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Journal of Magnetism and Magnetic Materials

Magnetic excitations and critical dynamics in RbMnF3: simulation versus theory and experiment

David Paul Landau, Shan-Ho Tsai, Alex Bunker

Published May 1, 2001• 3 citations
Publisher
DOI
10.1016/s0304-8853(00)00919-7

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Spin-dynamics techniques have been used to perform large-scale simulations of the dynamic behavior of the classical Heisenberg antiferromagnet in simple cubic lattices with linear sizes $L<~60.$ This system is widely recognized as an appropriate model for the magnetic properties of ${\mathrm{RbMnF}}_{3}.$ Time evolutions of spin configurations were determined numerically from coupled equations of motion for individual spins using an algorithm implemented by Krech et al., which is based on fourth-order Suzuki-Trotter decompositions of exponential operators. The dynamic structure factor was calculated from the space- and time-displaced spin-spin correlation function. The crossover from hydrodynamic to critical behavior of the dispersion curve and spin-wave half-width was studied as the temperature was increased towards the critical temperature. The dynamic critical exponent was estimated to be $z=(1.43\ifmmode\pm\else\textpm\fi{}0.03),$ which is slightly lower than the dynamic scaling prediction, but in good agreement with a recent experimental value. Direct, quantitative comparisons of both the dispersion curve and the line shapes obtained from our simulations with very recent experimental results for ${\mathrm{RbMnF}}_{3}$ are presented.

arXiv:cond-mat/9910429•Physical review. B, Condensed matter•Jan 1, 2000•28 citations
Spin-dynamics simulations have been used to investigate the dynamic behavior of RbMnF_3, treating it as a classical Heisenberg antiferromagnet on a simple cubic lattice. Time-evolutions of spin configurations were determined numerically from coupled equations of motion for individual spins using a new algorithm which is based on Suzuki-Trotter decompositions of exponential operators. The dynamic structure factor was calculated from the space- and time-displaced spin-spin correlation function. The crossover from hydrodynamic to critical behavior of the dispersion curve and spin-wave half-width was studied as the temperature was increased towards the critical value. The dynamic critical exponent was estimated to be z=(1.43\pm 0.03), which is slightly lower than the dynamic scaling prediction, but in good agreement with a recent experimental value. Comparisons are made of both the dispersion curve and the lineshapes obtained from our simulations with very recent experimental results for RbMnF_3 are presented.
Monte Carlo and spin dynamics simulations have been used to study the dynamic critical behavior of RbMnF3,{\mathrm{RbMnF}}_{3},RbMnF3​, treated as a classical Heisenberg antiferromagnet on a simple cubic lattice. In an attempt to understand the difference in the value of the dynamic critical exponent z between experiment and theory, we have used larger lattice sizes than in our previous simulations to better probe the asymptotic critical region in momentum. We estimate $z=1.49\ifmmode\pm\else\textpm\fi{}0.03,$ in good agreement with the renormalization-group theory and dynamic scaling predictions. In addition, the central peak in the dynamic structure factor at Tc,{T}_{c},Tc​, seen in experiments and previous simulations, but absent in the renormalization-group and mode-coupling theories, is shown to be solely in the longitudinal component.
Spin-dynamics techniques have been used to perform large-scale simulations of the dynamic behavior of the classical Heisenberg antiferromagnet in simple cubic lattices with linear sizes L< 60.L<~60.L< 60. This system is widely recognized as an appropriate model for the magnetic properties of RbMnF3.{\mathrm{RbMnF}}_{3}.RbMnF3​. Time evolutions of spin configurations were determined numerically from coupled equations of motion for individual spins using an algorithm implemented by Krech et al., which is based on fourth-order Suzuki-Trotter decompositions of exponential operators. The dynamic structure factor was calculated from the space- and time-displaced spin-spin correlation function. The crossover from hydrodynamic to critical behavior of the dispersion curve and spin-wave half-width was studied as the temperature was increased towards the critical temperature. The dynamic critical exponent was estimated to be $z=(1.43\ifmmode\pm\else\textpm\fi{}0.03),$ which is slightly lower than the dynamic scaling prediction, but in good agreement with a recent experimental value. Direct, quantitative comparisons of both the dispersion curve and the line shapes obtained from our simulations with very recent experimental results for RbMnF3{\mathrm{RbMnF}}_{3}RbMnF3​ are presented.