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Physical Review A

Optical cavity quantum electrodynamics with dark-state polaritons

Guang Lin, Jiangbin Gong, Jie Yang, Yihong Qi, Xiu‐Min Lin, Yueping Niu, Shuang Gong

Published Apr 11, 2014• 13 citations
Publisher

Abstract

We present a theoretical scheme to study optical cavity quantum electrodynamics using dark-state polaritons. Exploiting the highly tunable lifetimes of the photons in the form of cavity dark-state polaritons, we push the strong coupling of single optical photons to an effective two-level emitter in a Rydberg-blockade atomic ensemble to an unprecedented regime. The resulting Jaynes--Cummings model with extremely strong coupling is of fundamental interest. We discuss applications in controlled quantum Rabi oscillation, nonlinear spectroscopy of the Jaynes-Cummings ladder, as well as the generation of nonclassical states, all based on light-matter interactions in the optical domain.

DOI
10.1103/physreva.89.043815

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Scientific Reports•Mar 3, 2016•3 citations
We present a theoretical scheme to study optical cavity quantum electrodynamics using dark-state polaritons. Exploiting the highly tunable lifetimes of the photons in the form of cavity dark-state polaritons, we push the strong coupling of single optical photons to an effective two-level emitter in a Rydberg-blockade atomic ensemble to an unprecedented regime. The resulting Jaynes--Cummings model with extremely strong coupling is of fundamental interest. We discuss applications in controlled quantum Rabi oscillation, nonlinear spectroscopy of the Jaynes-Cummings ladder, as well as the generation of nonclassical states, all based on light-matter interactions in the optical domain.
The realization of a Jaynes-Cummings model in the optical domain is proposed for an atomic ensemble. The scheme exploits the collective coupling of the atoms to a quantized cavity mode and the nonlinearity introduced by coupling to high-lying Rydberg states. A two-photon transition resonantly couples the single-atom ground state $|g\ensuremath{\rangle}$ to a Rydberg state $|e\ensuremath{\rangle}$ via a nonresonant intermediate state $|i\ensuremath{\rangle}$, but due to the interaction between Rydberg atoms only a single atom can be resonantly excited in the ensemble. This restricts the state space of the ensemble to the collective ground state $|G\ensuremath{\rangle}$ and the collectively excited state $|E\ensuremath{\rangle}$ with a single Rydberg excitation distributed evenly on all atoms. The collectively enhanced coupling of all atoms to the cavity field with coherent coupling strengths which are much larger than the decay rates in the system leads to the strong coupling regime of the resulting effective Jaynes-Cummings model. We use numerical simulations to show that the cavity transmission can be used to reveal detailed properties of the Jaynes-Cummings ladder of excited states and that the atomic nonlinearity gives rise to highly nontrivial photon emission from the cavity. Finally, we suggest that the absence of interactions between remote Rydberg atoms may, due to a combinatorial effect, induce a cavity-assisted excitation blockade whose range is larger than the typical Rydberg dipole-dipole interaction length.
The coherent light-matter interaction at the single-photon and electronic qubit level promises to be a remarkable potential for nonclassical information processing. Besides the efforts of improving the figure of merit of the cavities, here we demonstrate strong anharmonicity in the polariton dressed states via dark state resonances in a highly dissipative cavity. It is shown that the vacuum Rabi oscillation occurs for a single quantum emitter inside a cavity even with the bosonic decay-to-interaction rate ratio exceeding 102{10}^{2}102, when the photon field is coupled to an auxiliary high-QQQ cavity. Moreover, photon blockade is observable in such a highly dissipative cavity quantum electrodynamics system. This study provides a promising platform for overcoming decoherence and advancing the coherent manipulation of polariton qubits.
This thesis covers a theoretical analysis of non-interacting and interacting quasi\nparticles, called polaritons. Polaritons are composites, based on photonic and atomic\nexcitations in a tunable and controlled manner. Dark-state polaritons, as a subclass\nof polaritons, are very curious objects, as they can act as a quantum memory of\nphotons within an ensemble of alkali-metal atoms in -type conguration which\nadmit electromagnetically induced transparency (EIT). This thesis focus on the\nformation of dark-state polaritons in degenerate two-level systems, where two light\nelds, a quantum probe and a classical driving eld, couple the same transition\nbetween the ground state and excited state manifold. An algorithm is going to\nbe derived in order to determine the dispersion relation and inherent composition\nof the dark-state polaritons in the degenerate two-level system. The algorithm is\nbased on a microscopic equation of motion technique and provides an extension of\nthe non-degenerate case. Depending on the polarization of the light elds, it will be\nshown that either one or two dark-state polaritons can exist. Further, the calculated\ndark-state polaritons can be used in order to perform a frequency conversion and\neven a conversion of linear light polarization.