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Physical Review A

Effects of nonlinearity on the optical diffraction of Bose-Einstein condensates: Direct integration of optically coupled multicomponent Gross-Pitaevskii equation

Taro Ando, Yoshiyuki Ohtaké, Junichi Kondo, Katsuhiro Nakamura

Published Feb 28, 2011• 1 citation
Publisher

Abstract

We investigate in detail the effects of nonlinearity on optical diffraction of Bose-Einstein condensates (BECs). By directly integrating the optically coupled two-component Gross-Pitaevskii equation in real space-time, comprehensive analyses of BEC optical diffraction phenomena are done under various conditions of light-pulse irradiation, total number of BEC atoms, etc., without using the adiabatic elimination approximation for an atomic excited state. Calculation results for the optical diffraction of ${}^{87}\text{Rb}$ BECs revealed that (1) the effect of nonlinearity on the atomic states causes the ``nonkinetic'' nonlinear effect in the Raman-Nath regime of diffraction, while the dynamics of BEC atoms due to the nonlinearity-induced repulsive forces works dominantly to produce the ``kinetic'' nonlinear effect in the Bragg regime of diffraction; (2) nonlinearity reduces the amplitude and frequency of the two-photon Rabi oscillation between BEC stationary and moving states, suggesting limitations in implementing the BEC Mach-Zehnder interferometer; and (3) the observed nonlinear effects are free from kinetic effects of the atomic excited state and not responsible for the optical transition process.

