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Physical Review A

Effect of antiresonant atom-field interactions on phase transitions in the Dicke model

G. Comer Duncan

Published Jan 1, 1974• 47 citations
Publisher

Abstract

The effect of the antiresonant atom-field interactions on the phase-transition property of the Dicke model is studied. A phase transition is shown to exist when the following inequality is satisfied between the coupling constant $\ensuremath{\lambda}$ and the ratio of the atomic transition frequency to the field frequency $\ensuremath{\epsilon}$: ${\ensuremath{\lambda}}^{2}>\frac{\ensuremath{\epsilon}}{4}$. Relative to the Dicke-model result the necessary value of ${\ensuremath{\lambda}}^{2}$ is thus smaller by a factor of \textonequarter{}. In addition it is established that the critical temperature is higher than in the Dicke model. A further significant difference between the two models is reflected in the properties of the "photon statistics." In the present model an additional polynomial temperature dependence in the powers of the average number of photons per atom is found. It is concluded that the effect of the antiresonant terms is not negligible concerning the thermodynamic properties of the system, in contrast to the evidence for many time-dependent properties studied previously.

DOI
10.1103/physreva.9.418

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The effect of the antiresonant atom-field interactions on the phase-transition property of the Dicke model is studied. A phase transition is shown to exist when the following inequality is satisfied between the coupling constant \ensuremathλ\ensuremath{\lambda}\ensuremathλ and the ratio of the atomic transition frequency to the field frequency \ensuremathϵ\ensuremath{\epsilon}\ensuremathϵ: \ensuremathλ2>\ensuremathϵ4{\ensuremath{\lambda}}^{2}>\frac{\ensuremath{\epsilon}}{4}\ensuremathλ2>4\ensuremathϵ​. Relative to the Dicke-model result the necessary value of \ensuremathλ2{\ensuremath{\lambda}}^{2}\ensuremathλ2 is thus smaller by a factor of \textonequarter{}. In addition it is established that the critical temperature is higher than in the Dicke model. A further significant difference between the two models is reflected in the properties of the "photon statistics." In the present model an additional polynomial temperature dependence in the powers of the average number of photons per atom is found. It is concluded that the effect of the antiresonant terms is not negligible concerning the thermodynamic properties of the system, in contrast to the evidence for many time-dependent properties studied previously.
The authors consider a system comprised of a collection of identical two-level atoms interacting with the electromagnetic field in the dipole approximation and with an externally applied steady-state coherent driving field. The atoms are considered to interact with each other only via the electromagnetic field and are assumed to be contained within a volume much smaller than a resonance wavelength. The system is treated as a quantum-statistical ensemble in the rotating frame, rotating at the carrier frequency of the externally applied coherent field. The Hamiltonian in this frame is explicitly time independent and the exact analog of a spin temperature is defined. The thermodynamic-Green's-function method is used to determine the thermodynamic equilibrium properties of the system in the rotating frame. This results in a nonlinear relation between the applied field and the field in the volume containing the atoms. The expression is a nonlinear function of the effective or "spin" temperature as well, and has the form of a first-order phase transition with the macroscopic atomic polarization as order parameter. In the low-"spin"-temperature limit, and for perfect tuning, the expression reduces to the exact form of the nonlinear relation for optical bistability derived by Bonifacio and Lugiato and relating the incident and transmitted fields for atoms in a ring cavity in the mean-field approximation. The results contain absorptive as well as dispersive contributions. These results predict essentially different behavior as a function of off tuning compared with behavior predicted by others using statistical steady-state models far from thermodynamic equilibrium. In the limit of zero value for the applied field amplitude, the results reduce to the conditions for the well-known second-order superradiant" phase transition. The condition for the existence of the second-order phase transition is shown to depend on the cavity tuning and the photon escape rate. The authors also show why, in light of the experiments in optical bistability, this second-order phase is difficult to observe.
The Dicke model generalized to the case where the dependence of the coupling constant on individual atoms is taken into account is investigated. It is shown that the generalized Dicke model exhibits a quantum phase transition from the normal phase to the superradiant phase in the thermodynamic limit, as well as the standard Dicke model. The mean photon number, the atomic inversion, the lowest excitation energy, and the entanglement entropy between the field and the atoms are evaluated analytically or numerically, and the critical behavior is examined. As a result, it turns out that the critical behavior in the generalized model is essentially the same as that in the standard model. This implies universality in the Dicke model.