\nIn the second part of the thesis, interacting polaritons in arrays of coupled QED\ncavities will be discussed. In rst place, the standard Jaynes-Cummings model is\ndiscussed in order to provide a better insight to polaritons in QED cavities. Then,\na modied Jaynes-Cummings model is introduced and derived in order to study\ndark-polaritons and their interaction. It will be shown that dark-polaritons directly\ndepend on the common single photon detuning of the two coupling elds, quantum\nprobe and classical driving eld. The interaction between dark-polaritons will be\ndiscussed where the emergence of dark-polariton bound pairs will be shown. By\ntuning the Stark-shift due to the classical control eld, the number and the composition\nof dark-polariton bound pairs can be controlled. It will be demonstrated\nthat there exists a dark-polariton bound pair which diers from the aforementioned\nones, because it represents a ground state of the system. Using that kind of a darkpolariton\nbound pair, storage and retrieval of a single photon can be performed,\neven though that the photons are in a two-photon bound state.\nIn the last part of the thesis, disorder between QED cavities will be introduced\nin a controlled manner through staggered inter-cavity photon hopping strengths J1\nand J2. Further, the appearance of a dark-polariton bound pair of a completely\ndierent type will be presented.
Light and matter can be unified under the strong coupling regime, creating superpositions of both, called dressed states or polaritons. After initially being demonstrated in bulk semiconductors and atomic systems ,strong coupling phenomena have been realized in solid state optical microcavities. They form an essential ingredient in the exciting physics spanning from many-body quantum coherence phenomena, like Bose-Einstein condensation and superfluidity, to cavity quantum electrodynamics (cQED). A widely used approach within cQED is the Jaynes-Cummings (JC) model that describes the interaction of a single fermionic two-level system with a single bosonic photon mode. For a photon number larger than one, known as quantum strong coupling (QSC), a significant anharmonicity is predicted for the ladder-like spectrum of dressed states. For optical transitions in semiconductor nanostructures, first signatures of the quantum strong coupling were recently published. In our latest report we applied advanced coherent nonlinear spectroscopy to explore a strongly coupled exciton-cavity system. Specifically, we measured and simulated its four-wave mixing (FWM) response, granting direct access to the first two rungs of the JC ladder. This paper summarizes the main results of Ref. 15 and adds FWM experiments obtained on a micropillar cavity in which a doublet of quantum dot (QD) excitons interacts with the cavity mode in the limit of weak to strong coupling.
The strong coupling of atoms and molecules to radiation field modes in optical cavities creates dressed matter/field states known as polaritons with controllable dynamical and energy transfer properties. We propose a multidimensional optical spectroscopy technique for monitoring polariton dynamics. The response of a two-level atom to the time-dependent coupling to a single-cavity mode is monitored through time-and-frequency-resolved single-photon coincidence measurements of spontaneous emission. Polariton population and coherence dynamics and its variation with cavity photon number and controlled by gating parameters are predicted by solving the Jaynes-Cummings model.
Manipulating the nature of photons emission is one of the basic tasks in quantum optics and photonics. The ever growing list of quantum applications requires a robust means of controlling the strongly coupled coherent interaction of photons and matter. Here, we investigate three-photon transmission spectra in a strongly coupled cavity polariton system and show that the correlation functions and transmitted photon stream can be optically manipulated. The dynamics of single photons and photon pairs at the polariton resonances can be changed by light from a single external coupling laser. At the "dark-state polariton," three-photon transmission is a perfectly coherent field in contrast to the strong photon-bunching behavior of a typical cavity quantum electrodynamics system. When the detuned probe light is tuned to the "bright polariton," the light exhibits a dramatic photon antibunching effect. Remarkably, the Fano-resonant asymmetric three-photon transmission caused by the interference between the dressed states leads to a new quantum feature that is strongly nonclassical (the third-order correlation function g((3))(0, 0) ≪ 1) and has a wide and tunable bandwidth. The dependence of the intrinsic third-order correlation and time symmetry of the photon stream on the controlled parameters is also examined. Strongly nonclassical, all-optically controllable multi-photon dynamics are very important for future quantum devices and metrology.