ω=0) is analyzed in the limits q=0 and q=Q=(π,π) in a square lattice as a function of the electron density n. The insulating limit (n→1) is described as a spin liquid (SL) state. An expression for the magnetic susceptibility is proposed which unifies the RPA and the SL concept in the presence of site percolation. It is shown that in a certain concentration region the static susceptibility is negative (i.e., a diamagnetic effect), which indicates the possibility of a superconducting state with an exchange mechanism of pairing.
The t-J-U model of high-Tc copper-oxide superconductors incorporates both the on-site Coulomb repulsion and kinetic exchange interaction and yields a semi-quantitative description of the static properties of those materials. We extend this analysis to dynamic quantities and address collective spin- and charge excitations in the correlated metallic state of the t-J-U model. We employ VWF+1/Nf approach that combines the variational wave function (VWF) approach with the expansion in the inverse number of fermionic flavors (1/Nf). It is shown that the resonant (paramagnon) contribution to the dynamic magnetic susceptibility remains robust as one interpolates between the Hubbard- and t-J-model limits, whereas the incoherent continuum undergoes substantial renormalization. Energy of the collective charge mode diminishes as the strong-coupling limit is approached. We also introduce the concept of effective kinetic exchange interaction that allows for a unified interpretation of magnetic dynamics in the Hubbard, t-J, and t-J-U models. The results are discussed in the context of recent resonant inelastic x-ray scattering experiments for the high-Tc cuprates.
We carry out a systematic study of collective spin and charge excitations for the canonical single-band Hubbard, t–J–U, and t–J models of high-temperature copper-oxide superconductors, both on electron- and hole-doped side of the phase diagram. A~recently developed variational wave function approach, combined with the expansion in the inverse number of fermionic flavors, is employed. All three models exhibit a substantial electron–hole asymmetry of magnetic excitations, with a robust paramagnon emerging for hole-doping, in agreement with available resonant inelastic X-ray scattering data for the cuprates. The t–J model yields additional high-energy peak in the magnetic spectrum that is not unambiguously identified in spectroscopy. For all considered Hamiltonians, the dynamical charge susceptibility contains a coherent mode for both hole- and electron doping, with overall bandwidth renormalization controlled by the on-site Coulomb repulsion. Away from the strong-coupling limit, the antiferromagnetic ordering tendency is more pronounced on the electron-doped side of the phase diagram.
The calculation of the induced spin density of a normal fermion system, such as the electron gas, in the limit of small wave numbers, is carried beyond the random phase approximation (R.P.A.) by the method of canonical transformation so as to include the first non-R.P.A. corrections. An expression for the induced spin density in the same limit, exact to all orders of particle-particle coupling, is then derived by more general methods of many-body perturbation theory. It depends only on the knowledge, to all orders of interparticle coupling, of the effective mass and the forward scattering of quasi-particles at the Fermi surface, and also yields the results of the extended R.P.A. on appropriate expansion. In the limit of zero wave number, the resulting expression for the magnetic susceptibility is found identical with that deduced by Landau from a phenomenological basis and may be regarded as an additional confirmation of the microscopic validity of the theory of the Fermi liquid.
The effects of the electron-phonon interaction on charge and spin dynamics are studied for the one-dimensional two-band Hubbard model by the exact diagonalization method. The parameters of the model are chosen to represent a hole-doped Cu-O system. Local charge fluctuations induced by phonons are expressed in terms of microscopic current and polarization, and it is shown that the dynamic charge transfer is strongly dependent on the phonon wave vector when the system is doped with holes. The dynamic magnetic structure factor is also found to be significantly modified by lattice distortion. In particular the lowest-energy spin excitations are greatly softened, indicating significant spin-phonon coupling. It is shown that the optical response is significantly modified as well due to coupling with the lattice over an energy range far exceeding the phonon energy. These results demonstrate the unconventional nature of the electron-phonon coupling in the strongly correlated electron systems. Its possible implications to the pairing mechanism in the cuprates are discussed.