The Dicke Hamiltonian describes the simplest quantum system with atoms interacting with photons: N two level atoms inside a perfectly reflecting cavity which allows only one electromagnetic mode. It has also been successfully employed to describe superconducting circuits which behave as artificial atoms coupled to a resonator. The system exhibits a transition to a superradiant phase at zero temperature. When the interaction strength reaches its critical value, both the number of photons and of atoms in excited states in the cavity, together with their fluctuations, exhibit a sudden increase from zero. Employing symmetry-adapted coherent states it is shown that these properties scale with the number of atoms, that their reported divergences at the critical point represent the limit when this number goes to infinity, and that in this limit they remain divergent in the superradiant phase. Analytical expressions are presented for all observables of interest, for any number of atoms. Comparisons with exact numerical solutions strongly support the results.
In this doctoral thesis, the thermodynamic phases und phase transitions of a generalised Dicke model are studied and characterised. Both, finite and vanishing temperatures are considered. The Dicke model of quantum optics describes collective phenomena which occur when light interacts with a many-atom system. In the thermodynamic limit, a so-called Hepp–Lieb superradiant phase transition sets in. A superradiant phase develops for low temperatures or strong coupling between light and atoms, which is characterised by a macroscopic excitation of the light field and a spontaneous, collective polarisation of the atoms. This thesis discusses a generalised version of the Dicke model, which is described by a quantum mechanical system consisting of three-level atoms in Lambda-configuration and two modes of a resonator. By means of the Holstein–Primakoff transformation, the Hamiltonian of this system is written in terms of four interacting, non-linear oscillators, which can be linearised in the thermodynamic limit, yielding the ground-state energy as well as the low-energy excitations. The phase diagram consisting of two superradiant phases separated by continuous and first-order phase transitions is derived. In order to clarify the question whether or not the superradiant phase transition of this generalised Dicke model can be observed experimentally for real atoms, the significance of the diamagnetic term is discussed. In contrast to the original Dicke model, superradiant phase transitions are possible in principle. This is due to the first-order phase transitions. In addition, a no-go theorem for continuous superradiant phase transitions is presented. The argument is based on the Thomas–Reiche–Kuhn sum rule. Last, we study the superradiant phase transition of the generalised Dicke model at finite temperatures. Therefore, the partition sum is computed and analysed in the thermodynamic limit using Laplace’s method. At finite temperatures, the properties of the phase diagram and phases remain. However, here all phase transitions are of first order.
The Dicke model describing an ensemble of two-state atoms interacting with a single quantized mode of the electromagnetic field (with omission of the ${\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{A}}^{2}$ term) exhibits a zero-temperature phase transition at a critical value of the dipole coupling strength. We propose a scheme based on multilevel atoms and cavity-mediated Raman transitions to realize an effective Dicke model operating in the phase transition regime. Optical light from the cavity carries signatures of the critical behavior, which is analyzed for the thermodynamic limit where the number of atoms is very large.
The Dicke Hamiltonian describes the simplest quantum system with atoms interacting with photons: NNN two-level atoms inside a perfectly reflecting cavity, which allows only one electromagnetic mode. It has also been successfully employed to describe superconducting circuits that behave as artificial atoms coupled to a resonator. The system exhibits a transition to a superradiant phase at zero temperature. When the interaction strength reaches its critical value, both the number of photons and atoms in excited states in the cavity, together with their fluctuations, exhibit a sudden increase from zero. By employing symmetry-adapted coherent states, it is shown that these properties scale with the number of atoms, their reported divergences at the critical point represent the limit when this number goes to infinity, and, in this limit, they remain divergent in the superradiant phase. Analytical expressions are presented for all observables of interest, for any number of atoms. Comparisons with exact numerical solutions strongly support the results.