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Infrared Physics & Technology

Superradiance and Raman scattering in three-level molecular system

A.V. Andreev, Sergei Sheetlin

Published Dec 1, 1996• 0 citations
Publisher
DOI
10.1016/s1350-4495(96)00015-1

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Superradiant Raman scattering of Rubidium atoms has been explored in the experiment [Nature 484, 78 (2012)] to prove the concept of the superradiant laser, which attracts significant attentions in quantum metrology due to the expected ultra-narrow linewidth down to millihertz. To better understand the physics involved in this experiment, we have developed a quantum master equation theory by treating the Rubidium atoms as three-level systems, and coupling them with a dressed laser and an optical cavity. Our simulations show different superradiant Raman scattering pulses for the systems within the crossover and strong coupling regime, and the shifted and broader spectrum of the steady-state Raman scattering. Thus, our studies provide a unified view on the superradiant Raman scattering pulses, and an alternative explanation to the broad spectrum of the steady-state Raman scattering, as observed in the experiment. In future, our theory can be readily applied to study other interesting phenomena relying on the superradiant Raman scattering, such as magnetic field sensing, real-time tracking of quantum phase, Dicke phase transition of non-equilibrium dynamics and so on.

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Superradiant Raman scattering of Rubidium atoms has been explored in the experiment [Nature 484, 78 (2012)] to prove the concept of the superradiant laser, which attracts significant attentions in quantum metrology due to the expected ultra-narrow linewidth down to millihertz. To better understand the physics involved in this experiment, we have developed a quantum master equation theory by treating the Rubidium atoms as three-level systems, and coupling them with a dressed laser and an optical cavity. Our simulations show different superradiant Raman scattering pulses for the systems within the crossover and strong coupling regime, and the shifted and broader spectrum of the steady-state Raman scattering. Thus, our studies provide a unified view on the superradiant Raman scattering pulses, and an alternative explanation to the broad spectrum of the steady-state Raman scattering, as observed in the experiment. In future, our theory can be readily applied to study other interesting phenomena relying on the superradiant Raman scattering, such as magnetic field sensing, real-time tracking of quantum phase, Dicke phase transition of non-equilibrium dynamics and so on.