DOI
10.1103/physreva.83.023619

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We investigate in detail the effects of nonlinearity on optical diffraction of Bose-Einstein condensates (BECs). By directly integrating the optically coupled two-component Gross-Pitaevskii equation in real space-time, comprehensive analyses of BEC optical diffraction phenomena are done under various conditions of light-pulse irradiation, total number of BEC atoms, etc., without using the adiabatic elimination approximation for an atomic excited state. Calculation results for the optical diffraction of 87Rb{}^{87}\text{Rb}87Rb BECs revealed that (1) the effect of nonlinearity on the atomic states causes the nonkinetic'' nonlinear effect in the Raman-Nath regime of diffraction, while the dynamics of BEC atoms due to the nonlinearity-induced repulsive forces works dominantly to produce the kinetic'' nonlinear effect in the Bragg regime of diffraction; (2) nonlinearity reduces the amplitude and frequency of the two-photon Rabi oscillation between BEC stationary and moving states, suggesting limitations in implementing the BEC Mach-Zehnder interferometer; and (3) the observed nonlinear effects are free from kinetic effects of the atomic excited state and not responsible for the optical transition process.
The advent of the laser as an intense, coherent light source gave birth to nonlinear optics, which now plays an important role in many areas of science and technology. One of the first applications of nonlinear optics was the production of coherent light of a new frequency by multi-wave mixing of several optical fields in a nonlinear medium. Until the experimental realization of Bose-Einstein Condensation (BEC) there had been no intense coherent source of matter-waves analogous to the optical laser. FEC has already been exploited to produce a matter-wave `laser' leading to the threshold of a new field of physics: nonlinear atom optics. Recently the first experiment in nonlinear atom optics was reported: the observation of coherent four wave mixing in which three sodium matter waves mix to produce a fourth. The experiment utilized light pulses to create two high-momentum wavepackets via Bragg diffraction from a stationary Bose- Einstein condensate. The high-momentum components and the remaining zero momentum condensate component interact to form a new momentum component due to the nonlinear self- interaction of the bosonic atoms. We develop a quantum mechanical description, based on the slowly-varying-envelope approximation to the time-dependent nonlinear Schrodinger equation (also called the Gross-Pitaevskii equation), to describe four-wave mixing in Bose-Einstein condensates and apply this description to understand the experimental observations and to make new predictions. We examine the role of phase-modulation, momentum and energy conservation (i.e., phase-matching), and particle number conservation in four-wave mixing of matter waves.
Rb Bose-Einstein condensate from a one-dimensional optical lattice. We use a range of lattice periods and timescales, including those beyond the Raman-Nath limit. We compare the results to numerical solutions of the Gross-Pitaevskii equation and classical calculations, with quantitative and qualitative agreement, respectively. The classical calculations predict that the envelope of the time-evolving diffraction pattern is shaped by caustics: singularities in the phase-space density of classical trajectories. This behavior becomes increasingly clear as the lattice period grows.
Nonlinear excitations in two-component Bose-Einstein condensates (BECs) described by two coupled Gross-Pitaevskii equations are investigated analytically and numerically. The beating phenomenon, the higher-harmonic generation, and the mixing of the excited modes are revealed by both variational approximation and numerical method. The strong excitations induced by the parametric resonance are also studied by time-periodic modulation for the intercomponent interaction. The resonance conditions in terms of the modulation frequency and the strength of intercomponent interaction are obtained analytically, which are confirmed by numerical method. Direct numerical simulations show that, when the resonance takes place, periodic phase separation and multisoliton configurations (including soliton trains, soliton pairs, and multidomain walls) can be excited. In particular, we demonstrate a method for formation of multisoliton configurations through parametric resonance in two-component BECs.
We study the dynamics of the atomic and molecular Bose-Einstein condensates (BECs) of 87Rb^{87}\text{R}\text{b}87Rb in a spherically symmetric trap coupled by stimulated Raman photoassociation process. Considering the higher order nonlinearity in the atom-atom interaction we analyze the dynamics of the system using coupled modified Gross-Pitaevskii (MGP) equations and compare it with mean-field coupled Gross-Pitaevskii (GP) dynamics. Considerable differences in the dynamics are obtained in these two approaches at large scattering length, i.e., for large values of peak-gas parameter ${x}_{pk}\ensuremath{\ge}{10}^{\ensuremath{-}3}$. We show how the dynamics of the coupled system is affected when the atom-molecule and molecule-molecule interactions are considered together with the atom-atom interaction and also when the strengths of these three interactions are increased. The effect of detuning on the efficiency of conversion of atomic fractions into molecules is demonstrated and the feasibility of maximum molecular BEC formation by varying the Raman detuning parameter at different values of time is explored. Thus by varying the Raman detuning and the scattering length for atom-atom interaction one can control the dynamics of the coupled atomic-molecular BEC system. We have also solved coupled Gross-Pitaevskii equations for atomic to molecular condensate formation through magnetic Feshbach resonance in a BEC of 85Rb^{85}\text{R}\text{b}85Rb. We found similar features for oscillations between atomic and molecular condensates noted in previous theoretical study and obtained fairly good agreement with the evolution of total atomic condensate observed experimentally.
We apply the concepts of nonlinear guided-wave optics to a Bose-Einstein condensate (BEC) trapped in an external potential. As an example, we consider a parabolic double-well potential and derive coupled-mode equations for the complex amplitudes of the BEC macroscopic collective modes. Our equations describe different regimes of the condensate dynamics, including the nonlinear Josephson effect for any separation between the wells. We demonstrate macroscopic self-trapping for both repulsive and attractive interactions, and confirm our results by direct numerical solution of the Gross-Pitaevskii-equation.
Bose–Einstein Condensation (BEC) of atomic gases has attracted a renewed theoretical and experimental interest in quantum many-body systems at extremely low temperatures (Pethick & Smith; 2002). This excitement stems from two favorable features: (1) by applying magnetic fields and lasers, most of the system parameters, such as the shape, dimensionality, internal states of the condensates, and even the strength of the interatomic interactions, are controllable; (2) due to the diluteness, the mean-field theory explains experiments quite well. In particular, the Gross–Pitaevskii (GP) equation demonstrates its validity as a basic equation for the condensate dynamics. The GP equation is the counterpart of the nonlinear Schrodinger (NLS) equation in nonlinear optics. Thus, a study based on nonlinear analysis is possible and important. In nonlinear physics, a soliton is remarkable object not only for the fact that exact solutions can be obtained but also for its usefulness as a communications tool due to its robustness. In general, solitons are formed under the balance between nonlinearity and dispersion. For atomic condensates, the former is attributed to the interatomic interactions, while the latter comes from the kinetic energy. Either dark or bright solitons are allowable depending on the positive or negative sign of the interatomic coupling constants g, respectively, and indeed have been observed in a quasione-dimensional (q1D) optically constructed waveguide (Strecker et al.; 2002) (Khaykovich et al.; 2002). Such matter-wave solitons are expected in atom optics for applications in atom laser, atom interferometry, and coherent atom transport (Meystre; 2002). In this chapter, we extend the analysis of the matter-wave solitons to a multicomponent case by considering the so-called spinor condensate (Stenger et al.; 1998) whose spin degrees of freedom are liberated under optical traps. Based on theoretical and experimental results, we introduce a new integrable model which describes the dynamical properties of the matter-wave soliton of spinor condensates (Ieda et al.; 2004a). We employ the inverse scattering method to solve this model exactly. As a result, we predict the occurrence of undiscovered physical phenomena such as macroscopic spin precession and spin switching. The chapter is organized as follows. In Sec. 2, the mean field theory of condensate is briefly reviewed. Section 3 introduces an effective interatomic coupling in a q1D condensate. Using these results, we consider a spinor condensate in q1D regime in Sec. 4. Then, in Sec. 5, we