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The Journal of Chemical Physics

Decoherence in an anharmonic oscillator coupled to a thermal environment: A semiclassical forward-backward approach

Yossi Elran, Paul W. Brumer

Published Jul 23, 2004• 34 citations
Publisher

Abstract

The decoherence of an anharmonic oscillator in a thermal harmonic bath is examined via a semiclassical approach. A computational strategy is presented and exploited to calculate the time dependence of the purity and the decay of individual matrix elements in the energy representation for a variety of initial states. The time dependence of the decoherence is found to depend on the temperature of the bath, the coupling strength, the initial state of the oscillator, and the choice of quantity measuring the decoherence. Recurrences in the purity and in the off-diagonal matrix elements are observed, as well as the collapse of these matrix elements to the diagonal, providing evidence for the retention of quantum coherence for time scales longer than that indicated by the purity. The results are used to analyze the utility of the Caldeira-Leggett and Redfield models of decoherence and to assess the dependence of dephasing rates on the degree of structure in phase space. In several cases we find that the dephasing dynamics can be described as an initial Zeno-effect regime, followed by a Caldeira-Leggett region, followed by recurrences.

DOI
10.1063/1.1766009

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The decoherence of an anharmonic oscillator in a thermal harmonic bath is examined via a semiclassical approach. A computational strategy is presented and exploited to calculate the time dependence of the purity and the decay of individual matrix elements in the energy representation for a variety of initial states. The time dependence of the decoherence is found to depend on the temperature of the bath, the coupling strength, the initial state of the oscillator, and the choice of quantity measuring the decoherence. Recurrences in the purity and in the off-diagonal matrix elements are observed, as well as the collapse of these matrix elements to the diagonal, providing evidence for the retention of quantum coherence for time scales longer than that indicated by the purity. The results are used to analyze the utility of the Caldeira-Leggett and Redfield models of decoherence and to assess the dependence of dephasing rates on the degree of structure in phase space. In several cases we find that the dephasing dynamics can be described as an initial Zeno-effect regime, followed by a Caldeira-Leggett region, followed by recurrences.
Vibrational decoherence of a "breathing sphere" oscillator in a thermal Lennard-Jones bath is examined using a classical analog approach. The equivalence between this approach and the linearized semiclassical initial value representation (IVR) is established and the method is exploited to produce a useful computational strategy that can efficiently evaluate the time dependence of the decoherence in these systems. A comparison between Harmonic and Morse "breathing sphere" models is presented and the rate of decoherence is found to depend on the choice of model, the initial state of the oscillator, the initial conditions of the bath (temperature, density), and the choice of quantity measuring the decoherence rate. The results are used to examine the utility of the Caldeira-Leggett model in this realistic system.
The forward–backward (FB) version of the semiclassical (SC) initial value representation (IVR) is used to study quantum coherence effects in the time-dependent probability distribution of an anharmonic vibrational coordinate and its quenching when coupled to a thermal bath. It is shown that the FB-IVR accurately reproduces the detailed quantum coherent structure in the weak coupling regime, and also describes how this coherence is quenched with an increase of the system–bath coupling and/or the bath temperature. Comparisons are made with other approximations and the physical implications are discussed.
We calculate the reduced density matrix for a system of coupled harmonic oscillators in a bosonic heat bath using the Born-Markov approximation and show that the expectation values of position and momentum evolve like classical quantities. We consider the cases where every oscillator is coupled to its own reservoir and where all oscillators are coupled to the same heat bath, pointing out the differences between these two models. In particular, for systems coupled to a common reservoir, we present an uncommon dissipation mechanism, which disappears, when the dynamics of the system are gouverned by the low frequency modes of the environment (Caldeira-Leggett limit). We also address the interesting phenomenon of reservoir-induced interactions.
The dynamics of a quantum anharmonic oscillator whose position is monitored by a Bose-Einstein condensate trapped in a symmetric double well potential is studied. The (nonexponential) decoherence induced on the oscillator by the measuring device is analyzed. A detailed quasiclassical and quantum analysis is presented. In the first case, for an arbitrary initial coherent state, two different decoherence regimes are observed: an initial Gaussian decay followed by a power law decay for longer times. The characteristic time scales of both regimes are reported. Analytical approximated expressions are obtained in the full quantum case where algebraic time decay of decoherence is observed.
We examine the effect of multilevels on decoherence and dephasing properties of a quantum system consisting of a non-ideal two level subspace, identified as the qubit and a finite set of higher energy levels above this qubit subspace. The whole system is under interaction with an environmental bath through a Caldeira-Leggett type coupling. The model interaction we use can generate nonnegligible couplings between the qubit states and the higher levels upto N∼10N\sim 10N∼10. In contrast to the pure two-level system, in a multilevel system the quantum information may leak out of the qubit subspace through nonresonant as well as resonant excitations induced by the environment. The decoherence properties of the qubit subspace is examined numerically using the master equation formalism of the system's reduced density matrix. We numerically examine the relaxation and dephasing times as the environmental frequency spectrum, the environmental temperature, and the multilevel system parameters are varied. We observe the influence of all energy scales in the noise spectrum on the short time dynamics implying the dominance of nonresonant transitions at short times. The relaxation and dephasing times calculated, strongly depend on NNN for 4<N<104< N<104<N<10 and saturate for $10
We study the effects of dissipation and decoherence induced on a harmonic oscillator by the coupling to a chaotic system with two degrees of freedom. Using the Feynman-Vernon approach and treating the chaotic system semiclassically, we show that the effects of the low-dimensional chaotic environment are in many ways similar to those produced by thermal baths. The classical correlation and response functions play important roles in both classical and quantum formulations. Our results are qualitatively similar to the high-temperature regime of the Caldeira-Leggett model.