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Physical review. B, Condensed matter

Excitation spectrum of the ferromagnetic Ising-Heisenberg chain at zero field

T. Schneider, E. Stoll

Published Apr 1, 1982• 26 citations
Publisher

Abstract

The excitation spectrum of the ferromagnetic $s=\frac{1}{2}$ Ising-Heisenberg chain as probed by dynamic form factors is studied. Exact results are presented for zero temperature, and the modifications introduced by thermally induced transitions are elucidated by finite-chain calculations. A particularly interesting result is the occurrence of a thermally induced resonance around zero frequency for an Ising-like model. Its origin is traced back to transitions involving magnon bound states. The resonance structure of the dynamic form factors associated with a Heisenberg-like system turns out to be less spectacular, because the contributions of different induced transitions nearly overlap on the frequency scale; so that rather broad resonance structures result. Our findings have an important bearing on related models with $s>\frac{1}{2}$, such as CsNi${\mathrm{F}}_{3}$, and on the soliton aspect of the classically treated systems.

DOI
10.1103/physrevb.25.4721

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The excitation spectrum of the ferromagnetic s=12s=\frac{1}{2}s=21​ Ising-Heisenberg chain as probed by dynamic form factors is studied. Exact results are presented for zero temperature, and the modifications introduced by thermally induced transitions are elucidated by finite-chain calculations. A particularly interesting result is the occurrence of a thermally induced resonance around zero frequency for an Ising-like model. Its origin is traced back to transitions involving magnon bound states. The resonance structure of the dynamic form factors associated with a Heisenberg-like system turns out to be less spectacular, because the contributions of different induced transitions nearly overlap on the frequency scale; so that rather broad resonance structures result. Our findings have an important bearing on related models with s>12s>\frac{1}{2}s>21​, such as CsNiF3{\mathrm{F}}_{3}F3​, and on the soliton aspect of the classically treated systems.
Results are presented and interpreted for the zero- and finite-temperature excitation spectrum of ferromagnetic Ising-Heisenberg chains, as probed by dynamic form factors. Finite-chain calculations demonstrate the occurrence of a thermally induced resonance centered around zero frequency, and a broadening of the magnon and two-magnon bound-state resonances at low TTT. The occurrence of bound states in the associated transitions demonstrates the failure of finite-order magnon perturbation theory.
We present analytic weak-coupling and numerical finite-chain results for the dynamic form factor associated with the out-of-plane fluctuations at zero temperature and zero field. The dynamic form factor associated with the in-plane fluctuations is treated numerically only. In the ferromagnetic regime, the dominant features are traced back to particle-hole pair continua and the associated bound states. With the approach toward the isotropic ferromagnet, the resonance associated with the bound state of the particle-hole pairs gradually exhausts the spectrum, corresponding in this limit to the magnon peak. In the antiferromagnetic regime, the spectrum is dominated by the particle-hole pair continuum. The analytic results for the dynamic form factor associated with the out-of-plane fluctuations reproduce and extend the well-known properties of the continuum model to leading order in the coupling constant. As expected from the relation between the six-vertex model and the xxz\mathrm{xxz}xxz chain, these properties include singular behavior of dynamic form factors depending continuously on the coupling constant.
We present results for the dynamic structure factor of the S=1∕2S=1∕2S=1∕2 bond alternating Heisenberg chain over a large range of frequencies and temperatures. Data are obtained from a numerical evaluation of thermal averages based on the calculation of all eigenvalues and eigenfunctions for chains of up to 20 spins. Interpretation is guided by the exact temperature dependence in the noninteracting dimer limit which remains qualitatively valid up to an interdimer exchange $\ensuremath{\lambda}\ensuremath{\approx}0.5$. The temperature induced central peak around zero frequency is clearly identified and aspects of the crossover to spin diffusion in its variation from low to high temperatures are discussed. The one-magnon peak acquires an asymmetric shape with increasing temperature. The two-magnon peak is dominated by the S=1S=1S=1 bound state which remains well defined up to temperatures of the order of JJJ. The variation with temperature and wave vector of the integrated intensity for one-magnon and two-magnon scattering and of the central peak are discussed.
Motivated by the lack of direct evidence with inelastic neutron scattering of the well documented bound state of Heisenberg ferromagnets, we use the time-dependent thermal density matrix renormalization group algorithm to study the temperature dependence of the dynamical spin structure factor of Heisenberg ferromagnetic spin chains. For spin 1/2, we show that the bound state appears as a well defined excitation with significant spectral weight in the temperature range $J/12\ensuremath{\lesssim}T\ensuremath{\lesssim}J/3$, pointing to the possibility of detecting it with inelastic neutron scattering near $k=\ensuremath{\pi}$ provided the temperature is neither too low nor too high---at low temperature, the spectral weight only grows as T3/2{T}^{3/2}T3/2 and, at high temperature, the bound state peak merges with the two-magnon continuum. For spin 1, the situation is more subtle because the bound state with two neighboring spin flips competes with an antibound state with two spin flips on the same site. As a consequence, the relative spectral weight of the bound state is smaller than for spin 1/2 and a weak resonance due to the antibound state appears in the continuum. A clearer signature of the bound state (antibound state) can be obtained if a negative (positive) biquadratic interaction is present.