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Journal of Applied Physics

Reentrant ferromagnetism in a two-dimensional Ising model with random nearest-neighbor interactions (abstract)

Noureddine Benayad, A. Benyoussef, N. Boccara

Published Apr 15, 1988• 0 citations
Publisher

Abstract

Reentrant behavior seems to be characteristic of systems with competing interactions even when no spin-glass phase exists. Using various methods (finite cluster approximation,1 mean-field renormalization,2 finite cluster renormalization, etc.) we determined the phase diagram of a two-dimensional square Ising model with random nearest-neighbor interactions Jij distributed according to P(Jij)=(1−p)δ(Jij−J)+pδ (Jij−αJ), where J>0 and 0>α>−1. Such a model has been considered by Wolff and Zittartz.3 These authors discussed its qualitative features and argued that a reentrant behavior should be observed. Our calculations agree with this conjecture.

DOI
10.1063/1.340578

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Physical review. B, Condensed matter•Mar 1, 1980•442 citations
Reentrant behavior seems to be characteristic of systems with competing interactions even when no spin-glass phase exists. Using various methods (finite cluster approximation,1 mean-field renormalization,2 finite cluster renormalization, etc.) we determined the phase diagram of a two-dimensional square Ising model with random nearest-neighbor interactions Jij distributed according to P(Jij)=(1−p)δ(Jij−J)+pδ (Jij−αJ), where J>0 and 0>α>−1. Such a model has been considered by Wolff and Zittartz.3 These authors discussed its qualitative features and argued that a reentrant behavior should be observed. Our calculations agree with this conjecture.
Motived by the $H\text{\ensuremath{-}}T$ phase diagram in the bcc Ising antiferromagnetic with nearest-neighbor interactions obtained by Monte Carlo simulation [Landau, Phys. Rev. B 16, 4164 (1977)] that shows a reentrant behavior at low temperature, with two critical temperatures in magnetic field about 2% greater than the critical value Hc=8J{H}_{c}=8JHc​=8J, we apply the effective field renormalization group (EFRG) approach in this model on three-dimensional lattices (simple cubic-sc and body centered cubic-bcc). We find that the critical curve TN(H){T}_{N}(H)TN​(H) exhibits a maximum point around of $H\ensuremath{\simeq}{H}_{c}$ only in the bcc lattice case. We also discuss the critical behavior by the effective field theory in clusters with one (EFT-1) and two (EFT-2) spins, and a reentrant behavior is observed for the sc and bcc lattices. We have compared our results of EFRG in the bcc lattice with Monte Carlo and series expansion, and we observe a good accordance between the methods.
The phase diagrams of the ferromagnetic two-dimensional mixed spin-1 and spin-1/2 Ising model with four-spin interaction J4 and next-nearest couplings J’ are investigated by the use of the finite cluster approximation based on single-site cluster theory. The state equations are derived for the two-dimensional square lattice. The phase diagram is qualitatively and quantitatively different from that obtained when the interaction J’ is ignored. In fact, the system exhibits a variety of interesting features resulting from the introduction of the next-nearest neighbor interaction (NNN). It undergoes two kinds of behavior according to the negative and the positive value of J’. In particular, for J4/J2=-4, the system keeps the coexistence of the two ground state up to J’-dependent finite temperature.
We consider a system of linear chains of Ising spins with short-range nearest-neighbor ferromagnetic interactions of strength K along the chains, and with infinite-range random interchain interactions of a Sherrington-Kirkpatrick type. Also included in the model is a local Gaussian random field with variance \ensuremath{\Delta}. In the replica symmetric case, the system is mapped exactly on the one-dimensional Ising model in a random field and a recursion method for calculating the spin-correlation functions is developed. For \ensuremath{\Delta}=0, an analytic relation for freezing temperature Tf{\mathit{T}}_{\mathit{f}}Tf​(K) is obtained. The replica-symmetric spin-glass phase is shown to be stable above the freezing temperature Tf{\mathit{T}}_{\mathit{f}}Tf​(K,\ensuremath{\Delta}), which is determined numerically.
We introduce a one dimensional Ising model with two competing interactions: nearest neighbor random couplings +/-J with equal probability and a positive infinite range coupling Lambda. At low temperature T the model exhibits a first order phase transition between a ferromagnetic state (with magnetization m(1) = 1 at T = 0) and a << ferrimagnetic >> state (with m(2) = 2/3 at T = 0), when the disorder strength J/Lambda is increased. For 5/12 < J/Lambda < 1, a whole spectrum of ferrimagnetic ground states with magnetization m(n) = 2/(n + 1) (n = 2, ..., infinity) is present while for J/lambda > 1 the ground state is given by a trivial one dimensional spin glass with m = 0. The main qualitative features of the model can be described by a simplified annealed model where the random couplings can arrange themselves to minimize free energy with the constraint that the number of positive couplings is fixed by the law of large numbers in the thermodynamic limit. This model is exactly solved at all temperatures and the diagram of phase is calculated.
The phase diagrams of Ising antiferromagnets in a magnetic field HHH are investigated for various values of the ratio RRR between nearest- and next-nearest-neighbor interaction. While meanfield approximations and the existing real-space renormalization-group treatments yield phase diagrams which are sometimes even qualitatively incorrect, accurate results are obtained from Monte Carlo calculations. For R<0R<0R<0 only an antiferromagnetically ordered phase exists. Its transition to the disordered phase is first order for temperatures below the tricritical point (Tt{T}_{t}Tt​,Ht{H}_{t}Ht​). For $R\ensuremath{\rightarrow}0$ also ${T}_{t}\ensuremath{\rightarrow}0$. For R=0R=0R=0 we find very good agreement with the results of M\"uller-Hartmann and Zittartz. For R>0R>0R>0 and H1<H<H2{H}_{1}<H<{H}_{2}H1​<H<H2​ a new phase with anomalous high ground-state degeneracy is found (two sublattices have only one-dimensional order). These sublattices undergo order-disorder transitions at T=0T=0T=0, such that for T>0T>0T>0 one is left with a "superantiferromagnetic" phase. At low temperatures in this phase a pronounced tendency is observed to form a simpler (2 \ifmmode\times\else\texttimes\fi{} 2) superstructure but with many antiphase domain boundaries. For $R\ensuremath{\rightarrow}\frac{1}{2}$ and H<H1H<{H}_{1}H<H1​ the regime of the antiferromagnetic phases goes to zero temperature, while for R>12R>\frac{1}{2}R>21​ the superantiferromagnetic phase exists also for H<H1H<{H}_{1}H<H1​. The order-disorder transition associated with this phase seems to have non-Ising critical exponents which vary as a function of RRR and HHH. Estimates for the exponents lead us to suggest that Suzuki's "weak universality" is valid. The behavior of the model at T=0T=0T=0 is related to known results on hard-core lattice gases. It is shown that it is useful to interpret the transitions at T=0T=0T=0 as generalized percolation transitions. Since the model may have applications to adsorbate phases in registered structures at (100) surfaces of cubic crystals, the transcription of our results to temperature-coverage phase diagrams and adsorption isotherms is discussed in detail, and possible experimental applications are mentioned.