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The Journal of Chemical Physics

Electromagnetically induced transparency with quantum interferometry

Anindita Bhattacharjee, Krishna Rai Dastidar

Published Feb 23, 2012• 0 citations
Publisher

Abstract

We have shown that electromagnetically induced transparency can be achieved by control-probe interferometry using two delayed phase-locked ultrashort pulses. Two vibrational wavepackets on the excited state, excited by two delayed phase-locked ultrashort pulses, interfere constructively or destructively leading to enhancement or suppression of absorption to a selective set of vibrational levels. Depending on the phase difference and the delay between the pulses with same carrier frequency, one can design different transparency windows between absorption peaks at consecutive even(odd) vibrational levels by eliminating absorption at odd(even) vibrational levels. We have shown that by switching the phase difference of two delayed femtosecond pulses, one can switch to complete elimination of absorption from enhanced absorption to a particular set of vibrational levels in the excited state. Thus, switching of transparency through window between odd vibrational levels to that between even vibrational levels is possible. By properly choosing the temporal width and the carrier frequency of the pulses, lossless transmission of complete or bands of frequencies of the pulses can be achieved through these transparency windows. Hence, designing of single- or multi-mode transparency windows in NaH molecule is feasible by control-probe quantum interferometry.

DOI
10.1063/1.3685419

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We have shown that electromagnetically induced transparency can be achieved by control-probe interferometry using two delayed phase-locked ultrashort pulses. Two vibrational wavepackets on the excited state, excited by two delayed phase-locked ultrashort pulses, interfere constructively or destructively leading to enhancement or suppression of absorption to a selective set of vibrational levels. Depending on the phase difference and the delay between the pulses with same carrier frequency, one can design different transparency windows between absorption peaks at consecutive even(odd) vibrational levels by eliminating absorption at odd(even) vibrational levels. We have shown that by switching the phase difference of two delayed femtosecond pulses, one can switch to complete elimination of absorption from enhanced absorption to a particular set of vibrational levels in the excited state. Thus, switching of transparency through window between odd vibrational levels to that between even vibrational levels is possible. By properly choosing the temporal width and the carrier frequency of the pulses, lossless transmission of complete or bands of frequencies of the pulses can be achieved through these transparency windows. Hence, designing of single- or multi-mode transparency windows in NaH molecule is feasible by control-probe quantum interferometry.
It has been shown that control over the design of single- or multimode-transparency windows can be achieved by control-probe quantum interferometry using two delayed phase-locked ultrashort pulses. We have investigated how single- or multimode-transparency windows can be designed by eliminating the absorption to a set of odd or even vibrational levels of a molecule covered by the spectral bandwidth of the pulses. Suppression of absorption can be achieved by controlling the quantum interference of two vibrational wave packets excited by these two pulses, leading to destructive interference of transition amplitudes for one set of vibrational levels even or odd. Simuntaneously the interference becomes constructive for the other set of odd or even vibrational levels, leading to absorption to these levels. Thus, a set of transparency windows is designed in between two absorption peaks at two consecutive odd (even) vibrational levels by eliminating absorption at even (odd) vibrational levels between two absorption peaks. If the spectral bandwidth of the pulse [full width at half maximum (FWHM)] is less than the energy difference between two consecutive absorption peaks, the pulse will be transmitted without absorption through the transparency window. However, for pulses with a larger spectral bandwidth (FWHM), a set of broad transparency windows will be generated and different bands of pulse frequencies will be transmitted through these windows. We have shown that coherent control of the design of transparency windows can be achieved by controlling pulse duration, carrier frequency, delay, and the phase difference of two ultrashort pulses.
A new scheme is suggested to manipulate the probe transitions (and hence the optical properties of atomic vapors) via double-control destructive and constructive quantum interferences. The influence of phase coherence between the two control transitions on the probe transition is also studied. The most remarkable feature of the present scheme is that the optical properties (absorption, transparency and dispersion) of an atomic system can be manipulated using this double-control multi-pathway interferences (multiple routes to excitation). It is also shown that a four-level system will exhibit a two-level resonant absorption because the two control levels (driven by the two control fields) form a dark state (and hence a destructive quantum interference occurs between the two control transitions). However, the present four-level system will exhibit electromagnetically induced transparency to the probe field when the three lower levels (including the probe level and the two control levels) form a three-level dark state. The present scenario has potential applications in new devices (e.g. logic gates and sensitive optical switches) and new techniques (e.g. quantum coherent information storage).
We propose and analyze an efficient scheme for suppressing the absorption of a weak probe field based on intersubband transitions in a four-level asymmetric coupled-quantum well (CQW) driven coherently by a probe laser field and a control laser field. By using the numerical simulation, we find that the magnitude of the transient absorption of the probe field is smaller than the three-level system based on the electromagnetically induced transparency (EIT) at line center of the probe transition, moreover, comparing with the scheme in three-level asymmetric double QW system, the transparency hole of the present work is much broader. By analyzing the steady-state process analytically and numerically, our results show that the probe absorption can be completely eliminated under the condition of Raman resonance (i.e. two-photon detuning is zero). Besides, we can observe one transparency window without requiring one- or two-photon detuning exactly vanish. This investigation may provide the possible scheme for EIT in solids by using CQW.
The influence of a phase-modulated control field on the phenomenon of electromagnetically induced transparency (EIT) is investigated theoretically. We show that the phase modulation changes the dispersive properties of the medium considerably since it results in temporal oscillations of the transparency window in frequency space. This is in marked contrast to the standard EIT setup, where the transparency window is fixed and determined by the two-photon resonance condition. In particular, we find that the phase modulation enables the propagation of probe pulses with disjoint frequency spectra at different times and allows the shifting of the central frequency of a probe pulse almost without distortion of its shape. We employ the time-dependent susceptibility of the medium to explain and analyze our results and demonstrate that this concept yields qualitative as well as quantitative agreement with the numerical integration of Maxwell-Bloch equations. Our theoretical model can be applied to other media with time-dependent susceptibilities.
Electromagnetically induced transparency suppresses optical absorption through destructive interference, playing a central role in light-matter interaction and quantum information science. We report matter-wave induced transparency, where atomic collisional interactions induce transmission through a lossy molecular potential for the incident atomic scattering waves. Using cesium Bose-Einstein condensates and modulation-induced Feshbach resonances, we realize a three-level atom-molecule coupled system with unprecedented flexibility. Under the dark state condition, a narrow and tunable transparency window appears within a broad dissipative collisional resonance. The transparency window linewidth is controlled by modulation-induced coupling. And scattering pathways are selectable via multifrequency Floquet modulation. These results establish an interference-based route for exploring programmable nonequilibrium and non-Hermitian physics, steering quantum chemistry and precision measurements.
We theoretically investigate the phenomenon of electromagnetically induced transparency (EIT) of a weak probe field in hybrid optomechanics with a single three-level (ΛΛΛ-type) atomic system. We report that, in the presence of optomechanical coupling and two transition coupling parameters of three-level atom (TLA), there occurs three distinct multiple EIT windows in the probe absorption spectrum. Moreover, the switching of multiple windows into double and single EIT windows can be obtained by suitably tuning the system parameters. Furthermore, the probe transmission spectrum have been studied. Based on our analytical and numerical work, we explain the occurrence of slow and fast light (superluminal) regimes, and enhancement of superluminal behaviour in the probe field transmission. This work demonstrates great potential in multi-channel waveguide, fiber optics and classical communication networks, multi-channel quantum information processing, real quality imaging, cloaking devices and delay lines & optical buffers for telecommunication.