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Journal of Physics B Atomic and Molecular Physics

Deflection of an atomic beam by a laser wave: transition between diffractive and diffusive regimes

Christian Tanguy, Serge Reynaud, Claude N. Cohen-Tannoudji

Published Dec 14, 1984• 72 citations
Publisher

Abstract

The exchange of momentum between atoms and photons in a deflection experiment is usually described by different formalisms depending on whether the interaction time T is shown or long compared with the radiative lifetime tau R . The authors present a new approach to this problem leading to a single theoretical expression valid in both limits and therefore allowing the transition between them to be studied. They interpret in this way the resonant Kapitza-Dirac effect and the optical Stern and Gerlach effect appearing in the short-time limit (T<< tau R ) as well as the deflection profiles usually deduced from a Fokker-Planck equation in the long-time limit (T>> tau R ). The transition between these two regimes is interpreted in terms of momentum transfer due to absorption and stimulated emission of laser photons, convoluted by the distribution of recoil due to spontaneously emitted photons.

DOI
10.1088/0022-3700/17/23/009

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The exchange of momentum between atoms and photons in a deflection experiment is usually described by different formalisms depending on whether the interaction time T is shown or long compared with the radiative lifetime tau R . The authors present a new approach to this problem leading to a single theoretical expression valid in both limits and therefore allowing the transition between them to be studied. They interpret in this way the resonant Kapitza-Dirac effect and the optical Stern and Gerlach effect appearing in the short-time limit (T<< tau R ) as well as the deflection profiles usually deduced from a Fokker-Planck equation in the long-time limit (T>> tau R ). The transition between these two regimes is interpreted in terms of momentum transfer due to absorption and stimulated emission of laser photons, convoluted by the distribution of recoil due to spontaneously emitted photons.
We have observed both diffractive and diffusive regimes in the transfer of momentum to an atomic beam by a standing-wave radiation field. The momentum transfer was measured by passing a well-collimated beam of sodium atoms through a focused standing-wave laser waist. A narrow velocity distribution beam was obtained by utilizing a supersonic expansion and a two-state system was realized by optically pumping the beam prior to the interaction. The transverse momentum transferred to the atomic beam by the radiation field was measured by scanning a detector downstream from the interaction. The overall momentum resolution of the apparatus is less than the momentum of a single photon. The transition from diffractive to diffusive behavior is associated with an increase in the average number of spontaneous decays occurring during the interaction. In the diffractive regime, spontaneous decay is insignificant and momentum transfer proceeds by pairs of absorption/stimulated emission processes. This produces momentum exchange quantized in even multiples of photon momentum, the so-called Kapitza-Dirac effect; the deflection patterns show oscillatory structure. In the diffusive regime, spontaneous decay is important and causes fluctuations in the radiative forces. In addition, the recoil distribution associated with spontaneous decay results in a washing out of the diffraction peaks associated with stimulated processes, resulting in a smooth deflection pattern.
Momentum transfer to atoms by a standing light wave is measured in the presence of spontaneous decay. As the number of spontaneous decays is increased, the well-known Kapitza-Dirac diffractive structure observed in the absence of spontaneous decay evolves into a smooth diffusive pattern. Theoretical treatments based on a diffusive model adequately describe the rms momentum transfers and the envelopes of the momentum distributions. However, we observe significant persistence of diffractive structure at our long interaction times and find that details of the deflection profiles are accurately predicted only when several spontaneous decays occur during the interaction.
We investigate to which extent the quantum nature of light modifies laser-induced atomic beam deflection in a plane standing wave. Our model considers a single two-level atom interacting with a single quantized standing wave mode of the electromagnetic field. We neglect spontaneous emission into other field modes, an approximation valid for short enough times. We find that there is an essential qualitative difference between the cases of a coherent field and a thermal field. For a coherent field, the atomic momentum distribution after interaction has two symmetric peaks on the wings and resembles the semiclassical result of Arimondo et al. [Phys. Rev. A 24, 898 (1981)]. For a thermal field, this distribution has its maximum at p = 0. It is characterized by a constant contribution at p = 0, some sharp interference features, and near-Gaussian wings. The only feature common to both cases is that in the Raman-Nath regime of scattering, the range on transverse momenta grows linearly with time at a rate proportional to 〈 n 〉 , where 〈 n 〉 is the mean number of photons in the field.
Deflection of an atom due to momentum transfer from a strong resonant standing electromagnetic wave is investigated theoretically in the limit of short atom-field interaction time. The translational and internal motions of the atom are treated quantum mechanically, while the field is treated classically. It is shown that momentum transfer from a standing wave to an atom proceeds at the induced or Rabi rate, rather than the spontaneous rate characteristic of radiation pressure. In a typical case, atomic deflections of order 1\ifmmode^\circ\else\textdegree\fi{} are achieved with 106{10}^{6}106 W/cm2{\mathrm{cm}}^{2}cm2 field intensity in a time less than the natural lifetime of the excited atom.
We have observed momentum transfer from a standing-wave light field to an atomic beam. The atomic beam is split symmetrically into two peaks whose separation increases with field strength. The short interaction time ensures that this deflection is due to induced forces; these are described using a semiclassical dressed-atom treatment, which gives good agreement with the data. In addition to the splitting, we have observed diffraction of the atomic beam due to the exchange of even numbers of photons with the field.