A two-level atom illuminated by a laser may be driven into a population-inverted steady state if it is coupled to a cavity. This is a result of the quantum nature of the electromagnetic field and is forbidden by the semiclassical theory. We numerically and analytically analyze this inversion. We find the maximum possible inversion and determine the rate of approach to the steady state. The quantized cavity modifies the electromagnetic vacuum seen by the atom; this connects our work to that on cavity-enhanced spontaneous emission and on dynamical line narrowing. Experimental signatures of the inversion and potential experimental difficulties are considered. For example, neither the presence of many atoms in the mode nor many modes in the cavity destroys the inversion.
Placing an optical cavity around a two-level atom modifies the electromagnetic vacuum to which it couples. Effects such as inhibited and enhanced spontaneous emission are known to result. Recently one of us predicted a new nonclassical effect of vacuum engineering.1 A two-level transition may be laser driven into an inverted steady state. Semiclassical theory forbids this fully quantum mechanical result. Unlike squeezing and antibunching, this inversion is not a property of the linearized quantum fluctuations. We present numerical and analytical results which clarify the physics of the inversion. The maximum inversion possible is determined. We attempt to identify obstacles to the experimental realization of steady-state inversion. Multiple atoms and multiple cavity modes do not destroy the effect. A significant difficulty appears to be localizing the atoms at the cavity beamwaist until they reach steady state. The inversion may be observed via fluorescence changes as the cavity is blocked and unblocked or via the presence of a fluoresence maximum as a function of the driving field intensity.
We study the coupled translational, electronic, and field dynamics of the combined system "a two-level atom + a single-mode quantized field + a standing-wave ideal cavity". We derive Hamilton -- Schr\\"odinger equations for probability amplitudes and averaged position and momentum of a point-like atom interacting with the quantized field in a standing-wave cavity. They constitute, in general, an infinite-dimensional set of equations with an infinite number of integrals of motion which may be reduced to a dynamical system with four degrees of freedom if the quantized field is supposed to be initially prepared in a Fock state. This system is found to produce semiquantum chaos with positive values of the maximal Lyapunov exponent. At large values of detuning
∣delta∣gg1, the Rabi atomic oscillations are usually shallow, and the dynamics is found to be almost regular. The Doppler -- Rabi resonance, deep Rabi oscillations that may occur at any large value of
∣delta∣ to be equal to
∣alphap0∣, is found numerically and described analytically (with
alpha to be the normalized recoil frequency and
p0 the initial atomic momentum). Two gedanken experiments are proposed to detect manifestations of semiquantum chaos in real experiments. In the chaotic regime values of the population inversion
zout, measured with atoms after transversing a cavity, are so sensitive to small changes in the initial inversion
zin that the probability of detecting any value of
zout in the admissible interval becomes almost unity in a short time. Chaotic wandering of a two-level atom in a quantized Fock field is shown to be fractal. Fractal-like structures, typical for chaotic scattering, are numerically found in the dependence of the time of exit of atoms from the cavity on their initial momenta.
We study the stochastic dynamics of the electromagnetic field in a lossless cavity interacting with a beam of two-level atoms, given that the atomic states are measured after they have crossed the cavity. The atoms first interact at the exit of the cavity with a classical laser field ℰ and then enter into a detector which measures their states. Each measurement disentangles the field and the atoms and changes in a random way the state |ψ(t)〉 of the cavity field. For weak atom-field coupling, the evolution of |ψ(t)〉 when many atoms cross the cavity and the detector is characterized by a succession of quantum jumps occurring at random times, separated by quasi-Hamiltonian evolutions, both of which depend on the laser field ℰ. For ℰ=0, the dynamics is the same as in the Monte Carlo wave function model of Dalibard et al. [Phys. Rev. Lett. 68, 580 (1992)] and Carmichael, An Open System Approach to Quantum Optics, Lecture Notes in Physics Vol. 18 (Springer, Berlin, 1991)]. The density matrix of the quantum field, obtained by averaging the projector |ψ(t)〉〈ψ(t)| over all results of the measurements, is independent of ℰ and follows the master equation of the damped harmonic oscillator at finite temperature. We provide numerical evidence showing that for large ℰ, an arbitrary initial field state |ψ(0)〉 evolves under the monitoring of the atoms and the measurements toward squeezed states |α,re2iφ〉, moving in the α-complex plane but with almost constant squeezing parameters r and φ. The values of r and φ are determined analytically. On the other hand, for ℰ=0, the dynamics transforms the initial state into Fock states |n〉 with fluctuating numbers of photons n, as shown in Kist et al. [J. Opt. B: Quantum Semiclassical Opt. 1, 251 (1999)]. In the last part, we derive the quantum jump dynamics from the linear quantum jump model proposed in Spehner and Bellissard [J. Stat. Phys. 104, 525 (2001)], for arbitrary open quantum systems having a Lindblad-type evolution. A careful derivation of the infinite jump rates limit, where the dynamics can be approximated by a diffusion process of the quantum state, is also presented.
The quantum mechanical master equation for a single two-level atom in a single-mode optical cavity is numerically solved in both the quantum and the semiclassical limits. The quantum limit of few cavity photons shows semiclassically forbidden behaviour such as steady state two-level population inversion. Qualitatively new fluorescent spectra, having sidebands broadened by the cavity interaction, also occur. The quantum theory of the single-atom laser with injected signal is presented. At the interface between its quantum and semiclassical dynamics we elucidate the signature of semiclassical limit cycles.
An exact solution for the problem of two two-level atoms interacting with a single-mode detuned quantized radiation field is presented. On resonance, an asymptotic result is derived for large coherent initial fields. It is shown that when the atoms are initially prepared in one of the semiclassical eigenstates, the atom-plus-field wavefunction remains almost factored into an atomic and a field part throughout the interaction. Under certain conditions, the atomic part evolves into a unique pure state at half-revival time. The effects of the cavity detuning on the dynamics of the atomic level occupation probabilities and emission spectra are studied. It is found, for non-symmetrical excitation, that far off-resonance the field acts like a virtual level by means of which the energy is transferred between the atoms. Due to non-zero detuning, nine-peaked spectra are observed and are given a clear explanation from the dressed-state viewpoint. It is established that in the case of symmetrical excitation, the intensity of the emission spectrum is two times larger than that in the case of non-symmetrical excitation.