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Physical Review Letters

Laser Cooling without Repumping: A Magneto-Optical Trap for Erbium Atoms

Jabez J. McClelland, J. Hanssen

Published Apr 14, 2006• 197 citations
Publisher

Abstract

We report on a novel mechanism that allows for strong laser cooling of atoms that do not have a closed cycling transition. This mechanism is observed in a magneto-optical trap (MOT) for erbium, an atom with a very complex energy level structure with multiple pathways for optical-pumping losses. We observe surprisingly high trap populations of over 10(6) atoms and densities of over 10(11) atoms cm(-3), despite the many potential loss channels. A model based on recycling of metastable and ground state atoms held in the quadrupole magnetic field of the trap explains the high trap population, and agrees well with time-dependent measurements of MOT fluorescence. The demonstration of trapping of a rare-earth atom such as erbium opens a wide range of new possibilities for practical applications and fundamental studies with cold atoms.

DOI
10.1103/physrevlett.96.143005

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We report on a novel mechanism that allows for strong laser cooling of atoms that do not have a closed cycling transition. This mechanism is observed in a magneto-optical trap (MOT) for erbium, an atom with a very complex energy level structure with multiple pathways for optical-pumping losses. We observe surprisingly high trap populations of over 10(6) atoms and densities of over 10(11) atoms cm(-3), despite the many potential loss channels. A model based on recycling of metastable and ground state atoms held in the quadrupole magnetic field of the trap explains the high trap population, and agrees well with time-dependent measurements of MOT fluorescence. The demonstration of trapping of a rare-earth atom such as erbium opens a wide range of new possibilities for practical applications and fundamental studies with cold atoms.
Laser cooling and trapping of heavy alkaline-earth element barium have been demonstrated for the first time ever. For any possible cycling transition in barium that could provide strong cooling forces, the excited state has a very large branching probability to metastable states. Additional lasers are thus needed to bring the atoms back in to the cooling cycle. In this work barium atoms were efficiently collected in a magneto-optical trap (MOT) by large optical forces from the strong 6s2 1S0 – 6s6p 1P1 transition. Trapping of barium has been achieved using up to seven lasers simultaneously. The properties of the barium MOT were characterized. The efficiency of capturing an atom from a thermal atomic beam into the MOT is 0.4(1) %. The developed scheme is very efficient for collecting atoms. Loss rate mechanisms from the trap were studied by observing the decay of the trap population. Typical lifetimes of the MOT cloud are on the order of one second and are limited mainly due to insufficient repumping of metastable states. The range of velocities from which barium atoms can be captured into the MOT is about 30 m/s. Different laser transitions were employed for repumping barium atoms from the 6s5d 3D1 and the 6s5d 3D2 states. They lead to similar trap populations and lifetimes. The temperature of the cold atomic barium cloud was determined to about 5 mK. Atomic properties of the 5d2 3F2 state were studied with trapped atoms, in particular it's lifetime was determined as 160(10) s. This work has shown a possible scheme to trap atoms with a leaky cooling cycle. Since atoms with such properties are the majority of the elements in the periodic table, the number of optically trapable elements can be significantly enlarged. Of particular high interest is radium, which is chemical homologue to barium. The interest in radium stems from it's high sensitivity to possible nuclear and electron permanent electric dipole moments (EDM's). An EDM violates parity as well as time reversal and is therefore of fundamental importance. Searches for such EDM's are among the main research goals of the recently commissioned TRImP facility at KVI.
Laser cooling on weak transitions is a useful technique for reaching ultracold temperatures in atoms with multiple valence electrons. However, for strongly magnetic atoms a conventional narrow-line magneto-optical trap (MOT) is destabilized by competition between optical and magnetic forces. We overcome this difficulty in Er by developing an unusual narrow-line MOT that balances optical and magnetic forces using laser light tuned to the blue side of a narrow (8 kHz) transition. The trap population is spin polarized with temperatures reaching below 2 muK. Our results constitute an alternative method for laser cooling on weak transitions, applicable to rare-earth-metal and metastable alkaline earth elements.
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We demonstrate sub-Doppler laser cooling and magneto-optical trapping of the rare earth element Holmium. Atoms are loaded from an atomic beam source and captured in six-beam σ+−σ−σ_+ - σ_-σ+​−σ−​ molasses using a strong J=15/2↔J=17/2J=15/2 \leftrightarrow J=17/2J=15/2↔J=17/2 cycling transition at λ=410.5nmλ=410.5 \rm nmλ=410.5nm. Due to the small difference in hyperfine splittings and Landé ggg-factors in the lower and upper levels of the cooling transition the MOT is self-repumped without additional repump light, and deep sub-Doppler cooling is achieved with the magnetic trap turned on. We measure the leakage out of the cycling transition to metastable states and find a branching ratio ∼10−5\sim 10^{-5}∼10−5 which is adequate for state resolved measurements on hyperfine encoded qubits.
We demonstrate laser cooling and magneto-optical trapping of europium. The atoms are optically pumped to a metastable state and then loaded from an atomic-beam source via conventional Zeeman slowing and magneto-optical trapping techniques using a $J=13/2\ensuremath{\leftrightarrow}J=15/2$ quasicyclic transition. The trapped populations contained up to $1\ifmmode\times\else\texttimes\fi{}{10}^{7}$ atoms, and a two-body loss rate is estimated as $1\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}10}\phantom{\rule{0.28em}{0ex}}{\mathrm{cm}}^{3}/\mathrm{s}$ from the nonexponential loss of atoms at high densities. We also observed leakage out of the quasicyclic transition to the two metastable states with J=9/2J=9/2J=9/2 and 11/211/211/2, which is adequate to pump the laser-cooled atoms back to the J=7/2J=7/2J=7/2 ground state.
We report the measurement of one-body loss rates for magnetically trapped metastable europium atoms and the study of their loss mechanism. The loss of atoms observed in a magneto-optical trap is not fully understood because of the indivisibility of the loss regarding optical pumpings due to the presence of cooling laser beams. We magnetically trap the atoms by directly loading from the magneto-optical trap and observe almost identical one-body loss rates of approximately 2.6 s−12.6\,\mathrm{s^{-1}}2.6s−1 for two isotopes: 151Eu\mathrm{{}^{151}Eu}151Eu and 153Eu\mathrm{{}^{153}Eu}153Eu. Our rate-equation-based model, combined with loss rate measurements carried out with repumpers, shows that blackbody radiation at room temperature drives E1 transitions and induces the observed losses.