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Laser & Photonics Review

Electromagnetically induced transparency‐based slow and stored light in warm atoms

Irina V. Novikova, R. L. Walsworth, Yanhong Xiao

Published Sep 20, 2011• 335 citations
Publisher

Abstract

Abstract This paper reviews recent efforts to realize a high‐efficiency memory for optical pulses using slow and stored light based on electromagnetically induced transparency (EIT) in ensembles of warm atoms in vapor cells. After a brief summary of basic continuous‐wave and dynamic EIT properties, studies using weak classical signal pulses in optically dense coherent media are discussed, including optimization strategies for stored light efficiency and pulse‐shape control, and modification of EIT and slow/stored light spectral properties due to atomic motion. Quantum memory demonstrations using both single photons and pulses of squeezed light are then reviewed. Finally a brief comparison with other approaches is presented.

DOI
10.1002/lpor.201100021

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Abstract This paper reviews recent efforts to realize a high‐efficiency memory for optical pulses using slow and stored light based on electromagnetically induced transparency (EIT) in ensembles of warm atoms in vapor cells. After a brief summary of basic continuous‐wave and dynamic EIT properties, studies using weak classical signal pulses in optically dense coherent media are discussed, including optimization strategies for stored light efficiency and pulse‐shape control, and modification of EIT and slow/stored light spectral properties due to atomic motion. Quantum memory demonstrations using both single photons and pulses of squeezed light are then reviewed. Finally a brief comparison with other approaches is presented.
The recent prospect of efficient, reliable, and secure quantum communication relies on the ability to coherently and reversibly map nonclassical states of light onto long-lived atomic states. A promising technique that accomplishes this employs Electromagnetically Induced Transparency (EIT), in which a strong classical control field modifies the optical properties of a weak signal field in such a way that a previously opaque medium becomes transparent to the signal field. The accompanying steep dispersion in the index of refraction allows for pulses of light to be decelerated, then stored as an atomic excitation, and later retrieved as a photonic mode. This dissertation presents the results of investigations into methods for optimizing the memory efficiency of this process in an ensemble of hot Rb atoms. We have experimentally demonstrated the effectiveness of two protocols for yielding the best memory efficiency possible at a given atomic density. Improving memory efficiency requires operation at higher optical depths, where undesired effects such as four-wave mixing (FWM) become enhanced and can spontaneously produce a new optical mode (Stokes field). We present the results of experimental and theoretical investigations of the FWM-EIT interaction under continuous-wave (cw), slow light, and stored light conditions. In particular, we provide evidence that indicates that while a Stokes field is generated upon retrieval of the signal field, any information originally encoded in a seeded Stokes field is not independently preserved during the storage process. We present a simple model that describes the propagation dynamics and provides an intuitive description of the EIT-FWM process.
Quantum memories play a pivotal role in establishing long-distance communication by entanglement swapping operations within quantum repeater nodes. Constructing such a quantum memory involves Electromagnetically Induced Transparency (EIT) within atomic vapors at room temperatures to store highly attenuated coherent light pulses down to the level of single photons. The photons may be generated from quantum nodes containing stationary quantum systems, such as atoms or semiconductor quantum dots (QDs). QDs serve as a potent source of quantum light, furnishing bright, precisely timed single photons of exceptional purity. While previous endeavors have demonstrated the integration of QDs with atomic vapors through techniques like “slow light,” the development of a dedicated quantum memory for QDs remains unmatched. In our study, we introduce an EIT quantum memory hosted within warm cesium vapor. Our approach exhibits a good efficiency in storing faint coherent light pulses at the single photon level. Moreover, the measured bandwidth of around 200 MHz approaches the Fourier-limited emission characteristics of QDs. We present initial efforts to match the emission from QDs with our quantum memory and discuss application scenarios of room temperature EIT quantum memories.
Quantum memory (QM) enables quantum state mapping between flying and stationary quantum states and is the building block of quantum information science, which enables to achieve a plethora of quantum information protocols, such as quantum state transfer across remote quantum nodes, distributed quantum logic gate, and quantum precession measurement network. Great progresses of quantum memories have been achieved, and electromagnetically induced transparency (EIT) is one of the well-understood approaches of QM. Quantum states of light are the essential quantum resources for implementing quantum enhanced task, and thus it is a long-standing goal to store and release non-classical states of light. This paper presents an up-to-date review on recent developments in EIT-based QM: EIT quantum memories have been realized in warm atomic cell, cold atoms and solid system, respectively; and EIT mechanism has been applied to store and release single photon, squeezed state, entangled photon pairs and multipartite entangled states of optical modes.
We present undergraduate-friendly instructions on how to produce light pulses propagating through warm Rubidium vapor with speeds less than 400 m/s, i.e., nearly a million times slower than c. We elucidate the role played by electromagnetically induced transparency (EIT) in producing slow light pulses and discuss how to achieve the required experimental conditions. The optical setup is presented, and details provided for preparation of pump, probe, and reference pulses of the required size, frequency, intensity, temporal width, and polarization purity. EIT-based slow light pulses provide the most widely studied architecture for creating quantum memories. Therefore, the basic concepts presented here are useful for physics and engineering majors who wish to get involved in the development of cutting-edge quantum technologies.
This thesis set out to investigate light storage based on dynamic electromagnetically induced transparency (EIT) in a room-temperature atomic ensemble of rubidium as a means to provide a quantum memory for single-photons created by a single rubidium atom coupled to a high-finesse optical resonator. Setting up the light storage medium presented a new addition to the research group's portfolio of experimental techniques and led to investigations of EIT, slow light and stored light in warm rubidium-87 vapour. Lambda level schemes connecting Zeeman or hyperfine substates on the D1 and D2 lines were addressed in rubidium vapour cells containing different buffer gases and different isotopic fractions of rubidium-87 and rubidium-85. Single beam spectroscopy with a weak probe was used to characterise the vapour cells. A numerical method to fit the D line spectrum to a theoretical model to include isotopic fractions and collisional broadening of a buffer gas has been implemented. Temperature and isotopic fractions could be reliably extracted from the fit parameters. For an offset-stabilisation of two lasers to address a lambda level scheme connecting the two different hyperfine groundstates in rubidium a phase locked loop including a frequency divider has been designed and implemented. Light storage and retrieval has been demonstrated using a Zeeman scheme on the D1 line. Two microsecond long classical light pulses containing one million photons on average were stored and retrieved with an efficiency of 15% after a delay of one microsecond. Several methods of attenuating the strong co-propagating control laser beam to allow for lowering the signal pulse intensity in future experiments are discussed.
Quantum memories can substantially increase the efficiency of long-distance communications by synchronizing entanglement swapping operations in quantum repeater nodes. To build a quantum memory, electromagnetically induced transparency (EIT) in atomic vapors can be exploited to coherently store light pulses even at room temperatures. As a quantum source of light, semiconductor quantum dots (QD) offer bright on-demand single photons with high purity.4 Interfacing QDs with atomic vapors has been shown by “slow light” but a quantum memory for QDs is yet to be demonstrated. In this work, we develop an EIT quantum memory hosted in warm cesium vapor. Storage of faint coherent light pulses on the single photon level shows high storage efficiency. A measured bandwidth in the order of 200 MHz makes the memory compatible with the Fourier-limited emission of QDs embedded in micropillar cavities. We show the first attempts to interface the emission from a QD-micropillar with our quantum memory by finetuning the emission wavelength of the emitters to one of the hyperfine transitions in Cs, where the EIT memory takes place. This work sets the base for a hybrid quantum memory based on atomic ensembles for an on-demand semiconductor single-photon source.